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arXiv:2303.00907 · Physical Review X

Quantum Dynamics of Attractive and Repulsive Polarons in a Doped MoSe 2 Monolayer

Di Huang, Kevin Sampson, Yue Ni, Zhida Liu, Danfu Liang, Kenji Watanabe, Takashi Taniguchi, Hebin Li, Eric W. Martin, Jesper Levinsen, Meera M. Parish, Emanuel Tutuc, Dmitry K. Efimkin, Xiaoqin Li

Published Mar 2, 2023• 41 citations
arXivHTMLPDF

Abstract

When mobile impurities are introduced and coupled to a Fermi sea, new quasiparticles known as Fermi polarons are formed.There are two interesting, yet drastically different regimes of the Fermi polaron problem: (i) the attractive polaron (AP) branch connected to pairing phenomena spanning the crossover from BCS superfluidity to the Bose-Einstein condensation of molecules and (ii) the repulsive branch (RP), which underlies the physics responsible for Stoner's itinerant ferromagnetism.Here, we study Fermi polarons in two-dimensional systems, where many questions and debates regarding their nature persist.The model system we investigate is a doped MoSe 2 monolayer.We find the observed AP-RP energy splitting and the quantum dynamics of attractive polarons agree with the predictions of polaron theory.As the doping density increases, the quantum dephasing of the attractive polarons remains constant, indicative of stable quasiparticles, while the repulsive polaron dephasing rate increases nearly quadratically.The dynamics of Fermi polarons are of critical importance for understanding the pairing and magnetic instabilities that lead to the formation of rich quantum phases found in a wide range of physical systems including nuclei, cold atomic gases, and solids.

