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arXiv:2207.07314 · SciPost Physics

Floquet fractional Chern insulators and competing phases in twisted bilayer graphene

Peng-Sheng Hu, Yihan Zhou, Zhao Liu

Published Oct 10, 2023• 4 citations
arXivHTMLPDF

Abstract

We study the many-body physics in twisted bilayer graphene coupled to periodic driving of a circularly polarized light when electron-electron interactions are taken into account. In the limit of high driving frequency \Omega Ω , we use Floquet theory to formulate the system by an effective static Hamiltonian truncated to the order of \Omega^{-2} Ω − 2 , which consists of a single-electron part and the screened Coulomb interaction. We numerically simulate this effective Hamiltonian by extensive exact diagonalization in the parameter space spanned by the twist angle and the driving strength. Remarkably, in a wide region of the parameter space, we identify Floquet fractional Chern insulator states in the partially filled Floquet valence bands. We characterize these topologically ordered states by ground-state degeneracy, spectral flow, and entanglement spectrum. In regions of the parameter space where fractional Chern insulator states are absent, we find topologically trivial charge density waves and band-dispersion-induced Fermi liquids which strongly compete with fractional Chern insulator states.

DOI
10.21468/scipostphys.15.4.148

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We study the many-body physics in twisted bilayer graphene coupled to periodic driving of a circularly polarized light when electron-electron interactions are taken into account. In the limit of high driving frequency \Omega Ω , we use Floquet theory to formulate the system by an effective static Hamiltonian truncated to the order of \Omega^{-2} Ω − 2 , which consists of a single-electron part and the screened Coulomb interaction. We numerically simulate this effective Hamiltonian by extensive exact diagonalization in the parameter space spanned by the twist angle and the driving strength. Remarkably, in a wide region of the parameter space, we identify Floquet fractional Chern insulator states in the partially filled Floquet valence bands. We characterize these topologically ordered states by ground-state degeneracy, spectral flow, and entanglement spectrum. In regions of the parameter space where fractional Chern insulator states are absent, we find topologically trivial charge density waves and band-dispersion-induced Fermi liquids which strongly compete with fractional Chern insulator states.
Twisted bilayer materials provide a versatile platform for realizing correlated topological states. Motivated by the recent experimental realization of atomic Bose-Einstein condensates in twisted bilayer optical lattices, we investigate the emergence of fractional topological phases in such systems. For experimentally realistic parameters, the single-particle spectrum hosts a pair of quasi-degenerate nearly flat moiré bands. We show using self-consistent Hartree-Fock calculations that atomic interactions spontaneously break time-reversal symmetry, lift the quasi-degeneracy, and generate an isolated nearly flat band with a nonzero Chern number. At fractional filling, exact diagonalization of the Hamiltonian projected to this band reveals a threefold degenerate ground-state manifold and a characteristic particle entanglement spectrum, providing strong evidence for a fractional Chern insulator. The resulting many-body gap is of order 10−3ER10^{-3}E_R10−3ER​, corresponding to a nanokelvin energy scale accessible to state-of-the-art cold-atom experiments. Our scheme requires neither spin-orbit coupling, as in transition metal dichalcogenides, nor a finite magnetic field, as in existing twisted-bilayer-graphene experiments, providing a highly tunable route to strongly correlated topological phases in twisted bilayer optical lattices.
Experimental realizations of Abelian fractional Chern insulators (FCIs) have demonstrated the potentials of moiré systems in synthesizing exotic quantum phases. Remarkably, twisted multilayer graphene system may also host non-Abelian states competing with charge density wave under Coulomb interaction. Here, through larger scale exact diagonalization simulations, we map out the quantum phase diagram for ν=1/2ν=1/2ν=1/2 system with electrons occupying the lowest moirè band of the double twisted bilayer graphene. By increasing the system size, we find the ground state has six-fold near degeneracy and with a finite spectral gap separating the ground states from excited states across a broad range of parameters. Further computation of many-body Chern number establish the topological order of the state, and we rule out possibility of charge density wave orders based on featureless density structure factor. Furthermore, we inspect the particle-cut entanglement spectrum to identify the topological state as a non-Abelian Moore-Read state. Combining all the above evidences we conclude that Moore-Read ground state dominates the quantum phase diagram for the double twisted bilayer graphene system for a broad range of coupling strength with realistic Coulomb interaction.
