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arXiv:2202.03860 · Physical Review Research

Quantum spin liquids of Rydberg excitations in a honeycomb lattice induced by density-dependent Peierls phases

Simon Ohler, Maximilian Kiefer-Emmanouilidis, Michael Fleischhauer

Published Feb 28, 2023• 11 citations
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Abstract

We show that the nonlinear transport of bosonic excitations in a two-dimensional honeycomb lattice of spin-orbit-coupled Rydberg atoms gives rise to disordered quantum phases which are topological and may be candidates for quantum spin liquids. As recently demonstrated by Lienhard et al. [Phys. Rev. X 10, 021031 (2020)] the spin-orbit coupling breaks time-reversal and chiral symmetries and leads to a tunable density-dependent complex hopping of spin excitations which behave as hard-core bosons. Using exact diagonalization (ED), we numerically investigate the phase diagram resulting from the competition between density-dependent and direct transport terms as well as density-density interactions. In mean-field approximation there is a phase transition from a condensate to a ${120}^{\ensuremath{\circ}}$ phase when the amplitude of the complex hopping exceeds that of the direct one. In the full model a new phase emerges close to the mean-field critical point as a result of quantum correlations induced by the density dependence of the complex hopping. We show that without density-density interactions this phase is a genuine disordered one, has large spin chirality, and is characterized by a nontrivial many-body Chern number. The Chern number is found to be robust to disorder. ED simulations of small lattices with up to 30 lattice sites give indications for a nondegenerate ground state with finite spin and collective gaps and thus for a bosonic integer quantum Hall phase, protected by $\mathrm{U}(1)$ symmetry. On the other hand, while staying finite, the many-body gap varies substantially when different twisted boundary conditions are applied, which points to a gapless phase. For very strong negative nonlinear hopping amplitudes we find another disordered regime with vanishing spin gap. This phase also has a large spin chirality and could be a gapless spin liquid but lies outside the parameter regime experimentally accessible in the Rydberg system.

