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arXiv:0709.4675 · Physical Review A

Measurement of the ac Stark shift with a guided matter-wave interferometer

Benjamin Deissler, K. J. Hughes, John H. Burke, Charles A. Sackett

Published Mar 14, 2008• 40 citations
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Abstract

The dynamic polarizability of $^{87}\mathrm{Rb}$ atoms was measured using a guided-wave Bose-Einstein condensate interferometer. Taking advantage of the large arm separations obtainable in our device, a well-calibrated laser beam is applied to one atomic packet and not the other, inducing a differential phase shift. The technique requires relatively low laser intensity and works for arbitrary optical frequencies. For off-resonant light, the ac polarizability is obtained with a statistical accuracy of 3% and a calibration uncertainty of 6%. On resonance, the dispersion-shaped behavior of the Stark shift is observed, but with a broadened linewidth that is attributed to collective light scattering effects. The resulting nonlinearity may prove useful for the production and control of squeezed quantum states.

DOI
10.1103/physreva.77.031604

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arXiv:cond-mat/0306305•Physical Review Letters•Feb 6, 2004•508 citations
The dynamic polarizability of 87Rb^{87}\mathrm{Rb}87Rb atoms was measured using a guided-wave Bose-Einstein condensate interferometer. Taking advantage of the large arm separations obtainable in our device, a well-calibrated laser beam is applied to one atomic packet and not the other, inducing a differential phase shift. The technique requires relatively low laser intensity and works for arbitrary optical frequencies. For off-resonant light, the ac polarizability is obtained with a statistical accuracy of 3% and a calibration uncertainty of 6%. On resonance, the dispersion-shaped behavior of the Stark shift is observed, but with a broadened linewidth that is attributed to collective light scattering effects. The resulting nonlinearity may prove useful for the production and control of squeezed quantum states.
An atom interferometer using Bose-Einstein condensates has been implemented and is used to measure the dynamic polarizability of 87Rb. An off-resonant standing-wave laser beam is used to manipulate the motion of atomic wavepackets in order to implement splitting and reflection operations. It is demonstrated that these operations can be performed with near unity fidelity. Interferometer times of up to 72 ms as well as arm separations of up to 0.42 mm are achieved experimentally. The primary limitation for guided-wave atom interferometers with a large arm separation is found to be the effect of the confining potential along the waveguide axis. Such a potential causes a spatially varying phase shift on the wavepackets as they propagate in the interferometer. Different parts of the cloud therefore interfere with different phases, leading to a reduction of the interferometer contrast. A model of the phase shifts on the wavepackets agrees well with the experimental data. In a different scheme in which the wavepackets oscillate freely in the confining potential, these phase shifts completely cancel. Interference is observed at times up to 0.9 s in this case, but with a fluctuating overall phase of the output, which is attributed to mechanical instabilities. Finally, the dynamic polarizability of 87Rb is measured. A well-calibrated laser beam is applied to one atomic packet and not the other, inducing a differential phase shift. This technique requires relatively low laser intensity and works for arbitrary optical frequencies. For offresonant light, the ac polarizability is obtained with a statistical accuracy of 3% and a calibration uncertainty of 6%. On resonance, the dispersion-shaped behavior of the Stark shift is observed, but with a broadened linewidth that is attributed to multiple and collective light scattering effects. The resulting nonlinearity may prove useful for the production and control of squeezed quantum states. In general, this work also demonstrates the applicability of condensate interferometry to practical measurements.
We demonstrate measurement of quadratic AC Stark shifts between Zeeman sublevels in an 87^{87}87Rb Bose--Einstein condensate using a multi-state atomic interferometer. The interferometer can detect a quadratic shift without being affected by relatively large state-independent shifts, thereby improving the measurement precision. We measure quadratic shifts in the total spin F=2F = 2F=2 state due to the light being near-resonant to the D1_11​ line. The agreement between the measured and theoretical detuning dependences of the quadratic shifts confirms the validity of the measurement. We also present results on the suppression of nonlinear spin evolution using near-resonant dual-color light pulses with opposite quadratic shifts.
We demonstrate that when laser light is circularly polarized and properly detuned, the ac Stark shift of an alkali-metal atom in its ground state takes the form of a pure Zeeman shift. The condition is satisfied when the laser frequency is between the D1D1D1 and D2D2D2 transition frequencies, with the size of the detuning from the D2D2D2 resonance twice that from the D1D1D1 resonance. The direction of the effective magnetic field is along the laser propagation axis, and its magnitude is proportional to the vector polarizability of the atom and to the laser intensity. We use stimulated Raman spectroscopy on an optically pumped slow atomic beam from a magneto-optical trap to measure the vector polarizability and saturated absorption spectroscopy to show that the scalar polarizability vanishes at the particular detuning.
We report a measurement of the dynamic (ac) scalar polarizability of the 5D3/2 state in 85Rb atoms at a laser wavelength of 1064 nm. Contrary to a recent measurement in Phys. Rev. A 104, 063304 (2021), the experiments are performed in a low-intensity regime in which the ac shift is less than the 5D3/2 state’s hyperfine structure, as utilized in numerous experiments with cold, trapped atoms. The extracted ac polarizability is α5D3/2=−499±59 a.u., within the uncertainty of the aforementioned previous result. The calibration of the 1064 nm light intensity, performed by analyzing light shifts of the D1 line, is the main source of uncertainty. Our results are useful for applications of the Rb 5D3/2 state in metrology, quantum sensing, and fundamental-physics research on Rydberg atoms and molecules.
An atomic polarizing white-color interferometer composed of the wave packets in the m=+1m=+1m=+1 and $m=\ensuremath{-}1$ states of the excited 3P1{}^{3}{P}_{1}3P1​ state of Ca, has been developed using a thermal atomic beam excited by a pair of two resonant lights at two separate zones under a homogeneous magnetic field. The interferometer generated the Ramsey fringes as a detuning of the rf frequency between two resonant lights from the Zeeman-frequency shift, while it generates white-color interference fringes as a detuning of laser frequency. The interferometer was used for the direct and short-time measurement of the Aharonov-Casher phase by removing the main part of dc Stark phase shift and without the influence of the frequency fluctuation of a laser. The measured dependence of the Aharonov-Casher phase on the electric field agreed with the predicted one within a relative uncertainty of 2.9%. The tensor polarizability in the 3P1{}^{3}{P}_{1}3P1​ state was determined to be ${\ensuremath{\alpha}}_{2}=2.623\ifmmode\pm\else\textpm\fi{}0.015 \mathrm{k}\mathrm{H}\mathrm{z}/(\mathrm{k}\mathrm{V}/\mathrm{c}\mathrm{m}{)}^{2}$ from the frequency shift between the m=+1m=+1m=+1 and $m=\ensuremath{-}1$ states.
A trapped-atom interferometer was demonstrated using gaseous Bose-Einstein condensates coherently split by deforming an optical single-well potential into a double-well potential. The relative phase between the two condensates was determined from the spatial phase of the matter wave interference pattern formed upon releasing the condensates from the separated potential wells. Coherent phase evolution was observed for condensates held separated by 13 microm for up to 5 ms and was controlled by applying ac Stark shift potentials to either of the two separated condensates.