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arXiv:2203.06885 · Physical Review A

Rydberg electromagnetically induced transparency and absorption of strontium triplet states in a weak microwave field

Yan-Li Zhou, Dong Yan, Weibin Li

Published May 19, 2022• 20 citations
arXivHTMLPDF

Abstract

We study theoretically laser excitation of Rydberg triplet states of strontium atoms in the presence of weak microwave (MW) fields. Starting from the ground state $5{s}^{2}{\phantom{\rule{0.16em}{0ex}}}^{1}{S}_{0}$, the Rydberg excitation is realized through the metastable, triplet $5s5{p}^{3}{P}_{1}$ state, whose decay rate ${\ensuremath{\gamma}}_{2}$ is $2\ensuremath{\pi}\ifmmode\times\else\texttimes\fi{}7.5$ kHz, much smaller than the one in the singlet state or alkali-metal atoms. The influences of ${\ensuremath{\gamma}}_{2}$ on the transparency and absorption spectrum in the electromagnetically induced transparency (EIT), and electromagnetically induced absorption (EIA) regime are examined. Narrow transparent windows (EIT) or absorption peaks (EIA) are found, whose distance in the spectrum depends on the Rabi frequency of the weak MW field. It is found that the spectrum exhibits higher contrast than using the singlet state or alkali-metal atoms in typical situations. Using the metastable intermediate state, we find that the resonance fluorescence of Sr gases exhibits very narrow peaks, which are modulated by the MW field. When the MW field is weaker than the probe and control light, the spectrum distance of these peaks is linearly proportional to ${\mathrm{\ensuremath{\Omega}}}_{m}$. This allows us to propose an alternative way to sense very weak MW fields through resonance fluorescence. Our study shows that the Sr triplet state could be used to develop the Rydberg MW electrometry that gains unique advantages.

