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arXiv:1606.07151 · New Journal of Physics

Experimental violation of the Leggett–Garg inequality in a three-level system

Hemant Katiyar, Aharon Brodutch, Dawei Lu, Raymond Laflamme

Published Jan 31, 2017• 48 citations
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Abstract

The Leggett–Garg (LG) test of macroscopic realism involves a series of dichotomic non-invasive measurements that are used to calculate a function which has a fixed upper bound for a macrorealistic system and a larger upper bound for a quantum system. The quantum upper bound depends on both the details of the measurement and the dimension of the system. Here we present an LG experiment on a three-level quantum system, which produces a larger theoretical quantum upper bound than that of a two-level quantum system. The experiment is carried out in nuclear magnetic resonance and consists of the LG test as well as a test of the ideal assumptions associated with the experiment, such as measurement non-invasiveness. The non-invasive measurements are performed via the modified ideal negative result measurement scheme on a three-level system. Once these assumptions are tested, the violation becomes small, despite the fact that the LG value itself is large. Our results showcase the advantages of using the modified measurement scheme that can reach higher LG values, since these leave a larger margin for violating the inequality in the face of experimental imperfections.

DOI
10.1088/1367-2630/aa5c51

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The Leggett–Garg (LG) test of macroscopic realism involves a series of dichotomic non-invasive measurements that are used to calculate a function which has a fixed upper bound for a macrorealistic system and a larger upper bound for a quantum system. The quantum upper bound depends on both the details of the measurement and the dimension of the system. Here we present an LG experiment on a three-level quantum system, which produces a larger theoretical quantum upper bound than that of a two-level quantum system. The experiment is carried out in nuclear magnetic resonance and consists of the LG test as well as a test of the ideal assumptions associated with the experiment, such as measurement non-invasiveness. The non-invasive measurements are performed via the modified ideal negative result measurement scheme on a three-level system. Once these assumptions are tested, the violation becomes small, despite the fact that the LG value itself is large. Our results showcase the advantages of using the modified measurement scheme that can reach higher LG values, since these leave a larger margin for violating the inequality in the face of experimental imperfections.
Investigating the boundary between a quantum mechanical description and a classical realistic view is of fundamental importance. The Leggett-Garg (LG) inequality provides a criterion to distinguish between quantum systems and classical systems, and can be used to prove the macroscopic superposition state. A larger upper bound of the LG function can be obtained in a multilevel system. Here, we present an experimental violation of the Leggett-Garg inequality in a three-level system using a nitrogen-vacancy center in diamond by ideal negative result measurements. The experimental maximum value of the Leggett-Garg function is ${K}_{3}^{\text{expt}}=1.625\ifmmode\pm\else\textpm\fi{}0.022$, which exceeds the L\"uders bound with a $5\ensuremath{\sigma}$ level of confidence.
Macroscopic Realism (MR) says that a macroscopic system is always determinately in one or other of the macroscopically distinguishable states available to it. The Leggett-Garg (LG) inequality was derived to allow experimental test of whether or not this doctrine is true; it is also often thought of as a temporal version of a Bell-inequality. Despite recent interest in the inequality, controversy remains regarding what would be shown by its violation. Here we resolve this controversy, which arises due to an insufficiently general and model-independent approach to the question so far. We argue that LG's initial characterisation of MR does not pick out a particularly natural realist position, so we articulate an operationally well-defined and well-motivated position in its place. We show that much weaker conditions than LG's are sufficient to derive the inequality: in the first instance, its violation only demonstrates that certain measurements fail to be non-disturbing at the operational level. We articulate three distinct species of MR-ist position, and argue that it is only the first of these which can be refuted by LG inequality violation. This first position is an attractive one, so ruling it out remains of interest, however. A crucial role is played in LG's argument by the assumption of noninvasive measurability. We show that this notion is ambiguous between the weaker notion of disturbance at the operational level, and the stronger notion of invasiveness at the ontic level of properties of the system. Ontic noninvasiveness would be required to rule out MR per se but this property is not entailed by MR, and its presence cannot be established in a model-independent way. It follows that despite the formal parallels, Bell's and LG's inequalities are not methodologically on a par. We close with some reflections on the implications of our analysis for the pedagogy of quantum superposition.
