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arXiv:2206.05465

Multi-state interferometric measurement of nonlinear AC Stark shift

Junnosuke Takai, Kosuke Shibata, Naota Sekiguchi, Takuya Hirano

Published Jun 11, 2022• 0 citations
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Abstract

We demonstrate measurement of quadratic AC Stark shifts between Zeeman sublevels in an $^{87}$Rb Bose--Einstein condensate using a multi-state atomic interferometer. The interferometer can detect a quadratic shift without being affected by relatively large state-independent shifts, thereby improving the measurement precision. We measure quadratic shifts in the total spin $F = 2$ state due to the light being near-resonant to the D$_1$ line. The agreement between the measured and theoretical detuning dependences of the quadratic shifts confirms the validity of the measurement. We also present results on the suppression of nonlinear spin evolution using near-resonant dual-color light pulses with opposite quadratic shifts.

DOI
10.48550/arxiv.2206.05465

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•Jan 1, 2008•3 citations
We demonstrate measurement of quadratic AC Stark shifts between Zeeman sublevels in an 87^{87}87Rb Bose--Einstein condensate using a multi-state atomic interferometer. The interferometer can detect a quadratic shift without being affected by relatively large state-independent shifts, thereby improving the measurement precision. We measure quadratic shifts in the total spin F=2F = 2F=2 state due to the light being near-resonant to the D1_11​ line. The agreement between the measured and theoretical detuning dependences of the quadratic shifts confirms the validity of the measurement. We also present results on the suppression of nonlinear spin evolution using near-resonant dual-color light pulses with opposite quadratic shifts.
The authors develop an experimental method for measuring the quadratic ac Stark shifts between Zeeman sublevels in an 87{}^{87}87Rb Bose--Einstein condensate using a multistate atomic interferometer. The measured quadratic shifts are shown in good agreement with the theoretical calculations. The method could be useful for improving atomic sensors, such as magnetometers and atomic clocks.
The dynamic polarizability of 87Rb^{87}\mathrm{Rb}87Rb atoms was measured using a guided-wave Bose-Einstein condensate interferometer. Taking advantage of the large arm separations obtainable in our device, a well-calibrated laser beam is applied to one atomic packet and not the other, inducing a differential phase shift. The technique requires relatively low laser intensity and works for arbitrary optical frequencies. For off-resonant light, the ac polarizability is obtained with a statistical accuracy of 3% and a calibration uncertainty of 6%. On resonance, the dispersion-shaped behavior of the Stark shift is observed, but with a broadened linewidth that is attributed to collective light scattering effects. The resulting nonlinearity may prove useful for the production and control of squeezed quantum states.
The ac Stark shift (also known as the ``light shift'') is one of the most important physical processes that arises in precision spectroscopy, affecting the basic understanding of field-matter interactions, measurements of fundamental constants, and even the atomic clocks onboard GPS satellites. Although the theory of the ac Stark shift was fully developed by the 1960s and 1970s, precision tests of theory have, for the most part, been few. Taking advantage of recent developments in atomic clock technology, specifically the pulsed approach to atomic signal generation, which allows frequency measurements with a resolution of $\ensuremath{\sim}{10}^{\ensuremath{-}15}$, we demonstrate a methodology for measuring the ac Stark shift. Here, we report results from a precision examination of the ac Stark shift in a vapor phase system, examining the resonant frequency of the 87Rb^{87}\text{Rb}87Rb 0-0 hyperfine transition for a perturbing laser tuned over a broad optical frequency range (18 GHz) around the D1{D}_{1}D1​ absorption resonance. Over the full frequency range the agreement between semiclassical theory and experiment is very good (better than $5\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}2}$), and in our experiments we test both the frequency dependence of the scalar and tensor components of the light shift.
In a recent letter [Auzinsh {\it{et. al.}} (physics/0403097)] we have analyzed the noise properties of an idealized atomic magnetometer that utilizes spin squeezing induced by a continuous quantum nondemolition measurement. Such a magnetometer measures spin precession of NNN atomic spins by detecting optical rotation of far-detuned probe light. Here we consider maximally squeezed probe light, and carry out a detailed derivation of the contribution to the noise in a magnetometric measurement due to the differential AC Stark shift between Zeeman sublevels arising from quantum fluctuations of the probe polarization.
We demonstrate that when laser light is circularly polarized and properly detuned, the ac Stark shift of an alkali-metal atom in its ground state takes the form of a pure Zeeman shift. The condition is satisfied when the laser frequency is between the D1D1D1 and D2D2D2 transition frequencies, with the size of the detuning from the D2D2D2 resonance twice that from the D1D1D1 resonance. The direction of the effective magnetic field is along the laser propagation axis, and its magnitude is proportional to the vector polarizability of the atom and to the laser intensity. We use stimulated Raman spectroscopy on an optically pumped slow atomic beam from a magneto-optical trap to measure the vector polarizability and saturated absorption spectroscopy to show that the scalar polarizability vanishes at the particular detuning.
An atom interferometer using Bose-Einstein condensates has been implemented and is used to measure the dynamic polarizability of 87Rb. An off-resonant standing-wave laser beam is used to manipulate the motion of atomic wavepackets in order to implement splitting and reflection operations. It is demonstrated that these operations can be performed with near unity fidelity. Interferometer times of up to 72 ms as well as arm separations of up to 0.42 mm are achieved experimentally. The primary limitation for guided-wave atom interferometers with a large arm separation is found to be the effect of the confining potential along the waveguide axis. Such a potential causes a spatially varying phase shift on the wavepackets as they propagate in the interferometer. Different parts of the cloud therefore interfere with different phases, leading to a reduction of the interferometer contrast. A model of the phase shifts on the wavepackets agrees well with the experimental data. In a different scheme in which the wavepackets oscillate freely in the confining potential, these phase shifts completely cancel. Interference is observed at times up to 0.9 s in this case, but with a fluctuating overall phase of the output, which is attributed to mechanical instabilities. Finally, the dynamic polarizability of 87Rb is measured. A well-calibrated laser beam is applied to one atomic packet and not the other, inducing a differential phase shift. This technique requires relatively low laser intensity and works for arbitrary optical frequencies. For offresonant light, the ac polarizability is obtained with a statistical accuracy of 3% and a calibration uncertainty of 6%. On resonance, the dispersion-shaped behavior of the Stark shift is observed, but with a broadened linewidth that is attributed to multiple and collective light scattering effects. The resulting nonlinearity may prove useful for the production and control of squeezed quantum states. In general, this work also demonstrates the applicability of condensate interferometry to practical measurements.