DOI
10.1103/physreva.105.053714

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Abstract A scheme for measuring microwave (MW) electric (E) fields is proposed based on bichromatic electromagnetically induced transparency (EIT) in Rydberg atoms. A bichromatic control field drives the excited state transition, whose absorption shows three EIT windows. When a MW field drives the Rydberg transition, the EIT windows split and six transmission peaks appear. It is interesting to find that the peak-to-peak distance of transmission spectrum is sensitive to the MW field strength, which can be used to measure MW E-field. Simulation results show that the measurement accuracy could be increased by about 4 times, and the minimum detectable strength of the MW E-field may be improved by about 3 times compared with the common EIT scheme. After the Doppler averaging, the minimum detectable MW E-field strength is about 5 times larger than that without Doppler effect. Also, we investigate other effects on the sensitivity of the system.
Transient response of four-level cold Rb atoms with light and microwave (MW) fields is investigated via electromagnetically induced transparency (EIT) theoretically. The local control laser acts as a switch. When the control field is weak, the population transition channel from state 53 D 5/2 to state 5 S 1/2 is closed, which leads to that the transient absorption for the probe field monotonically decreases to its steady state. Nevertheless, when the control field becomes strong, the transition channel is open, which gives rise to that the transient absorption for the probe laser will be oscillatorily damped to the steady-state value, and transient negative absorption appears. A third MW field can induce splitting of the time-dependent EIT transmission spectrum, and the stable splitting distance shows a linear dependence on the continuous MW electric (E) field strength. Furthermore, the simulation results show that the temporal medium transmission signals are sensitive to the E-field strength of local MW pulse, and can be used to sense pulsed MW fields.
Abstract We present the electromagnetically induced transparency (EIT) spectra of cold Rydberg four-level cascade atoms consisting of the 6S1/2 → 6P3/2 → 7S1/2 → 60P3/2 scheme. A coupling laser drives the Rydberg transition, a dressing laser couples two intermediate levels and a weak probe laser probes the EIT signal. We numerically solve the Bloch equations and investigate the dependence of the probe transmission rate signal on the coupling and dressing lasers. We find that the probe transmission rate can display an EIT or electromagnetically induced absorption (EIA) profile, depending on the Rabi frequencies of the coupling and dressing lasers. When we increase the Rabi frequency of the coupling laser and keep the Rabi frequency of the probe and dressing laser fixed, flipping of the EIA to EIT spectrum occurs at the critical coupling Rabi frequency. When we apply a microwave field coupling the transition 60P3/2 → 61S1/2, the EIT spectrum shows Autler–Townes splitting, which is employed to measure the microwave field. The theoretical measurement sensitivity can be 1.52 × 10−2 nV⋅cm−1⋅Hz−1/2 at the EIA–EIT flipping point.
We present an electromagnetically induced transparency and Aulter-Townes (EIT-AT) spectrum of a Rydberg three-level atom that is dressed with a microwave field in a room-temperature cesium cell. The EIT is a quantum coherent effect produced by the interaction of atoms with electromagnetic waves, which leads to the decrease of the absorption for a weak resonant probe laser. AT splitting refers to the phenomenon, that the absorption line splits when an electromagnetic field that is in resonance or near resonance acts on the transition of atoms. Rydberg atoms are extremely sensitive to an external electric field due to their large polarizabilities and microwave transition dipole moments, which can be used to measure the external field. In this work, a Rydberg three-level EIT is used to detect Rydberg atom and AT splitting induced by the microwave field. Cesium levels 6S1/2, 6P3/2 and 50S1/2 constitute a Rydberg three-level system, in which a weak probe laser locking to the transition from 6S1/2 to 6P3/2 couples ground-state transition and the strong coupling laser resonates on the Rydberg transition from 6P2/3 to 50S1/2. The two Rydberg levels 50S1/2 and 50P1/2 are coupled with the microwave field at a frequency of 30.852 GHz, leading to the AT splitting of EIT line and forming an EIT-AT spectrum, which is used to measure the electric field amplitude of microwave. In order to further study the EIT-AT splitting characteristics of the Rydberg levels, we carry out a series of measurements by changing the microwave field. The experimental results show a broadened EIT-AT signal for the weak field range and the four-peak spectrum for the strong field, which is attributed to the inhomogeneity of the microwave field. The microwave in cesium cell, emitted by a function generator, shows inhomogeneous behavior such that the atoms interacting with the laser field experience the different fields, leading to the line broadened and multi-peak EIT-AT spectra. For the microwave transition of nS1/2-nP1/2 in this paper, a pair of EIT-AT lines should be obtained for an electric field value. The broadening of the EIT-AT spectrum and the multi-peak structure here are due to the inhomogeneity of the microwave field measurement. We propose a method to increase the spatial resolution by reducing the length of cesium cell. The result in this work provides a method of measuring the field amplitude and monitoring the distribution of microwave electric field, meanwhile the spatial resolution of the measurements can be improved by reducing the size of the cell.
Abstract Quantum electrometric sensing properties of a four-level system are theoretically investigated for microwave (MW) field measurement in thermal Rydberg atoms. In the considered system, the phenomenon of electromagnetically induced transparency (EIT) is invoked to study the impact of microwave (MW) field strength on its optical response. The amplitude of the MW electric field is obtained directly by measuring the height and frequency of EIT peaks. Further, for MW frequency measurement, the probe spectra are examined for red and blue MW detuned cases. It is found that the responsiveness of 133Cs for MW electric field as well as frequency is relatively higher than 87Rb. The overall sensitivity of both these atoms can be enhanced by the convenient setting of the system and field parameters.
A scheme for the measurement of a microwave (MW) electric field is proposed via multi-photon coherence in Rydberg atoms. It is based on the three-photon electromagnetically induced absorption (TPEIA) spectrum. In this process, the multi-photon produces a narrow absorption peak, which has a larger magnitude than the electromagnetically induced transparency (EIT) peak under the same conditions. The TPEIA peak is sensitive to MW fields, and can be used to measure MW electric field strength. We found that the magnitude of TPEIA peaks shows a linear relationship with the MW field strength. The simulation results show that the minimum detectable strength of the MW fields is about 1/10 of that based on an common EIT effect, and the probe sensitivity could be improved by about four times. Furthermore, the MW sensing based on three-photon coherence seems to be robust against the changes in the control field and shows a broad tunability, and the scheme may be useful for designing novel MW sensing devices.