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arXiv:2112.09447 · Nature Photonics

Sequential generation of multiphoton entanglement with a Rydberg superatom

Chao-Wei Yang, Yong Hui Yu, Jun Li, Bo Jing, Xiao‐Hui Bao, Jian-Wei Pan

Published Aug 11, 2022• 69 citations
arXivHTMLPDF
DOI
10.1038/s41566-022-01054-3

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Owing to the unique physical characteristics of Rydberg atoms, which play an important role in quantum information and quantum computation, the theoretical and applied research of Rydberg atoms have become the hot spots of scientific research in recent years. With the large polarizability of Rydberg atoms, even a small electric field could cause a considerable electric dipole moment, resulting in a strong dipole-dipole interaction between Rydberg atoms. The multiple excitations of the Rydberg states are strongly inhibited because of the strong dipole interaction between atoms within a mesoscopic interaction (blockade) region. We call this phenomenon the dipole blockade effect. The dipole blockade effect makes it possible to build single-photon quantum devices, implement quantum gates, generate quantum entanglement, and simulate many-body quantum problems, etc. A Rydberg atomic ensemble in the same blockade region can be regarded as a superatom. In the same way, if these atoms trapped in two optical dipole traps, each sub-ensemble can be considered as a sub-superatom which is closely related to the superatom. According to the fact that two Rydberg sub-superatoms can be strongly correlated due to sharing no more than one excited Rydberg atom, we study correlated collective excitation and quantum entanglement between two Rydberg sub-superatoms in a steady state. With the superatom model, the problem of exponentially increasing system size with the number of atoms can be circumvented to a certain extent in studying many-body physics. By solving the two-body Lindblad’s master equation accurately, we obtain the analytical expressions for the collective excitation probabilities of the two sub-superatoms, and the concurrence measuring the bipartite entanglement between them. Our results show that they are all sensitive to the number of atoms in each Rydberg superatom: the bigger (including more atoms) the Rydberg superatom, the higher the collective Rydberg excitation probability is. And that the maximally entangled state can only be obtained with two equal-sized Rydberg superatoms. When this condition is fulfilled, the mesoscopic entanglement can be generated by adding the number of atoms in each Rydberg superatom. This may provide an attractive platform for studying the quantum-classical correspondence and have potential promising applications in quantum information processing.

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Remote entanglement of matter qubits plays an important role in quantum networks and quantum repeater. Collective excitations generated via Rydberg blockade in an atomic ensemble-known as Rydberg superatoms-are promising candidates due to collectively enhanced atom-photon coupling and Rydberg-enabled nonlinearity. Here, we experimentally realize remote entanglement between two Rydberg superatoms via single-photon interference. The two setups are separated by 3 m and linked with two 20-m fibers, operated with independent control lasers. We verify that the entanglement generated is free from high-order excitation noise that is a key drawback in the traditional Duan-Lukin-Cirac-Zoller scheme. This Letter paves the way for entangling long-distance separated Rydberg superatoms at a high rate, as the success probability of a single-photon-based entangling scheme scales with the square root of the channel transmittance.