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arXiv:2204.07765 · Physical Review A

Experimental violation of the Leggett-Garg inequality with a single-spin system

Maimaitiyiming Tusun, Wei Dong Cheng, Zihua Chai, Yang Wu, Ya Wang, Xing Rong, Jiangfeng Du

Published Apr 22, 2022• 7 citations
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Abstract

Investigating the boundary between a quantum mechanical description and a classical realistic view is of fundamental importance. The Leggett-Garg (LG) inequality provides a criterion to distinguish between quantum systems and classical systems, and can be used to prove the macroscopic superposition state. A larger upper bound of the LG function can be obtained in a multilevel system. Here, we present an experimental violation of the Leggett-Garg inequality in a three-level system using a nitrogen-vacancy center in diamond by ideal negative result measurements. The experimental maximum value of the Leggett-Garg function is ${K}_{3}^{\text{expt}}=1.625\ifmmode\pm\else\textpm\fi{}0.022$, which exceeds the L\"uders bound with a $5\ensuremath{\sigma}$ level of confidence.

DOI
10.1103/physreva.105.042613

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Investigating the boundary between a quantum mechanical description and a classical realistic view is of fundamental importance. The Leggett-Garg (LG) inequality provides a criterion to distinguish between quantum systems and classical systems, and can be used to prove the macroscopic superposition state. A larger upper bound of the LG function can be obtained in a multilevel system. Here, we present an experimental violation of the Leggett-Garg inequality in a three-level system using a nitrogen-vacancy center in diamond by ideal negative result measurements. The experimental maximum value of the Leggett-Garg function is K3expt=1.625\ifmmode±\else\textpm\fi0.022{K}_{3}^{\text{expt}}=1.625\ifmmode\pm\else\textpm\fi{}0.022K3expt​=1.625\ifmmode±\else\textpm\fi0.022, which exceeds the L"uders bound with a 5\ensuremathσ5\ensuremath{\sigma}5\ensuremathσ level of confidence.
The Leggett–Garg (LG) test of macroscopic realism involves a series of dichotomic non-invasive measurements that are used to calculate a function which has a fixed upper bound for a macrorealistic system and a larger upper bound for a quantum system. The quantum upper bound depends on both the details of the measurement and the dimension of the system. Here we present an LG experiment on a three-level quantum system, which produces a larger theoretical quantum upper bound than that of a two-level quantum system. The experiment is carried out in nuclear magnetic resonance and consists of the LG test as well as a test of the ideal assumptions associated with the experiment, such as measurement non-invasiveness. The non-invasive measurements are performed via the modified ideal negative result measurement scheme on a three-level system. Once these assumptions are tested, the violation becomes small, despite the fact that the LG value itself is large. Our results showcase the advantages of using the modified measurement scheme that can reach higher LG values, since these leave a larger margin for violating the inequality in the face of experimental imperfections.
Leggett-Garg inequality (LGI) is used to detect whether the macroscopic superposition state exists. Classical systems obey the LGI, but quantum systems may violate it. In the multilevel system, different state update rules determine different upper bounds of LGI. In this work, we experimentally test the LGI in a three-level trapped-ion system under the L\"uders and the von Neumann state update rules, respectively. The maximum observed value of the Leggett-Garg correlator under the von Neumann state update rule is ${K}_{3}=1.739\ifmmode\pm\else\textpm\fi{}0.014$, which demonstrates a violation of the L\"uders bound by 17 standard deviations and is by far the most significant violation under the specific model. The method used in our experiment could also be used in other multilevel experiments in the trapped-ion system.
Leggett-Garg inequalities are tests of macroscopic realism that can be violated by quantum mechanics. In this letter, we realise photonic Leggett-Garg tests on a three-level system and implement measurements that admit three distinct measurement outcomes, rather than the usual two. In this way we obtain violations of three- and four-time Leggett-Garg inequalities that are significantly in excess of those obtainable in standard Leggett-Garg tests. We also report violations the quantum-witness equality up to the maximum permitted for a three-outcome measurement. Our results highlight differences between spatial and temporal correlations in quantum mechanics.
Leggett-Garg inequalities are tests of macroscopic realism that can be violated by quantum mechanics. In this letter, we realise photonic Leggett-Garg tests on a three-level system and implement measurements that admit three distinct measurement outcomes, rather than the usual two. In this way we obtain violations of three- and four-time Leggett-Garg inequalities that are significantly in excess of those obtainable in standard Leggett-Garg tests. We also report violations the quantum-witness equality up to the maximum permitted for a three-outcome measurement. Our results highlight differences between spatial and temporal correlations in quantum mechanics.
Leggett-Garg inequalities (LGIs) have been proposed in order to assess how far the predictions of quantum mechanics defy "macroscopic realism." With LGIs, correlations of measurements performed on a single system at different times are described. We report on an experiment that demonstrates the violation of an LGI with neutrons. The final measured value of the Leggett-Garg correlator K=1.120±0.007(stat)±0.019(sys), obtained in a neutron interferometric experiment, is clearly above the limit K=1 predicted by macrorealistic theories. The experimental results are analyzed within the framework of dynamical theory of neutron diffraction, evidently reproducing the obtained values.
We report an experimental study of recently formulated entropic Leggett-Garg inequality (ELGI) by Usha Devi et al. [Phys. Rev. A 87, 052103 (2013)]. This inequality places a bound on the statistical measurement outcomes of dynamical observables describing a macrorealistic system. Such a bound is not necessarily obeyed by quantum systems, and therefore provides an important way to distinguish quantumness from classical behavior. Here we study ELGI using a two-qubit nuclear magnetic resonance system. To perform the noninvasive measurements required for the ELGI study, we prepare the system qubit in a maximally mixed state as well as use the ``ideal negative result measurement'' procedure with the help of an ancilla qubit. The experimental results show a clear violation of ELGI by over four standard deviations. These results agree with the predictions of quantum theory. The violation of ELGI is attributed to the fact that certain joint probabilities are not legitimate in the quantum scenario, in the sense they do not reproduce all the marginal probabilities. Using a three-qubit system, we also demonstrate that three-time joint probabilities do not reproduce certain two-time marginal probabilities.