Engineering light-matter interactions at the quantum level has been central to the pursuit of quantum optics for decades. Traditionally, this has been done by coupling emitters, typically natural atoms and ions, to quantized electromagnetic fields in optical and microwave cavities. In these systems, the emitter is approximated as an idealized dipole, as its physical size is orders of magnitude smaller than the wavelength of light. Recently, artificial atoms made from superconducting circuits have enabled new frontiers in light-matter coupling, including the study of ``giant'' atoms which cannot be approximated as simple dipoles. Here, we explore an implementation of a giant artificial atom, formed from a transmon qubit coupled to propagating microwaves at multiple points along an open transmission line. The nature of this coupling allows the qubit radiation field to interfere with itself, leading to some striking giant-atom effects. For instance, we observe strong frequency-dependent couplings of the qubit energy levels to the electromagnetic modes of the transmission line. Combined with the ability to in situ tune the qubit energy levels, we show that we can modify the relative coupling rates of multiple qubit transitions by more than an order of magnitude. By doing so, we engineer a metastable excited state, allowing us to operate the giant transmon as an effective lambda system where we clearly demonstrate electromagnetically induced transparency.
Engineering light-matter interactions at the quantum level has been central to the pursuit of quantum optics for decades. Traditionally, this has been done by coupling emitters, typically natural atoms and ions, to quantized electromagnetic fields in optical and microwave cavities. In these systems, the emitter is approximated as an idealized dipole, as its physical size is orders of magnitude smaller than the wavelength of light. Recently, artificial atoms made from superconducting circuits have enabled new frontiers in light-matter coupling, including the study of ``giant'' atoms which cannot be approximated as simple dipoles. Here, we explore an implementation of a giant artificial atom, formed from a transmon qubit coupled to propagating microwaves at multiple points along an open transmission line. The nature of this coupling allows the qubit radiation field to interfere with itself, leading to some striking giant-atom effects. For instance, we observe strong frequency-dependent couplings of the qubit energy levels to the electromagnetic modes of the transmission line. Combined with the ability to in situ tune the qubit energy levels, we show that we can modify the relative coupling rates of multiple qubit transitions by more than an order of magnitude. By doing so, we engineer a metastable excited state, allowing us to operate the giant transmon as an effective lambda system where we clearly demonstrate electromagnetically induced transparency.
Artificially engineered atoms, built using superconducting electrical circuits, have had a broad impact on the field of quantum information and quantum computing. Based on the Josephson effect, superconducting qubits have provided a robust platform for engineering light-matter interactions at the single-photon level. The ability to precisely control and manipulate single photons using superconducting qubits and cavities, a field now popularly known as circuit quantum electrodynamics (circuit QED), has enabled new and novel regimes in quantum physics, which previously remained inaccessible. For instance, the coupling between individual photons and artificial atoms have been shown to reach the ultrastrong and deep-strong regimes, a feat which is difficult to achieve with natural atoms. The superconducting circuit platform is now a promising contender for building large-scale quantum processors, attracting large investments from academic, industry and government players. \n \nThis thesis uses superconducting circuits to engineer photon interactions in two separate studies. The first is aimed at studying the physics of ``giant" artificial-atoms. The second study explores the route towards building a quantum heat engine using two parametrically-coupled, superconducting microwave cavities. We review the theoretical ideas and concepts which motivate our work, along with discussions of the design methodology, simulations, fabrication, measurement setup and the experimental findings. \n \nIn the first study, we explore a giant artificial atom, formed from a transmon qubit, which is coupled to propagating microwaves at multiple points along an open transmission line. The multipoint coupling nature of the transmon allows its radiated field to interfere with itself leading to some striking ``giant" atom effects. For instance, we observe strong frequency dependent couplings of the transmon's transition levels to its electromagnetic environment, a feature which is not observed with ordinary artificial atoms. We measure large on/off ratios, as high as 380, for the coupling rate of the ket0−ket1 transition. Furthermore, we show that we can enhance or suppress the coupling rate of the ket1−ket2 transition relative to the ket0−ket1 transition, by more than a factor of 200. The relative modulation of the coupling rates was exploited to engineer a metastable