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arXiv:2210.01174 · Physical review. B./Physical review. B

Two-dimensional polaron spectroscopy of Fermi superfluids

Ivan Amelio

Published Mar 30, 2023• 9 citations
arXivHTMLPDF

Abstract

Multidimensional spectroscopy is becoming an increasingly popular tool and there is an ongoing effort to access electronic transitions and many-body dynamics in correlated materials. We apply the protocol recently proposed by Wang [Phys. Rev. A 107, 013305 (2023)] to extract two-dimensional polaron spectra in a Fermi superfluid with an impurity. The bath is described by a BCS ansatz and it assumed that the impurity can scatter at most one quasiparticle pair. The spectral response contains a symmetric contribution, which carries the same information as Ramsey spectra, and an asymmetric one. While a priori it may seem promising to probe the quasiparticle gap from the asymmetric contribution, we show explicitly that this is not the case and, in the absence of incoherent processes, multidimensional spectroscopy does not bring much additional information. Our calculation is suitable for ultracold gases, but we discuss implications for exciton polarons in two-dimensional materials.

DOI
10.1103/physrevb.107.104519

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Multidimensional spectroscopy is becoming an increasingly popular tool and there is an ongoing effort to access electronic transitions and many-body dynamics in correlated materials. We apply the protocol recently proposed by Wang [Phys. Rev. A 107, 013305 (2023)] to extract two-dimensional polaron spectra in a Fermi superfluid with an impurity. The bath is described by a BCS ansatz and it assumed that the impurity can scatter at most one quasiparticle pair. The spectral response contains a symmetric contribution, which carries the same information as Ramsey spectra, and an asymmetric one. While a priori it may seem promising to probe the quasiparticle gap from the asymmetric contribution, we show explicitly that this is not the case and, in the absence of incoherent processes, multidimensional spectroscopy does not bring much additional information. Our calculation is suitable for ultracold gases, but we discuss implications for exciton polarons in two-dimensional materials.
We calculate the exact spectral function of a single impurity repulsively interacting with a bath of fermions in one-dimensional lattices, by deriving the explicit expression of the form factor for both regular Bethe states and the irregular spin-flip state and η-pairing state, based on the exactly solvable one-dimensional Hubbard model. While at low impurity momentum Q∼0 the spectral function is dominated by two power-law Fermi singularities, at large momentum we observe that the two singularities develop into two-sided distributions and eventually become anomalous Fermi singularities at the boundary of the Brillouin zone (i.e., Q=±π), with the power-law tails extending toward low energy. Near the quarter filling of the Fermi bath, we also find two broad polaron peaks at large impurity momentum, collectively contributed by many excited many-body states with non-negligible form factors. Our exact results of those distinct features in one-dimensional Fermi polarons, which have no correspondences in two and three dimensions, could be readily probed in cold-atom laboratories by trapping highly imbalanced two-component fermionic atoms into one-dimensional optical lattices.
We have developed a microscopic many-body theory of two-dimensional coherent spectroscopy (2DCS) for a model of polarons in one-dimensional (1D) materials. Our theory accounts for contributions from all three processes: excited-state emission (ESE), ground-state bleaching (GSB), and excited-state absorption (ESA). While the ESE and GSB contributions can be accurately described using Chevy's ansatz with one-particle-hole excitation, the ESA process requires information about the many-body eigenstates involving two impurities. To calculate these double polaron states, we have extended Chevy's ansatz with one-particle-hole excitation. The validity of this ansatz was verified by comparing our results with an exact calculation using Bethe's ansatz. Our numerical results reveal that in, the weak interaction limit, the ESA contribution cancels out the total ESE and GSB contributions, resulting in less significant spectral features. However, for strong interactions, the features of the ESA contribution and the combined ESE and GSB contributions remain observable in the 2DCS spectra. These features provide valuable information about the interactions between polarons. Additionally, we have investigated the mixing time dynamics, which characterize the quantum coherences of the polaron resonances. Overall, our theory provides a comprehensive framework for understanding and interpreting the 2DCS spectra of polarons in 1D materials, shedding light on their interactions and coherent dynamics.
We study polaron excitations induced by an impurity interacting with a two-dimensional p+ipp+ipp+ip Fermi superfluid. As the Fermi-Fermi pairing interaction is tuned, the background Fermi superfluid undergoes a topological phase transition. We show that such a transition is accompanied by a discontinuity in the second derivative of the polaron energy, regardless of the impurity-fermion interaction. We also identify a polaron to trimer crossover when the Fermi superfluid is in the strongly interacting, thus topologically trivial, regime. However, the trimer state is metastable against the molecular state where the impurity binds a Bogoliubov quasiparticle from the Fermi superfluid. By comparing the polaron to molecule transition in our system with that of an impurity in a noninteracting Fermi sea, we find that pairing interactions in the background Fermi superfluid effectively facilitate the impurity-fermion binding. Our results suggest the possibility of using the impurity as a probe for detecting topological phase transitions in the background; they also reveal interesting competitions between various many-body states in the system.
We study a type of Fermi polaron induced by an impurity interacting with an ultracold Fermi superfluid. Due to the three-component nature of the system, the polaron can become trimerlike with a nonuniversal energy spectrum. We identify multiple avoided crossings between impurity- and trimerlike solutions in both the attractive and the repulsive polaron spectra. In particular, the widths of avoided crossings gradually increase as the Fermi superfluid undergoes a crossover from the BCS side towards the Bose-Einstein condensate side, which suggests instabilities towards three-body losses. Such losses can be reduced for interaction potentials with small effective ranges. We also demonstrate, using the second-order perturbation theory, that the mean-field evaluation of the fermion-impurity interaction energy is inadequate even for small fermion-impurity scattering lengths, due to the essential effects of Fermi superfluid and short-range physics in such a system. Our results are practically useful for cold-atom experiments on mixtures.
We theoretically analyze inverse radio-frequency (rf) spectroscopy experiments in two-component Fermi gases. We consider a small number of impurity atoms interacting strongly with a bath of majority atoms. In two-dimensional geometries we find that the main features of the rf spectrum correspond to an attractive polaron and a metastable repulsive polaron. Our results suggest that the attractive polaron has been observed in a recent experiment [B. Fr\"ohlich et al., Phys. Rev. Lett. 106, 105301 (2011)].
We present a full microscopic many-body calculation of a recently-proposed nonlinear two-dimensional spectroscopy for Fermi polarons, and show that the quantum coherence between the attractive and repulsive polarons, which has never been experimentally examined, can be unambiguously revealed via quantum beats at the two off-diagonal crosspeaks in the two-dimensional spectrum. We predict that particle-hole excitations make the two crosspeaks asymmetric and lead to an additional side peak near the diagonal repulsive polaron peak. Our simulated spectra can be readily examined in future cold-atom experiments, where the two-dimensional spectroscopy is to be implemented by using a Ramsey interference sequence of rf pulses in the time domain. Our results also provide a first-principle understanding of the recent two-dimensional coherent spectroscopy of interacting excitons and trions in doped monolayer transition metal dichalcogenides.