Tailoring the decay rate of structured quantum emitters into their environment opens new avenues for nonlinear quantum optics, collective phenomena, and quantum communications. Here, we demonstrate a novel coupling scheme between an artificial molecule comprising two identical, strongly coupled transmon qubits and two microwave waveguides. In our scheme, the coupling is engineered so that transitions between states of the same (opposite) symmetry, with respect to the permutation operator, are predominantly coupled to one (the other) waveguide. The symmetry-based coupling selectivity, as quantified by the ratio of the coupling strengths, exceeds a factor of 30 for both waveguides in our device. In addition, we implement a Raman process activated by simultaneously driving both waveguides, and show that it can be used to coherently couple states of different symmetry in the single-excitation manifold of the molecule. Using that process, we implement frequency conversion across the waveguides, mediated by the molecule, with efficiency of about 95%. Finally, we show that this coupling arrangement makes it possible to straightforwardly generate spatially separated Bell states propagating across the waveguides. We envisage further applications to quantum thermodynamics, microwave photodetection, and photon-photon gates.
Artificially engineered atoms, built using superconducting electrical circuits, have had a broad impact on the field of quantum information and quantum computing. Based on the Josephson effect, superconducting qubits have provided a robust platform for engineering light-matter interactions at the single-photon level. The ability to precisely control and manipulate single photons using superconducting qubits and cavities, a field now popularly known as circuit quantum electrodynamics (circuit QED), has enabled new and novel regimes in quantum physics, which previously remained inaccessible. For instance, the coupling between individual photons and artificial atoms have been shown to reach the ultrastrong and deep-strong regimes, a feat which is difficult to achieve with natural atoms. The superconducting circuit platform is now a promising contender for building large-scale quantum processors, attracting large investments from academic, industry and government players. \n \nThis thesis uses superconducting circuits to engineer photon interactions in two separate studies. The first is aimed at studying the physics of ``giant" artificial-atoms. The second study explores the route towards building a quantum heat engine using two parametrically-coupled, superconducting microwave cavities. We review the theoretical ideas and concepts which motivate our work, along with discussions of the design methodology, simulations, fabrication, measurement setup and the experimental findings. \n \nIn the first study, we explore a giant artificial atom, formed from a transmon qubit, which is coupled to propagating microwaves at multiple points along an open transmission line. The multipoint coupling nature of the transmon allows its radiated field to interfere with itself leading to some striking ``giant" atom effects. For instance, we observe strong frequency dependent couplings of the transmon's transition levels to its electromagnetic environment, a feature which is not observed with ordinary artificial atoms. We measure large on/off ratios, as high as
380, for the coupling rate of the
ket0−ket1 transition. Furthermore, we show that we can enhance or suppress the coupling rate of the
ket1−ket2 transition relative to the
ket0−ket1 transition, by more than a factor of
200. The relative modulation of the coupling rates was exploited to engineer a metastable state in the giant transmon and demonstrate electromagnetically-induced transparency (EIT), a typical signature of a lambda system. Our results show that we can transform the ladder structure of an ordinary transmon into a more interesting lambda system using a giant transmon, thereby paving the way for exploring new possibilities to study three-level physics in a waveguide-QED setting. \n \nExtending giant atom physics to multiple giant atoms, we then explore a device with two giant artificial atoms connected in a braided configuration to a transmission line. The braided topology of the qubits, offers an interesting regime where the qubits can interact with each other in a decoherence-free environment, where the interaction is mediated by virtual photons in the transmission line. We probe the resonant behavior of the qubits at two different frequency bias points, where we observe qualitatively different scattering behavior. Furthermore, when probing for the Autler-Townes Splitting (ATS), multiple resonances are observed for both resonant and off-resonant cases instead of the familiar doublet in the ATS spectroscopy. This comes as a surprise as the frequency-level spacings in both qubits are nominally identical. We believe these features could be an indication of a novel resonant interaction between the qubits facilitated by the braided topology. An effort to understand this theoretically is underway. \n \nFor our second study, we explore a system with two parametrically-coupled superconducting resonators, which implements an optomechanical-like interaction in an all-electrical network. The nonlinear nature of this interaction is mediated by a superconducting quantum interference device (SQUID), where the current in one resonator couples to the photon number in the other resonator. We propose to use this system to build a ``photonic piston" engine in the quantum regime. We motivate the feasibility of the proposal by reviewing key theoretical results which demonstrate an Otto-cycle by appropriately driving the system with noise. Our experimental findings demonstrate the crucial nonlinear coupling that is required for the engine to work. We also show that we can increase the coupling strength between the resonators depending on the chosen flux operating point.