state in the giant transmon and demonstrate electromagnetically-induced transparency (EIT), a typical signature of a lambda system. Our results show that we can transform the ladder structure of an ordinary transmon into a more interesting lambda system using a giant transmon, thereby paving the way for exploring new possibilities to study three-level physics in a waveguide-QED setting. \n \nExtending giant atom physics to multiple giant atoms, we then explore a device with two giant artificial atoms connected in a braided configuration to a transmission line. The braided topology of the qubits, offers an interesting regime where the qubits can interact with each other in a decoherence-free environment, where the interaction is mediated by virtual photons in the transmission line. We probe the resonant behavior of the qubits at two different frequency bias points, where we observe qualitatively different scattering behavior. Furthermore, when probing for the Autler-Townes Splitting (ATS), multiple resonances are observed for both resonant and off-resonant cases instead of the familiar doublet in the ATS spectroscopy. This comes as a surprise as the frequency-level spacings in both qubits are nominally identical. We believe these features could be an indication of a novel resonant interaction between the qubits facilitated by the braided topology. An effort to understand this theoretically is underway. \n \nFor our second study, we explore a system with two parametrically-coupled superconducting resonators, which implements an optomechanical-like interaction in an all-electrical network. The nonlinear nature of this interaction is mediated by a superconducting quantum interference device (SQUID), where the current in one resonator couples to the photon number in the other resonator. We propose to use this system to build a ``photonic piston" engine in the quantum regime. We motivate the feasibility of the proposal by reviewing key theoretical results which demonstrate an Otto-cycle by appropriately driving the system with noise. Our experimental findings demonstrate the crucial nonlinear coupling that is required for the engine to work. We also show that we can increase the coupling strength between the resonators depending on the chosen flux operating point.
Experiments utilizing quantum optics have progressed rapidly in last few decades, particularly in the context of quantum computation, simulation, and communication. Early work in this field focused on implementations of cavity quantum electrodynamics (QED), where atoms, either natural or artificial, are strongly coupled to the confined photonic modes of cavities. However, in recent years, achieving strong coupling between atoms and itinerant photons has also gained significant interest for its applications in quantum networking. To this end, many atomic platforms are attempting to realize the waveguide QED architecture: atoms that interact with the continua of propagating photonic modes within a waveguide. In this thesis, we realize the strong-coupling regime of a waveguide QED architecture by coupling superconducting artificial atoms, typically operated as qubits, to one-dimensional transmission lines. We first demonstrate that superconducting qubits in a waveguide QED system can be used as high-quality quantum emitters. We then leverage the quantum interference between the simultaneous emission from multiple qubits in order to generate non-classical, spatially entangled, and directional itinerant microwave photons. These types of photons are particularly useful for remote entanglement and quantum communication protocols. Finally, we demonstrate that superconducting qubits can be engineered to enter novel regimes of light-matter interactions that are difficult, or even impossible, to achieve in other atomic platforms. In particular, we realize the giant-atom regime of waveguide QED, where the atom can no longer be treated as a point-like object. We use our giant atoms to implement tunable atom-waveguide couplings, as well as decoherence-free waveguide-mediated interactions between multiple atoms.
In quantum-optics experiments with both natural and artificial atoms, the atoms are usually small enough that they can be approximated as pointlike compared to the wavelength of the electromagnetic radiation with which they interact. However, superconducting qubits coupled to a meandering transmission line, or to surface acoustic waves, can realize "giant artificial atoms" that couple to a bosonic field at several points which are wavelengths apart. Here, we study setups with multiple giant atoms coupled at multiple points to a one-dimensional (1D) waveguide. We show that the giant atoms can be protected from decohering through the waveguide, but still have exchange interactions mediated by the waveguide. Unlike in decoherence-free subspaces, here the entire multiatom Hilbert space (2^{N} states for N atoms) is protected from decoherence. This is not possible with "small" atoms. We further show how this decoherence-free interaction can be designed in setups with multiple atoms to implement, e.g., a 1D chain of atoms with nearest-neighbor couplings or a collection of atoms with all-to-all connectivity. This may have important applications in quantum simulation and quantum computing.
