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arXiv:2104.04119 · Science

Probing topological spin liquids on a programmable quantum simulator

Giulia Semeghini, Harry Levine, Alexander Keesling, Sepehr Ebadi, Tout T. Wang, Dolev Bluvstein, Ruben Verresen, Hannes Pichler, M. W. Kalinowski, Rhine Samajdar, Ahmed Omran, Subir Sachdev A, Ashvin Vishwanath, Markus Greiner, Vladan Vuletić, Mikhail D. Lukin

Published Dec 2, 2021• 778 citations
arXivHTMLPDF

Abstract

Quantum spin liquids, exotic phases of matter with topological order, have been a major focus in physics for the past several decades. Such phases feature long-range quantum entanglement that can potentially be exploited to realize robust quantum computation. We used a 219-atom programmable quantum simulator to probe quantum spin liquid states. In our approach, arrays of atoms were placed on the links of a kagome lattice, and evolution under Rydberg blockade created frustrated quantum states with no local order. The onset of a quantum spin liquid phase of the paradigmatic toric code type was detected by using topological string operators that provide direct signatures of topological order and quantum correlations. Our observations enable the controlled experimental exploration of topological matter and protected quantum information processing.

DOI
10.1126/science.abi8794

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Quantum spin liquids, exotic phases of matter with topological order, have been a major focus in physics for the past several decades. Such phases feature long-range quantum entanglement that can potentially be exploited to realize robust quantum computation. We used a 219-atom programmable quantum simulator to probe quantum spin liquid states. In our approach, arrays of atoms were placed on the links of a kagome lattice, and evolution under Rydberg blockade created frustrated quantum states with no local order. The onset of a quantum spin liquid phase of the paradigmatic toric code type was detected by using topological string operators that provide direct signatures of topological order and quantum correlations. Our observations enable the controlled experimental exploration of topological matter and protected quantum information processing.
Quantum phases with topological order, such as quantum spin liquids, have been the focus of explorations for several decades. Such phases feature a number of remarkable properties including long-range quantum entanglement. Moreover, they can be potentially exploited for the realization of robust quantum computation, as exemplified by the paradigmatic toric code model. While some indications that such phases may be present in frustrated condensed matter systems have been previously reported, so far quantum spin liquids have eluded direct experimental detection. In this talk, I will show how a programmable quantum simulator based on Rydberg atom arrays can be used to realize and probe quantum spin liquid states. In our approach, atoms are placed on the links of a kagome lattice and coherent evolution under Rydberg blockade enables the transition into frustrated quantum states with no local order. We detect the onset of a quantum spin liquid phase of the toric code type by measuring topological string operators in two complementary bases. The properties of this state are further revealed using a lattice with non-trivial topology, representing a step towards the realization of a topological qubit. Our observations open the door to the controlled experimental exploration of topological quantum matter, and could enable the investigation of new methods for topologically protected quantum information processing.
Dual-species arrays of ultracold neutral atoms have recently attracted increased interest due to the ability to independently control different atomic species and tune the interatomic interactions. This capability provides additional flexibility essential for both quantum computing and quantum simulation. In this work we theoretically investigate a quantum spin liquid (QSL) state to be simulated on a programmable quantum simulator based on a dual-species atomic array, arranged on a Kagome lattice. The Kagome lattice is formed by corner sharing triangles. This specific spatial arrangement enhances the competing interactions between atoms and is often considered as a model for realizing QSL states. When the atoms are excited into Rydberg states, long-range interactions result in Rydberg blockade. The geometric frustration of the Kagome lattice, combined with the Rydberg blockade, drives the system into exotic phases with topological order and long-range entanglement. To drive an array into the QSL state, we use a sweep-hold-sweep protocol, when the atoms are quasi-adiabatically excited into Rydberg state with individually controlled detuning from the resonance for each atomic species. The filling fraction, indicating emergence of a QSL state, is represented by a density of Rydberg excitations. We identified the conditions required for QSL state in a dual-species array with non-uniform interaction energies. We calculated the correlation length and studied the mutual information as a function of the size of the subset of the system. The existence of a topological order was proved by estimating the Kitaev-Preskill topological quantum entanglement entropy, and further confirmed by evaluating diagonal and off-diagonal topological string operators, which respectively probe the classical dimer-covering structure and the quantum coherence between distinct dimer configurations.
