Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:2207.14509

Two-dimensional spectroscopic diagnosis of quantum coherence in Fermi polarons

Jia Wang, Hui Hu, Xia-Ji Liu

Published Jul 29, 2022• 0 citations
arXivHTMLPDF

Abstract

We present a full microscopic many-body calculation of a recently-proposed nonlinear two-dimensional spectroscopy for Fermi polarons, and show that the quantum coherence between the attractive and repulsive polarons, which has never been experimentally examined, can be unambiguously revealed via quantum beats at the two off-diagonal crosspeaks in the two-dimensional spectrum. We predict that particle-hole excitations make the two crosspeaks asymmetric and lead to an additional side peak near the diagonal repulsive polaron peak. Our simulated spectra can be readily examined in future cold-atom experiments, where the two-dimensional spectroscopy is to be implemented by using a Ramsey interference sequence of rf pulses in the time domain. Our results also provide a first-principle understanding of the recent two-dimensional coherent spectroscopy of interacting excitons and trions in doped monolayer transition metal dichalcogenides.

DOI
10.48550/arxiv.2207.14509

Related papers

Microscopic many-body theory of two-dimensional coherent spectroscopy of exciton polarons in one-dimensional materials

Jia Wang, Hui Hu, Xia-Ji Liu

We have developed a microscopic many-body theory of two-dimensional coherent spectroscopy (2DCS) for a model of polarons in one-dimensional (1D) materials. Our theory accounts for contributions from all three processes: excited-state emission (ESE), ground-state bleaching (GSB), and excited-state absorption (ESA). While the ESE and GSB contributions can be accurately described using Chevy's ansatz with one-particle-hole excitation, the ESA process requires information about the many-body eigenstates involving two impurities. To calculate these double polaron states, we have extended Chevy's ansatz with one-particle-hole excitation. The validity of this ansatz was verified by comparing our results with an exact calculation using Bethe's ansatz. Our numerical results reveal that in, the weak interaction limit, the ESA contribution cancels out the total ESE and GSB contributions, resulting in less significant spectral features. However, for strong interactions, the features of the ESA contribution and the combined ESE and GSB contributions remain observable in the 2DCS spectra. These features provide valuable information about the interactions between polarons. Additionally, we have investigated the mixing time dynamics, which characterize the quantum coherences of the polaron resonances. Overall, our theory provides a comprehensive framework for understanding and interpreting the 2DCS spectra of polarons in 1D materials, shedding light on their interactions and coherent dynamics.

arXiv:2306.11998•Physical review. B./Physical review. B•May 13, 2024•0 citations

Two-dimensional polaron spectroscopy of Fermi superfluids

Ivan Amelio

Multidimensional spectroscopy is becoming an increasingly popular tool and there is an ongoing effort to access electronic transitions and many-body dynamics in correlated materials. We apply the protocol recently proposed by Wang [Phys. Rev. A 107, 013305 (2023)] to extract two-dimensional polaron spectra in a Fermi superfluid with an impurity. The bath is described by a BCS ansatz and it assumed that the impurity can scatter at most one quasiparticle pair. The spectral response contains a symmetric contribution, which carries the same information as Ramsey spectra, and an asymmetric one. While a priori it may seem promising to probe the quasiparticle gap from the asymmetric contribution, we show explicitly that this is not the case and, in the absence of incoherent processes, multidimensional spectroscopy does not bring much additional information. Our calculation is suitable for ultracold gases, but we discuss implications for exciton polarons in two-dimensional materials.

arXiv:2210.01174•Physical review. B./Physical review. B•Mar 30, 2023•9 citations

Fermi polarons in two dimensions

Richard Schmidt, Tilman Enss, Ville Pietilä +1 more

We theoretically analyze inverse radio-frequency (rf) spectroscopy experiments in two-component Fermi gases. We consider a small number of impurity atoms interacting strongly with a bath of majority atoms. In two-dimensional geometries we find that the main features of the rf spectrum correspond to an attractive polaron and a metastable repulsive polaron. Our results suggest that the attractive polaron has been observed in a recent experiment [B. Fr\"ohlich et al., Phys. Rev. Lett. 106, 105301 (2011)].

arXiv:1110.1649•Physical Review A•Feb 7, 2012•157 citations

Quantum Dynamics of Attractive and Repulsive Polarons in a Doped MoSe 2 Monolayer