Breakthrough experiments have recently realized fractional Chern insulators (FCIs) in moiré materials. However, all states observed are Abelian; the possible existence of more exotic non-Abelian FCIs remains controversial both experimentally and theoretically. Here, we investigate the competition between charge density wave (CDW) order, gapless composite fermion liquid (CFL), and non-Abelian Moore-Read states at half filling of a moiré band. Although ground-state (quasi)degeneracies and spectral flow are not sufficient for distinguishing between charge order and Moore-Read states, we find evidence using entanglement spectroscopy that both these states of matter can be realized with Coulomb interactions. By further analyzing the graviton excitations of Moore-Read states, we unveil that the ground states exhibit a mixed behavior of Pfaffian and anti-Pfaffian, despite the weak breaking of particle-hole symmetry. In a double twisted bilayer graphene model, transitions between these phases can be driven by the coupling strength between the layers: at weak coupling there is a CFL phase and at strong coupling a CDW order emerges. Remarkably, however, there is compelling evidence for a non-Abelian Moore-Read FCI phase at intermediate coupling.
We show theoretically that periodically driven systems with short range Hubbard interactions offer a feasible platform to experimentally realize fractional Chern insulator states. We exemplify the procedure for both the driven honeycomb and the square lattice, where we derive the effective steady state band structure of the driven system by using the Floquet theory and subsequently study the interacting system with exact numerical diagonalization. The fractional Chern insulator state equivalent to the 1/3 Laughlin state appears at 7/12 total filling (1/6 filling of the upper band). The state also features spontaneous ferromagnetism and is thus an example of the spontaneous breaking of a continuous symmetry along with a topological phase transition. We discuss light-driven graphene and shaken optical lattices as possible experimental systems that can realize such a state.
Motivated by the higher Chern bands of twisted graphene multilayers, we consider flat bands with arbitrary Chern number C with ideal quantum geometry. While C > 1 bands differ from Landau levels, we show that these bands host exact fractional Chern insulator (FCI) ground states for short-range interactions. We show how to decompose ideal higher Chern bands into separate ideal bands with Chern number 1 that are intertwined through translation and rotation symmetry. The decomposed bands admit an SU ( C ) action that combines real space and momentum space translations. Remarkably, they also allow for analytic construction of exact many-body ground states, such as generalized quantum Hall ferromagnets and FCIs, including flavor-singlet Halperin states and Laughlin ferromagnets in the limit of short-range interactions. In this limit, the SU ( C ) action is promoted to a symmetry on the ground-state subspace. While flavor singlet states are translation symmetric, the flavor ferromagnets correspond to translation broken states and admit charged skyrmion excitations corresponding to a spatially varying density wave pattern. We confirm our analytic predictions with numerical simulations of ideal bands of twisted chiral multilayers of graphene, and discuss consequences for experimentally accessible systems such as monolayer graphene twisted relative to a Bernal bilayer. Published by the American Physical Society 2023
Abstract Magic-angle twisted bilayer graphene has recently become a thriving material platform realizing correlated electron phenomena taking place within its topological flat bands. Several numerical and analytical methods have been applied to understand the correlated phases therein, revealing some similarity with the quantum Hall physics. In this work, we provide a Mott-Hubbard perspective for the TBG system. Employing the large-scale density matrix renormalization group on the lattice model containing the projected Coulomb interactions only, we identify a first-order quantum phase transition between the insulating stripe phase and the quantum anomalous Hall state with the Chern number of ±1. Our results not only shed light on the mechanism of the quantum anomalous Hall state discovered at three-quarters filling, but also provide an example of the topological Mott insulator, i.e., the quantum anomalous Hall state in the strong coupling limit.