Experiments utilizing quantum optics have progressed rapidly in last few decades, particularly in the context of quantum computation, simulation, and communication. Early work in this field focused on implementations of cavity quantum electrodynamics (QED), where atoms, either natural or artificial, are strongly coupled to the confined photonic modes of cavities. However, in recent years, achieving strong coupling between atoms and itinerant photons has also gained significant interest for its applications in quantum networking. To this end, many atomic platforms are attempting to realize the waveguide QED architecture: atoms that interact with the continua of propagating photonic modes within a waveguide. In this thesis, we realize the strong-coupling regime of a waveguide QED architecture by coupling superconducting artificial atoms, typically operated as qubits, to one-dimensional transmission lines. We first demonstrate that superconducting qubits in a waveguide QED system can be used as high-quality quantum emitters. We then leverage the quantum interference between the simultaneous emission from multiple qubits in order to generate non-classical, spatially entangled, and directional itinerant microwave photons. These types of photons are particularly useful for remote entanglement and quantum communication protocols. Finally, we demonstrate that superconducting qubits can be engineered to enter novel regimes of light-matter interactions that are difficult, or even impossible, to achieve in other atomic platforms. In particular, we realize the giant-atom regime of waveguide QED, where the atom can no longer be treated as a point-like object. We use our giant atoms to implement tunable atom-waveguide couplings, as well as decoherence-free waveguide-mediated interactions between multiple atoms.
Abstract We propose an efficient scheme for microwave-to-optical quantum frequency conversion mediated by a single atom simultaneously coupled to a superconducting microwave resonator and an optical cavity. The atom mediates efficient interactions between the two electromagnetic modes via non-linear frequency mixing owing to the presence of huge microwave transition dipole moments between nearby Rydberg states as well as suitable optical transitions between low-lying states. In the regime of four-wave mixing with off-resonant fields, the excited states can be adiabatically eliminated, leading to an effective Hamiltonian that directly describes the two-mode interaction responsible for the frequency conversion. However, in this regime, the converter is slow, hence sensitive to losses due to cavity decays. To enhance the performance of the conversion process, we employ pulse engineering to tailor the atom-field couplings. The resulting protocol exhibits high robustness against decoherence and parameter fluctuations, making it well suited for realistic experimental implementations. Our scheme provides a promising route toward high-fidelity and scalable hybrid quantum interfaces connecting superconducting and optical quantum networks.
We demonstrate a superconducting artificial atom with strong unidirectional coupling to a microwave photonic waveguide.Our artificial atom is realized by coupling a transmon qubit to the waveguide at two spatially separated points with time-modulated interactions.Direction-sensitive interference arising from the parametric couplings in our scheme results in a nonreciprocal response, where we measure a forward/backward ratio of spontaneous emission exceeding 100.We verify the quantum nonlinear behavior of this artificial chiral atom by measuring the resonance fluorescence spectrum under a strong resonant drive and observing well-resolved Mollow triplets.Further, we demonstrate chirality for the second transition energy of the artificial atom and control it with a pulse sequence to realize a qubit-state-dependent nonreciprocal phase on itinerant photons.Our demonstration puts forth a superconducting hardware platform for the scalable realization of several key functionalities pursued within the paradigm of chiral quantum optics, including quantum networks with all-to-all connectivity, driven-dissipative stabilization of many-body entanglement, and the generation of complex nonclassical states of light.
Artificial atoms non-locally coupled to waveguides -- the so-called giant atoms -- offer new opportunities for the control of light and matter. In this work, we show how to use an array of non-locally coupled transmon "molecules" to engineer a passive photonic controlled gate for waveguide photons. In particular, we show that a conditional elastic phase shift between counter-propagating photons arises from the interplay between direction-dependent couplings, engineered through an interplay of non local interactions and molecular binding strength; and the nonlinearity of the transmon array. We analyze the conditions under which a maximal
π-phase shift -- and hence a CZ gate -- is obtained, and characterize the gate fidelity as a function of key experimental parameters, including finite transmon nonlinearities, emitter spectral inhomogeneities, and limited cooperativity. Our work opens the use of giant atoms as key elements of microwave photonic quantum computing devices.
Engineering light-matter interactions at the quantum level has been central to the pursuit of quantum optics for decades. Traditionally, this has been done by coupling emitters, typically natural atoms and ions, to quantized electromagnetic fields in optical and microwave cavities. In these systems, the emitter is approximated as an idealized dipole, as its physical size is orders of magnitude smaller than the wavelength of light. Recently, artificial atoms made from superconducting circuits have enabled new frontiers in light-matter coupling, including the study of ``giant'' atoms which cannot be approximated as simple dipoles. Here, we explore an implementation of a giant artificial atom, formed from a transmon qubit coupled to propagating microwaves at multiple points along an open transmission line. The nature of this coupling allows the qubit radiation field to interfere with itself, leading to some striking giant-atom effects. For instance, we observe strong frequency-dependent couplings of the qubit energy levels to the electromagnetic modes of the transmission line. Combined with the ability to in situ tune the qubit energy levels, we show that we can modify the relative coupling rates of multiple qubit transitions by more than an order of magnitude. By doing so, we engineer a metastable excited state, allowing us to operate the giant transmon as an effective lambda system where we clearly demonstrate electromagnetically induced transparency.