Di Huang, Kevin Sampson, Yue Ni +11 more

When mobile impurities are introduced and coupled to a Fermi sea, new quasiparticles known as Fermi polarons are formed.There are two interesting, yet drastically different regimes of the Fermi polaron problem: (i) the attractive polaron (AP) branch connected to pairing phenomena spanning the crossover from BCS superfluidity to the Bose-Einstein condensation of molecules and (ii) the repulsive branch (RP), which underlies the physics responsible for Stoner's itinerant ferromagnetism.Here, we study Fermi polarons in two-dimensional systems, where many questions and debates regarding their nature persist.The model system we investigate is a doped MoSe 2 monolayer.We find the observed AP-RP energy splitting and the quantum dynamics of attractive polarons agree with the predictions of polaron theory.As the doping density increases, the quantum dephasing of the attractive polarons remains constant, indicative of stable quasiparticles, while the repulsive polaron dephasing rate increases nearly quadratically.The dynamics of Fermi polarons are of critical importance for understanding the pairing and magnetic instabilities that lead to the formation of rich quantum phases found in a wide range of physical systems including nuclei, cold atomic gases, and solids.

arXiv:2303.00907•Physical Review X•Mar 2, 2023•41 citations

Observation of Coherent Multiorbital Polarons in a Two-Dimensional Fermi Gas

Nelson Darkwah Oppong, Luis Riegger, Oscar Bettermann +5 more

We report on the experimental observation of multiorbital polarons in a two-dimensional Fermi gas of ^{173}Yb atoms formed by mobile impurities in the metastable ^{3}P_{0} orbital and a Fermi sea in the ground-state ^{1}S_{0} orbital. We spectroscopically probe the energies of attractive and repulsive polarons close to an orbital Feshbach resonance and characterize their coherence by measuring the quasiparticle residue. For all probed interaction parameters, the repulsive polaron is a long-lived quasiparticle with a decay rate more than 2 orders of magnitude below its energy. We formulate a many-body theory, which accurately treats the interorbital interactions in two dimensions and agrees well with the experimental results. Our work paves the way for the investigation of many-body physics in multiorbital ultracold Fermi gases.

arXiv:1901.09105•Physical Review Letters•May 17, 2019•75 citations

Variational approach to the Fermi polaron problem in two dimensions

Yi-Fan Qu, Pavel E. Dolgirev, Eugene Demler +1 more

We develop a non-Gaussian variational approach that enables us to study both equilibrium and far-from-equilibrium physics of the two-dimensional Fermi polaron. This method provides an unbiased analysis of the polaron-to-molecule phase transition without relying on truncations in the total number of particle-hole excitations. Our results—which include the ground-state energy and quasiparticle residue—are in qualitative agreement with the known Monte Carlo calculations. The main advantage of the non-Gaussian states compared to conventional numerical methods is that they enable us to explore long-time polaron evolution and, in particular, study various spectral properties accessible to both solid-state and ultracold atom experiments. We design two types of radiofrequency spectroscopies to measure polaronic and molecular spectral functions. Depending on the parameter regime, we find that these spectral functions and fermionic density profiles near the impurity either display long-lived oscillations between the repulsive and attractive polaron branches or exhibit fast relaxational dynamics to the molecular state.