Understanding topological matter is an outstanding challenge across several disciplines of physical science.Programmable quantum simulators have emerged as a powerful approach to studying such systems.While quantum spin liquids of paradigmatic toric code type have recently been realized in the laboratory, controlled exploration of topological phases with non-Abelian excitations remains an open problem.We introduce and analyze a new approach to simulating topological matter based on periodic driving.Specifically, we describe a model for a so-called Floquet spin liquid, obtained through a periodic sequence of parallel quantum gate operations that effectively simulates the Hamiltonian of the non-Abelian spin liquid in Kitaev's honeycomb model.We show that this approach, including the toolbox for preparation, control, and readout of topological states, can be efficiently implemented in state-of-the-art experimental platforms.One specific implementation scheme is based on Rydberg atom arrays and utilizes recently demonstrated coherent qubit transport combined with controlled-phase gate operations.We describe methods for probing the non-Abelian excitations, and the associated Majorana zero modes, and simulate possible fusion and braiding experiments.Our analysis demonstrates the potential of programmable quantum simulators for exploring topological phases of matter.Extensions including simulation of Kitaev materials and lattice gauge theories are also discussed.
Abstract Quantum spin liquids are elusive but paradigmatic examples of strongly correlated quantum states that are characterized by long-range quantum entanglement. Recently, signatures of a gapped topological Z2{{\mathbb{Z}}}_{2}Z2​ Z 2 spin liquid have been observed in a system of Rydberg atoms; however, the full capability of these platforms to realize quantum spin liquids extends far beyond this state alone. Here, we propose the realization of a different class of spin liquids in a honeycomb array of Rydberg atoms. Exploring the system’s quantum phase diagram using density-matrix renormalization group and exact diagonalization calculations, we identify several density-wave-ordered phases and a trimer spin liquid ground state with an emergent U(1) × U(1) local symmetry. This liquid state originates from superpositions of classical trimer configurations on the dual triangular lattice in the regime where third-nearest-neighbor atoms lie within the Rydberg blockade radius. Finally, we discuss the conditions to enhance the preparation fidelity of this state by a general Rydberg-blockade-based projection mechanism, test the robustness of the trimer spin liquid phase in a range of realistic parameters, and outline methods for its experimental detection.
Recent atomic physics experiments and numerical works have reported complementary signatures of the emergence of a topological quantum spin liquid in models with blockade interactions. However, the specific mechanism stabilizing such a phase remains unclear. Here, we introduce an exact relation between an Ising-Higgs lattice gauge theory on the kagome lattice and blockaded models on Ruby lattices. This relation elucidates the origin of previously observed topological spin liquids by directly linking the latter to a deconfined phase of a solvable gauge theory. By means of exact diagonalization and unbiased quantum Monte Carlo simulations, we show that the deconfined phases extend in a broad region of the parameter space; these states are characterized by a large ground state overlap with resonating valence bond wave functions. These blockaded models include both creation or annihilation and hopping dynamics, and can be experimentally realized with Rydberg-dressed atoms, offering novel and controllable platforms for the engineering and characterization of spin liquid states.
Arrays of Rydberg atoms constitute a highly tunable, strongly interacting venue for the pursuit of exotic states of matter. We develop a strategy for accessing a family of fractionalized phases known as quantum spin liquids in two-dimensional Rydberg arrays. We specifically use effective field theory methods to study arrays assembled from Rydberg chains tuned to an Ising phase transition that famously hosts emergent fermions propagating within each chain. This highly entangled starting point allows us to naturally access spin liquids familiar from Kitaev's honeycomb model---albeit from an entirely different framework. In particular, we argue that finite-range repulsive Rydberg interactions, which frustrate nearby symmetry-breaking orders, can enable coherent propagation of emergent fermions between the chains in which they were born. Delocalization of emergent fermions across the full two-dimensional Rydberg array yields a gapless Z2{\mathbb{Z}}_{2}Z2​ spin liquid with a single massless Dirac cone. Here, the Rydberg occupation numbers exhibit universal power-law correlations that provide a straightforward experimental diagnostic of this phase. We further show that explicitly breaking symmetries perturbs the gapless spin liquid into gapped, topologically ordered descendants: Breaking lattice symmetries generates toric-code topological order, whereas introducing Floquet-mediated chirality generates non-Abelian Ising topological order. In the toric-code phase, we analytically construct microscopic incarnations of non-Abelian defects, which can be created and transported by dynamically controlling the atom positions in the array. Our work suggests that appropriately tuned Rydberg arrays provide a cold-atoms counterpart of solid-state ``Kitaev materials'' and, more generally, it spotlights a different angle for pursuing experimental platforms for Abelian and non-Abelian fractionalization.