DOI
10.1103/physrevresearch.5.013157

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We show that the nonlinear transport of bosonic excitations in a two-dimensional honeycomb lattice of spin-orbit-coupled Rydberg atoms gives rise to disordered quantum phases which are topological and may be candidates for quantum spin liquids. As recently demonstrated by Lienhard et al. [Phys. Rev. X 10, 021031 (2020)] the spin-orbit coupling breaks time-reversal and chiral symmetries and leads to a tunable density-dependent complex hopping of spin excitations which behave as hard-core bosons. Using exact diagonalization (ED), we numerically investigate the phase diagram resulting from the competition between density-dependent and direct transport terms as well as density-density interactions. In mean-field approximation there is a phase transition from a condensate to a 120\ensuremath∘{120}^{\ensuremath{\circ}}120\ensuremath∘ phase when the amplitude of the complex hopping exceeds that of the direct one. In the full model a new phase emerges close to the mean-field critical point as a result of quantum correlations induced by the density dependence of the complex hopping. We show that without density-density interactions this phase is a genuine disordered one, has large spin chirality, and is characterized by a nontrivial many-body Chern number. The Chern number is found to be robust to disorder. ED simulations of small lattices with up to 30 lattice sites give indications for a nondegenerate ground state with finite spin and collective gaps and thus for a bosonic integer quantum Hall phase, protected by U(1)\mathrm{U}(1)U(1) symmetry. On the other hand, while staying finite, the many-body gap varies substantially when different twisted boundary conditions are applied, which points to a gapless phase. For very strong negative nonlinear hopping amplitudes we find another disordered regime with vanishing spin gap. This phase also has a large spin chirality and could be a gapless spin liquid but lies outside the parameter regime experimentally accessible in the Rydberg system.
We derive a parton mean-field Hamiltonian for Rydberg excitations on a honeycomb lattice with nearest and density-dependent, complex next-nearest neighbor hopping. Numerical results obtained from exact diagonalization of small systems have given indications for a ground state that is a chiral spin liquid (CSL) []. Here we provide further evidence for this. Calculating the ground-state wavefunction self-consistently, we show that the mean-field Hamiltonian fulfills the requirements for a CSL ground state, resulting from a projected symmetry group classification and verify the expected twofold topological degeneracy on a torus. Furthermore we find very good overlap with the ground-state wavefunctions obtained by exact diagonalization of the original Hamiltonian.
We theoretically investigate, within Schwinger-boson mean-field theory, the transition from a gapped Z2{\mathbb{Z}}_{2}Z2​ quantum spin liquid, in a ${J}_{1}\text{\ensuremath{-}}{J}_{2}$ Heisenberg spin-12\frac{1}{2}21​ system in a honeycomb lattice, to a chiral Z2{\mathbb{Z}}_{2}Z2​ spin-liquid phase under the presence of time-reversal symmetry-breaking scalar chiral interaction (with amplitude ${J}_{\ensuremath{\chi}}$). We numerically obtain a phase diagram of this ${J}_{1}\text{\ensuremath{-}}{J}_{2}\text{\ensuremath{-}}{J}_{\ensuremath{\chi}}$ system, where different ground states are distinguished based on the gap and the nature of excitation spectrum, topological invariant of the excitations, the nature of spin-spin correlation, and the symmetries of the mean-field parameters. The chiral Z2{\mathbb{Z}}_{2}Z2​ state is characterized by the nontrivial Chern number of the excitation bands and lack of long-range magnetic order, which leads to a large thermal Hall coefficient.
We investigate the nature of quantum phases arising in chiral interacting Hamiltonians recently realized in Rydberg atom arrays. We classify all possible fermionic chiral spin liquids with U(1)\mathrm{U}(1)U(1) global symmetry using parton construction on the honeycomb lattice. The resulting classification includes six distinct classes of gapped quantum spin liquids: the corresponding variational wavefunctions obtained from two of these classes accurately describe the Rydberg many-body ground state at 1/21/21/2 and 1/41/41/4 particle density. Complementing this analysis with tensor network simulations, we conclude that both particle filling sectors host a spin liquid with the same topological order of a $\ensuremath{\nu}\phantom{\rule{0.16em}{0ex}}=\phantom{\rule{0.16em}{0ex}}1/2$ fractional quantum Hall effect. At density 1/21/21/2, our results clarify the phase diagram of the model, while at density 1/41/41/4, they provide an explicit construction of the ground-state wavefunction with almost unit overlap with the microscopic one. These findings pave the way to the use of parton wavefunctions to guide the discovery of quantum spin liquids in chiral Rydberg models.
Abstract Quantum spin liquids are elusive but paradigmatic examples of strongly correlated quantum states that are characterized by long-range quantum entanglement. Recently, signatures of a gapped topological Z2{{\mathbb{Z}}}_{2}Z2​ Z 2 spin liquid have been observed in a system of Rydberg atoms; however, the full capability of these platforms to realize quantum spin liquids extends far beyond this state alone. Here, we propose the realization of a different class of spin liquids in a honeycomb array of Rydberg atoms. Exploring the system’s quantum phase diagram using density-matrix renormalization group and exact diagonalization calculations, we identify several density-wave-ordered phases and a trimer spin liquid ground state with an emergent U(1) × U(1) local symmetry. This liquid state originates from superpositions of classical trimer configurations on the dual triangular lattice in the regime where third-nearest-neighbor atoms lie within the Rydberg blockade radius. Finally, we discuss the conditions to enhance the preparation fidelity of this state by a general Rydberg-blockade-based projection mechanism, test the robustness of the trimer spin liquid phase in a range of realistic parameters, and outline methods for its experimental detection.
Arrays of Rydberg atoms constitute a highly tunable, strongly interacting venue for the pursuit of exotic states of matter. We develop a strategy for accessing a family of fractionalized phases known as quantum spin liquids in two-dimensional Rydberg arrays. We specifically use effective field theory methods to study arrays assembled from Rydberg chains tuned to an Ising phase transition that famously hosts emergent fermions propagating within each chain. This highly entangled starting point allows us to naturally access spin liquids familiar from Kitaev's honeycomb model---albeit from an entirely different framework. In particular, we argue that finite-range repulsive Rydberg interactions, which frustrate nearby symmetry-breaking orders, can enable coherent propagation of emergent fermions between the chains in which they were born. Delocalization of emergent fermions across the full two-dimensional Rydberg array yields a gapless Z2{\mathbb{Z}}_{2}Z2​ spin liquid with a single massless Dirac cone. Here, the Rydberg occupation numbers exhibit universal power-law correlations that provide a straightforward experimental diagnostic of this phase. We further show that explicitly breaking symmetries perturbs the gapless spin liquid into gapped, topologically ordered descendants: Breaking lattice symmetries generates toric-code topological order, whereas introducing Floquet-mediated chirality generates non-Abelian Ising topological order. In the toric-code phase, we analytically construct microscopic incarnations of non-Abelian defects, which can be created and transported by dynamically controlling the atom positions in the array. Our work suggests that appropriately tuned Rydberg arrays provide a cold-atoms counterpart of solid-state ``Kitaev materials'' and, more generally, it spotlights a different angle for pursuing experimental platforms for Abelian and non-Abelian fractionalization.
We show that resonant dipole–dipole interactions between Rydberg atoms in a triangular lattice can give rise to artificial magnetic fields for spin excitations. We consider the coherent dipole–dipole coupling between np and ns Rydberg states and derive an effective spin-1/2 Hamiltonian for the np excitations. By breaking time-reversal symmetry via external fields, we engineer complex hopping amplitudes for transitions between two rectangular sub-lattices. The phase of these hopping amplitudes depends on the direction of the hop. This gives rise to a staggered, artificial magnetic field which induces non-trivial topological effects. We calculate the single-particle band structure and investigate its Chern numbers as a function of the lattice parameters and the detuning between the two sub-lattices. We identify extended parameter regimes where the Chern number of the lowest band is C=1C=1C=1 or C=2C=2C=2 .