We report an experimental study of recently formulated entropic Leggett-Garg inequality (ELGI) by Usha Devi et al. [Phys. Rev. A 87, 052103 (2013)]. This inequality places a bound on the statistical measurement outcomes of dynamical observables describing a macrorealistic system. Such a bound is not necessarily obeyed by quantum systems, and therefore provides an important way to distinguish quantumness from classical behavior. Here we study ELGI using a two-qubit nuclear magnetic resonance system. To perform the noninvasive measurements required for the ELGI study, we prepare the system qubit in a maximally mixed state as well as use the ``ideal negative result measurement'' procedure with the help of an ancilla qubit. The experimental results show a clear violation of ELGI by over four standard deviations. These results agree with the predictions of quantum theory. The violation of ELGI is attributed to the fact that certain joint probabilities are not legitimate in the quantum scenario, in the sense they do not reproduce all the marginal probabilities. Using a three-qubit system, we also demonstrate that three-time joint probabilities do not reproduce certain two-time marginal probabilities.
Macroscopic realism (MR) is the view that a system may possess definite properties at any time independent of past or future measurements, and may be tested experimentally using the Leggett-Garg inequalities (LGIs). In this work we advance the study of LGIs in two ways using experiments carried out on a nuclear magnetic resonance spectrometer. Firstly, we addresses the fact that the LGIs are only necessary conditions for MR but not sufficient ones. We implement a recently-proposed test of necessary and sufficient conditions for MR which consists of a combination of the original four three-time LGIs augmented with a set of twelve two-time LGIs. We explore different regimes in which the two- and three-time LGIs may each be satisfied or violated. Secondly, we implement a recent proposal for a measurement protocol which determines the temporal correlation functions in an approximately non-invasive manner. It employs a measurement of the velocity of a dichotomic variable Q, continuous in time, from which a possible sign change of Q may be determined in a single measurement of an ancilla coupled to the velocity. This protocol involves a significantly different set of assumptions to the traditional ideal negative measurement protocol and a comparison with the latter is carried out.
A recent paper by Souza, Oliveira and Sarthour (SOS) reports the experimental violation of a Leggett–Garg (LG) inequality (sometimes referred to as a temporal Bell inequality). The inequality tests for quantum mechanical superposition: if the inequality is violated, the dynamics cannot be explained by a large class of classical theories under the heading of macrorealism. Experimental tests of the LG inequality are beset by the difficulty of carrying out the necessary so-called 'non-invasive' measurements (which for the macrorealist will extract information from a system of interest without disturbing it). SOS argue that they nevertheless achieve this difficult goal by putting the system in a maximally mixed state. The system then allegedly undergoes no perturbation during their experiment. Unfortunately, the method is ultimately unconvincing to a skeptical macrorealist and so the conclusions drawn by SOS are unjustified.
Macroscopic realism is the thesis that macroscopically observable properties must always have definite values. The idea was introduced by Leggett and Garg (1985), who wished to show a conflict with the predictions of quantum theory, by using it to derive an inequality that quantum theory violates. However, Leggett and Garg's analysis required not just the assumption of macroscopic realism per se, but also that the observable properties could be measured non-invasively. In recent years there has been increasing interest in experimental tests of the violation of the Leggett-Garg inequality, but it has remained a matter of controversy whether this second assumption is a reasonable requirement for a macroscopic realist view of quantum theory. In a recent critical assessment Maroney and Timpson (2014) identified three different categories of macroscopic realism, and argued that only the simplest category could be ruled out by Leggett-Garg inequality violations. Allen, Maroney, and Gogioso (2016) then showed that the second of these approaches was also incompatible with quantum theory in Hilbert spaces of dimension 4 or higher. However, we show that the distinction introduced by Maroney and Timpson between the second and third approaches is not noise tolerant, so unfortunately Allen's result, as given, is not directly empirically testable. In this paper we replace Maroney and Timpson's three categories with a parameterization of macroscopic realist models, which can be related to experimental observations in a noise tolerant way, and recover the original definitions in the noise-free limit. We show how this parameterization can be used to experimentally rule out classes of macroscopic realism in Hilbert spaces of dimension 3 or higher, without any use of the non-invasive measurability assumption. Even for relatively low precision experiments, this will rule out the original category of macroscopic realism, that is tested by the Leggett-Garg inequality, while as the precision of the experiments increases, all cases of the second category and many cases of the third category, will become experimentally ruled out.