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arXiv:2209.07254 · Physical Review A

Experimental violation of the Leggett-Garg inequality in a three-level trapped-ion system

Tianxiang Zhan, Chun-Wang Wu, Manchao Zhang, Qingqing Qin, Xueying Yang, Hu Han, Wenbo Su, Jie Zhang, Ting Chen, Yi Xie, Wei Wu, Ping-Xing Chen

Published Jan 25, 2023• 9 citations
arXivHTMLPDF

Abstract

Leggett-Garg inequality (LGI) is used to detect whether the macroscopic superposition state exists. Classical systems obey the LGI, but quantum systems may violate it. In the multilevel system, different state update rules determine different upper bounds of LGI. In this work, we experimentally test the LGI in a three-level trapped-ion system under the L\"uders and the von Neumann state update rules, respectively. The maximum observed value of the Leggett-Garg correlator under the von Neumann state update rule is ${K}_{3}=1.739\ifmmode\pm\else\textpm\fi{}0.014$, which demonstrates a violation of the L\"uders bound by 17 standard deviations and is by far the most significant violation under the specific model. The method used in our experiment could also be used in other multilevel experiments in the trapped-ion system.

DOI
10.1103/physreva.107.012424

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Leggett-Garg inequality (LGI) is used to detect whether the macroscopic superposition state exists. Classical systems obey the LGI, but quantum systems may violate it. In the multilevel system, different state update rules determine different upper bounds of LGI. In this work, we experimentally test the LGI in a three-level trapped-ion system under the L"uders and the von Neumann state update rules, respectively. The maximum observed value of the Leggett-Garg correlator under the von Neumann state update rule is K3=1.739\ifmmode±\else\textpm\fi0.014{K}_{3}=1.739\ifmmode\pm\else\textpm\fi{}0.014K3​=1.739\ifmmode±\else\textpm\fi0.014, which demonstrates a violation of the L"uders bound by 17 standard deviations and is by far the most significant violation under the specific model. The method used in our experiment could also be used in other multilevel experiments in the trapped-ion system.
Investigating the boundary between a quantum mechanical description and a classical realistic view is of fundamental importance. The Leggett-Garg (LG) inequality provides a criterion to distinguish between quantum systems and classical systems, and can be used to prove the macroscopic superposition state. A larger upper bound of the LG function can be obtained in a multilevel system. Here, we present an experimental violation of the Leggett-Garg inequality in a three-level system using a nitrogen-vacancy center in diamond by ideal negative result measurements. The experimental maximum value of the Leggett-Garg function is ${K}_{3}^{\text{expt}}=1.625\ifmmode\pm\else\textpm\fi{}0.022$, which exceeds the L\"uders bound with a $5\ensuremath{\sigma}$ level of confidence.
The Leggett-Garg inequality (LGI) delineates a boundary between quantum and classical systems. While the temporal quantum correlations represented by LGIs have been extensively investigated in the Hermitian domain, the exploration of LGIs under non-Hermitian conditions remains scarce. Theoretical conjectures posit that nonunitary dynamics could transcend the boundary of LGIs set by Hermitian quantum mechanics, yet its empirical validation is lacking. Here, we demonstrate the enhanced violation of LGIs in a non-Hermitian system of a parity-time (PT\mathcal{PT}PT)-symmetric trapped-ion qubit. The upper bounds of both the third-order parameter K3{K}_{3}K3​ and fourth-order parameter K4{K}_{4}K4​ increase with dissipation and can reach the maximum value when the system approaches the exceptional point, where ${K}_{3}={C}_{21}+{C}_{32}\ensuremath{-}{C}_{31}$ is comprising three two-time correlations and ${K}_{4}={C}_{21}+{C}_{32}+{C}_{43}\ensuremath{-}{C}_{41}$ is comprising four correlations. We also find that the lower bounds of K3{K}_{3}K3​ and K4{K}_{4}K4​ exhibit distinctive behaviors, where the lower bound of K3{K}_{3}K3​ remains constant, but that of K4{K}_{4}K4​ depends on the target states and measurement operators. These findings reveal a pronounced correlation between the dissipative nature of a quantum system and its temporal correlations.
The Leggett–Garg (LG) test of macroscopic realism involves a series of dichotomic non-invasive measurements that are used to calculate a function which has a fixed upper bound for a macrorealistic system and a larger upper bound for a quantum system. The quantum upper bound depends on both the details of the measurement and the dimension of the system. Here we present an LG experiment on a three-level quantum system, which produces a larger theoretical quantum upper bound than that of a two-level quantum system. The experiment is carried out in nuclear magnetic resonance and consists of the LG test as well as a test of the ideal assumptions associated with the experiment, such as measurement non-invasiveness. The non-invasive measurements are performed via the modified ideal negative result measurement scheme on a three-level system. Once these assumptions are tested, the violation becomes small, despite the fact that the LG value itself is large. Our results showcase the advantages of using the modified measurement scheme that can reach higher LG values, since these leave a larger margin for violating the inequality in the face of experimental imperfections.
We apply the Leggett-Garg inequalities (LGIs) to the cases of classical and quantum unstable systems. For classical systems the two assumptions of macroscopic realism and noninvasive measurements imply that the three-measurement string K3{K}_{3}K3​ is identically equal to 1. Also, for quantum-mechanical systems, for which the two assumptions are, in general, not valid, we find that K3=1{K}_{3}=1K3​=1 for purely exponential decays (${K}_{3}\ensuremath{\le}1$ is the general LGI). On the other hand, the necessary deviations from the exponential decay law at short and long times predicted by quantum mechanics lead to values of ${K}_{3}\ensuremath{\ne}1$. Moreover, a strict violation K3>1{K}_{3}>1K3​>1 typically occurs at short times. Thus, we conclude that experiments in which such deviations from the exponential decay law have been observed should also have in their data violations of the LGIs.
Leggett-Garg inequalities (LGIs) have been proposed in order to assess how far the predictions of quantum mechanics defy "macroscopic realism." With LGIs, correlations of measurements performed on a single system at different times are described. We report on an experiment that demonstrates the violation of an LGI with neutrons. The final measured value of the Leggett-Garg correlator K=1.120±0.007(stat)±0.019(sys), obtained in a neutron interferometric experiment, is clearly above the limit K=1 predicted by macrorealistic theories. The experimental results are analyzed within the framework of dynamical theory of neutron diffraction, evidently reproducing the obtained values.
Leggett-Garg inequalities are tests of macroscopic realism that can be violated by quantum mechanics. In this letter, we realise photonic Leggett-Garg tests on a three-level system and implement measurements that admit three distinct measurement outcomes, rather than the usual two. In this way we obtain violations of three- and four-time Leggett-Garg inequalities that are significantly in excess of those obtainable in standard Leggett-Garg tests. We also report violations the quantum-witness equality up to the maximum permitted for a three-outcome measurement. Our results highlight differences between spatial and temporal correlations in quantum mechanics.