Waveguide circuit quantum electrodynamics (waveguide circuit QED) studies light-matter interaction with superconducting circuits in one dimension. In circuit QED, natural atoms are replaced by superconducting qubits consisting of a non-linear Josephson junction, resulting in an anharmonic energy spectrum just like real atoms. With superconducting qubits, it is possible to study quantum optical phenomena and reach new regimes hard to achieve with real atoms due to weak coupling to the electromagnetic field. The reduction to one dimension in waveguide QED increases the electromagnetic field's directionality, which results in reduced losses. In this thesis, we first introduce circuit quantisation, giving the basis for the next part, where we investigate a transmon, a charge-insensitive artificial atom, coupled to a semi-infinite transmission line. An atom coupled to a semi-infinite waveguide is referred to as an atom in front of a mirror and is the subject of all appended papers. We proceed by summarising Paper I and III's main results: in Paper I, we investigate the spontaneous emission of a transmon coupled to a semi-infinite transmission line, where we take time-delay effects into account. We find that the system dynamics strongly depend on the coupling strength to the transmission line and the atom's position with respect to the electromagnetic field, leading to the Purcell effect or the convergence to a dark state with finite excitation probability. In the high-impedance regime, which we investigate in Paper III, the properties of the transmon coupled to the high-impedance transmission line change drastically. It becomes highly reflective and creates its own cavity with the mirror, resulting in the emergence of cavity modes and vacuum Rabi oscillations in the spontaneous emission dynamics. In the next chapter of the thesis, we demonstrate how to quantise an electromagnetic field and derive a light-matter interaction Hamiltonian within dipole approximation. We then give an introduction to open quantum systems and derive the quantum-optical master equation in Lindblad form. Furthermore, we introduce the dressed state picture, where the interaction of light and matter is so strong that the individual energy levels of light and matter are no longer separable. Both the quantum optical master equation and the dressed state picture are relevant in Paper II and IV. In Paper II, an experimental collaboration, we perform several experiments to characterise and discriminate different decay rates of a superconducting qubit coupled to the end of a transmission line. One experiment measured the atomic fluorescence spectral density, which shows an asymmetry for off-resonant driving, resulting from pure dephasing: an effect that we explain in more detail in this thesis and Paper II. In Paper IV, we theoretically investigate amplification mechanisms realised by different set-ups of an atom coupled to a semi-infinite waveguide. In the considered systems, the amplification of a probe field happens either due to population inversion between the pure states or dressed states or multi-photon processes. We find that compared to an open waveguide, we can achieve a higher gain in the amplification with a semi-infinite waveguide.
The nonlocal emitter-waveguide coupling, which gives birth to the so called giant atom, represents a new paradigm in the field of quantum optics and waveguide QED. In this paper, we investigate the single-photon scattering in a one-dimensional waveguide on a two-level or three-level giant atom. Thanks to the natural interference induced by the back and forth photon transmitted/reflected at the atom-waveguide coupling points, the photon transmission can be dynamically controlled by the periodic phase modulation via adjusting the size of the giant atom. For the two-level giant-atom setup, we demonstrate the energy shift which is dependent on the atomic size. For the driven three-level giant-atom setup, it is of great interest that, the interference effect between different atomic transition paths, can lead to a complete transmission window, analogous to the electromagnetically induced transparency and beyond the two-photon resonance mechanism, and the width of the transmission valleys (reflection range) is tunable in terms of the atomic size. Our investigation will be beneficial to the photon or phonon control in quantum network based on mesoscopical or even macroscopical quantum nodes involving the giant atom.
The absorption of photons in a three-level atom can be controlled and manipulated by applying a coherent drive at one of the atomic transitions. The situation where the absorption is fully canceled, and the atom thus has been turned completely transparent, has been coined electromagnetically induced transparency (EIT). The characteristics of EIT is a narrow transparency window associated with a fluorescence quench at its center frequency, indicating that inelastic scattering at this particular point is suppressed. The emergence of EIT-like transparency windows is common in waveguide quantum electrodynamics (QED) when multiple closely spaced quantum emitters are coupled to a waveguide. The transparency depends on the separation and energy detuning of the atoms. In this work, we study a number of different setups with two-level atoms in waveguide QED that all exhibit EIT-like transparency windows. Unlike the case of a genuine three-level atom, no drive fields are required in the systems we consider, and the coherent coupling of energy levels is mediated by the waveguide. We specifically distinguish between systems with genuine EIT-like dynamics and those that exhibit a transparency window but lack the fluorescence quench. The systems that we consider consist of both small and giant atoms, which can be experimentally realized with artificial atoms coupled to either photons or phonons. These systems can offer a simpler route to many EIT applications since the need for external driving is eliminated.