DOI
10.1103/physrevx.13.011029

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When mobile impurities are introduced and coupled to a Fermi sea, new quasiparticles known as Fermi polarons are formed.There are two interesting, yet drastically different regimes of the Fermi polaron problem: (i) the attractive polaron (AP) branch connected to pairing phenomena spanning the crossover from BCS superfluidity to the Bose-Einstein condensation of molecules and (ii) the repulsive branch (RP), which underlies the physics responsible for Stoner's itinerant ferromagnetism.Here, we study Fermi polarons in two-dimensional systems, where many questions and debates regarding their nature persist.The model system we investigate is a doped MoSe 2 monolayer.We find the observed AP-RP energy splitting and the quantum dynamics of attractive polarons agree with the predictions of polaron theory.As the doping density increases, the quantum dephasing of the attractive polarons remains constant, indicative of stable quasiparticles, while the repulsive polaron dephasing rate increases nearly quadratically.The dynamics of Fermi polarons are of critical importance for understanding the pairing and magnetic instabilities that lead to the formation of rich quantum phases found in a wide range of physical systems including nuclei, cold atomic gases, and solids.
Polaron quasiparticles are formed when a mobile impurity is coupled to the elementary excitations of a many-particle background. In the field of ultracold atoms, the study of the associated impurity problem has attracted a growing interest over the last fifteen years. Polaron quasiparticle properties are essential to our understanding of a variety of paradigmatic quantum many-body systems realized in ultracold atomic gases and in the solid state, from imbalanced Bose–Fermi and Fermi–Fermi mixtures to fermionic Hubbard models. In this topical review, we focus on the so-called repulsive polaron branch, which emerges as an excited many-body state in systems with underlying attractive interactions such as ultracold atomic mixtures, and is characterized by an effective repulsion between the impurity and the surrounding medium. We give a brief account of the current theoretical and experimental understanding of repulsive polaron properties, for impurities embedded in both fermionic and bosonic media, and we highlight open issues deserving future investigations.
The Fermi polaron, formed by an impurity interacting with a surrounding Fermi sea, exemplifies the canonical quasiparticle concept as a cornerstone in our description of quantum many-body systems across a wide range of energy scales. Experiments on atomic quantum gases have provided profound insights into the universal nature of the Fermi polaron. While most previous studies have focused on the case of zero impurity momentum, finite-momentum properties have remained largely uncharted. Here, we investigate the moving Fermi polaron by combining a novel Raman acceleration scheme with high-precision radio-frequency spectroscopy, exploring the quasiparticle dispersion relation over a wide range of momenta. We compare our measurements of energy shifts and spectral linewidths with a microscopic theory and reach quantitative agreement for all momenta. For low momenta, we find the energy of the moving polaron to be fully consistent with the Fermi liquid picture of a dressed particle with a constant effective mass. At high momenta, the polaron approaches the behavior of a weakly interacting bare particle, featuring small energy shifts and weak broadening. For intermediate momenta, broadening is generally larger and, most strikingly, the behavior differs for attractive and repulsive polarons. While the repulsive polaron exhibits a smooth connection between both regimes along with a monotonic change of the energy shift, the attractive case shows a peculiar non-monotonic behavior. With increasing momentum, the attractive polaron enters a regime where its energy deviates from the constant effective mass expression and broadening suddenly increases. By comparing this observation with theory, we show that this abrupt behavior coincides with the attractive polaron entering a molecule-hole continuum, where it is no longer the ground state. We interpret this as a motion-induced polaron-molecule transition.
Polarons are quasiparticles relevant across many fields in physics: from condensed matter to atomic physics. Here, we study the quasiparticle properties of two-dimensional strongly interacting Bose polarons in atomic Bose–Einstein condensates and polariton gases. Our studies are based on the non-self consistent T-matrix approximation adapted to these physical systems. For the atomic case, we study the spectral and quasiparticle properties of the polaron in the presence of a magnetic Feshbach resonance. We show the presence of two polaron branches: an attractive polaron, a low-lying state that appears as a well-defined quasiparticle for weak attractive interactions, and a repulsive polaron, a metastable state that becomes the dominant branch at weak repulsive interactions. In addition, we study a polaron arising from the dressing of a single itinerant electron by a quantum fluid of polaritons in a semiconductor microcavity. We demonstrate the persistence of the two polaron branches whose properties can be controlled over a wide range of parameters by tuning the cavity mode.
We investigate the metastable repulsive branch of a mobile impurity coupled to a degenerate Fermi gas via short-range interactions. We show that the quasiparticle lifetime of this repulsive Fermi polaron can be experimentally probed by driving Rabi oscillations between weakly and strongly interacting impurity states. Using a time-dependent variational approach, we find that we can accurately model the impurity Rabi oscillations that were recently measured for repulsive Fermi polarons in both two and three dimensions. Crucially, our theoretical description does not include relaxation processes to the lower-lying attractive branch. Thus, the theory-experiment agreement demonstrates that the quasiparticle lifetime is dominated by many-body dephasing within the upper repulsive branch rather than by relaxation from the upper branch itself. Our findings shed light on recent experimental observations of persistent repulsive correlations, and have important consequences for the nature and stability of the strongly repulsive Fermi gas.
Quasiparticles and their interactions are a key part of our understanding of quantum many-body systems. Quantum simulation experiments with cold atoms have in recent years advanced our understanding of isolated quasiparticles, but so far they have provided limited information regarding their interactions and possible bound states. Here, we show how exploring mobile impurities immersed in a Bose-Einstein condensate (BEC) in a two-dimensional lattice can address this problem. First, the spectral properties of individual impurities are examined, and in addition to the attractive and repulsive polarons known from continuum gases, we identify a new kind of quasiparticle stable for repulsive boson-impurity interactions. The spatial properties of polarons are calculated showing that there is an increased density of bosons at the site of the impurity both for repulsive and attractive interactions. We then derive an effective Schrödinger equation describing two polarons interacting via the exchange of density oscillations in the BEC, which takes into account strong impurity-boson two-body correlations. Using this, we show that the attractive nature of the effective interaction between two polarons combined with the two-dimensionality of the lattice leads to the formation of bound states - i.e. bipolarons. The wave functions of the bipolarons are examined showing that the ground state is symmetric under particle exchange and therefore relevant for bosonic impurities, whereas the first excited state is doubly degenerate and odd under particle exchange making it relevant for fermionic impurities. Our results show that quantum gas microscopy in optical lattices is a promising platform to explore the spatial properties of polarons as well as to finally observe the elusive bipolarons.
We consider the Fermi polaron problem of an impurity hopping around a two-dimensional square lattice and interacting with a sea of fermions at given filling factor. When the interaction is attractive, we find standard Fermi polaron quasiparticles, categorized as attractive polarons and repulsive polarons. When the interaction becomes repulsive, interestingly, we observe an unconventional highly excited polaron quasiparticle, sharply peaked at the corner of the first Brillouin zone with momentum $\mathbf{k}=(\ifmmode\pm\else\textpm\fi{}\ensuremath{\pi},\ifmmode\pm\else\textpm\fi{}\ensuremath{\pi})$. This super Fermi polaron branch arises from the dressing of the impurity's motion with holes, instead of particles of fermions. We show that super Fermi polarons become increasingly well defined with increasing impurity-fermion repulsions and might be considered as a precursor of Nagaoka ferromagnetism, which would appear at sufficiently large repulsions and at large filling factors. We also investigate the temperature dependence of super Fermi polarons and find that they are thermally robust against the significant increase in temperature.