arXiv:2209.10998•Physical Review Research•Mar 25, 2026•0 citations
We present a full microscopic many-body calculation of a recently-proposed nonlinear two-dimensional spectroscopy for Fermi polarons, and show that the quantum coherence between the attractive and repulsive polarons, which has never been experimentally examined, can be unambiguously revealed via quantum beats at the two off-diagonal crosspeaks in the two-dimensional spectrum. We predict that particle-hole excitations make the two crosspeaks asymmetric and lead to an additional side peak near the diagonal repulsive polaron peak. Our simulated spectra can be readily examined in future cold-atom experiments, where the two-dimensional spectroscopy is to be implemented by using a Ramsey interference sequence of rf pulses in the time domain. Our results also provide a first-principle understanding of the recent two-dimensional coherent spectroscopy of interacting excitons and trions in doped monolayer transition metal dichalcogenides.
We have developed a microscopic many-body theory of two-dimensional coherent spectroscopy (2DCS) for a model of polarons in one-dimensional (1D) materials. Our theory accounts for contributions from all three processes: excited-state emission (ESE), ground-state bleaching (GSB), and excited-state absorption (ESA). While the ESE and GSB contributions can be accurately described using Chevy's ansatz with one-particle-hole excitation, the ESA process requires information about the many-body eigenstates involving two impurities. To calculate these double polaron states, we have extended Chevy's ansatz with one-particle-hole excitation. The validity of this ansatz was verified by comparing our results with an exact calculation using Bethe's ansatz. Our numerical results reveal that in, the weak interaction limit, the ESA contribution cancels out the total ESE and GSB contributions, resulting in less significant spectral features. However, for strong interactions, the features of the ESA contribution and the combined ESE and GSB contributions remain observable in the 2DCS spectra. These features provide valuable information about the interactions between polarons. Additionally, we have investigated the mixing time dynamics, which characterize the quantum coherences of the polaron resonances. Overall, our theory provides a comprehensive framework for understanding and interpreting the 2DCS spectra of polarons in 1D materials, shedding light on their interactions and coherent dynamics.
Multidimensional spectroscopy is becoming an increasingly popular tool and there is an ongoing effort to access electronic transitions and many-body dynamics in correlated materials. We apply the protocol recently proposed by Wang [Phys. Rev. A 107, 013305 (2023)] to extract two-dimensional polaron spectra in a Fermi superfluid with an impurity. The bath is described by a BCS ansatz and it assumed that the impurity can scatter at most one quasiparticle pair. The spectral response contains a symmetric contribution, which carries the same information as Ramsey spectra, and an asymmetric one. While a priori it may seem promising to probe the quasiparticle gap from the asymmetric contribution, we show explicitly that this is not the case and, in the absence of incoherent processes, multidimensional spectroscopy does not bring much additional information. Our calculation is suitable for ultracold gases, but we discuss implications for exciton polarons in two-dimensional materials.
We theoretically analyze inverse radio-frequency (rf) spectroscopy experiments in two-component Fermi gases. We consider a small number of impurity atoms interacting strongly with a bath of majority atoms. In two-dimensional geometries we find that the main features of the rf spectrum correspond to an attractive polaron and a metastable repulsive polaron. Our results suggest that the attractive polaron has been observed in a recent experiment [B. Fr\"ohlich et al., Phys. Rev. Lett. 106, 105301 (2011)].
When mobile impurities are introduced and coupled to a Fermi sea, new quasiparticles known as Fermi polarons are formed.There are two interesting, yet drastically different regimes of the Fermi polaron problem: (i) the attractive polaron (AP) branch connected to pairing phenomena spanning the crossover from BCS superfluidity to the Bose-Einstein condensation of molecules and (ii) the repulsive branch (RP), which underlies the physics responsible for Stoner's itinerant ferromagnetism.Here, we study Fermi polarons in two-dimensional systems, where many questions and debates regarding their nature persist.The model system we investigate is a doped MoSe 2 monolayer.We find the observed AP-RP energy splitting and the quantum dynamics of attractive polarons agree with the predictions of polaron theory.As the doping density increases, the quantum dephasing of the attractive polarons remains constant, indicative of stable quasiparticles, while the repulsive polaron dephasing rate increases nearly quadratically.The dynamics of Fermi polarons are of critical importance for understanding the pairing and magnetic instabilities that lead to the formation of rich quantum phases found in a wide range of physical systems including nuclei, cold atomic gases, and solids.
We report on the experimental observation of multiorbital polarons in a two-dimensional Fermi gas of ^{173}Yb atoms formed by mobile impurities in the metastable ^{3}P_{0} orbital and a Fermi sea in the ground-state ^{1}S_{0} orbital. We spectroscopically probe the energies of attractive and repulsive polarons close to an orbital Feshbach resonance and characterize their coherence by measuring the quasiparticle residue. For all probed interaction parameters, the repulsive polaron is a long-lived quasiparticle with a decay rate more than 2 orders of magnitude below its energy. We formulate a many-body theory, which accurately treats the interorbital interactions in two dimensions and agrees well with the experimental results. Our work paves the way for the investigation of many-body physics in multiorbital ultracold Fermi gases.
We develop a non-Gaussian variational approach that enables us to study both equilibrium and far-from-equilibrium physics of the two-dimensional Fermi polaron. This method provides an unbiased analysis of the polaron-to-molecule phase transition without relying on truncations in the total number of particle-hole excitations. Our results—which include the ground-state energy and quasiparticle residue—are in qualitative agreement with the known Monte Carlo calculations. The main advantage of the non-Gaussian states compared to conventional numerical methods is that they enable us to explore long-time polaron evolution and, in particular, study various spectral properties accessible to both solid-state and ultracold atom experiments. We design two types of radiofrequency spectroscopies to measure polaronic and molecular spectral functions. Depending on the parameter regime, we find that these spectral functions and fermionic density profiles near the impurity either display long-lived oscillations between the repulsive and attractive polaron branches or exhibit fast relaxational dynamics to the molecular state.