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arXiv:2112.00614 · Physical review. B./Physical review. B

Spatial emergence of off-diagonal long-range order throughout the BCS-BEC crossover

L. Pisani, P. Pieri, Giancarlo Calvanese Strinati

Published Feb 7, 2022• 6 citations
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Abstract

In a superfluid system, off-diagonal long-range order is expected to be exhibited in the appropriate reduced density matrices when the relevant particles (either bosons or fermion pairs) are considered to recede sufficiently far apart from each other. This concept is usually exploited to identify the value of the condensate density, without explicit concern, however, as to the spatial range over which this asymptotic condition can effectively be achieved. Here, based on a diagrammatic approach that includes beyond-mean-field pairing fluctuations in the broken-symmetry phase at the level of the $t$-matrix also with the inclusion of the Gorkov-Melik-Barkhudarov (GMB) correction, we present a systematic study of the two-particle reduced density matrix for a superfluid fermionic system undergoing the BCS-BEC crossover, when the entities to recede far apart from each other evolve with continuity from largely overlapping Cooper pairs in the BCS limit to dilute composite bosons in the BEC limit. By this approach, we not only provide the coupling and temperature dependence of the condensate density at the level of our diagrammatic approach, which includes the GMB correction, but we also obtain the evolution of the spatial dependence of the two-particle reduced density matrix, from a power law at low temperature to an exponential dependence at high temperature in the superfluid phase, when the interparticle coupling spans the BCS-BEC crossover. Our results put limitations on the minimum spatial extent of a finite-size system for which superfluid correlations can effectively be established.

DOI
10.1103/physrevb.105.054505

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In a superfluid system, off-diagonal long-range order is expected to be exhibited in the appropriate reduced density matrices when the relevant particles (either bosons or fermion pairs) are considered to recede sufficiently far apart from each other. This concept is usually exploited to identify the value of the condensate density, without explicit concern, however, as to the spatial range over which this asymptotic condition can effectively be achieved. Here, based on a diagrammatic approach that includes beyond-mean-field pairing fluctuations in the broken-symmetry phase at the level of the ttt-matrix also with the inclusion of the Gorkov-Melik-Barkhudarov (GMB) correction, we present a systematic study of the two-particle reduced density matrix for a superfluid fermionic system undergoing the BCS-BEC crossover, when the entities to recede far apart from each other evolve with continuity from largely overlapping Cooper pairs in the BCS limit to dilute composite bosons in the BEC limit. By this approach, we not only provide the coupling and temperature dependence of the condensate density at the level of our diagrammatic approach, which includes the GMB correction, but we also obtain the evolution of the spatial dependence of the two-particle reduced density matrix, from a power law at low temperature to an exponential dependence at high temperature in the superfluid phase, when the interparticle coupling spans the BCS-BEC crossover. Our results put limitations on the minimum spatial extent of a finite-size system for which superfluid correlations can effectively be established.
We consider the current correlation function for a three-dimensional system of fermions embedded in a homogeneous background and mutually interacting via an attractive short-range potential, below the (superconducting) critical temperature. Diagrammatic contributions in the broken-symmetry phase are identified, which yield for the (wave-vector and frequency-dependent) current correlation function the fermionic BCS approximation in the weak-coupling limit and the bosonic Bogoliubov approximation in the strong-coupling limit (whereby composite bosons form as bound-fermion pairs). The temperature dependence of the superfluid density (from the BCS exponential behavior at weak coupling to a power-law behavior at strong coupling) and the form of the Pippard-like kernel at zero temperature are explicitly obtained from weak to strong coupling. Quite generally, it is shown that the Pippard-like kernel is the sum of a local (London-like) term and of a nonlocal component, the local term being dominant in the strong-coupling limit and the nonlocal component in the BCS (weak-coupling) limit. It is also shown that the range of the nonlocal component is determined by the coherence length measuring the spatial correlations of the amplitude of the order parameter, namely, the correlations among different Cooper pairs (or composite bosons), rather than between the fermionic partners of a given pair. In addition, a prescription is provided for mapping the fermionic onto the bosonic diagrammatic theories in the broken-symmetry phase, thus complementing what has been already done in the normal phase.
It has long been known that the critical temperature of a BCS weak-coupling superfluid gets considerably reduced when the Gorkov-Melik-Barkhudarov (G-MB) correction is considered, whereby particle-hole excitations affect the two-fermion scattering in the medium responsible the formation of Cooper pairs. Here, by a careful analysis which takes into account the wave-vector and frequency dependence of the pair propagator (which gets increasingly important away from the weak coupling limit where the G-MB correction was originally derived) we extend the effects of the G-MB correction throughout the BCSBEC crossover. In particular, the Feynman diagram responsible for the G-MB correction is inserted in a partially self-consistent T-matrix scheme; the resulting equations are solved numerically and yield a curve for the critical temperature which agrees very well with the Quantum Monte Carlo data available in the crossover region.
The equation for the gap parameter represents the main equation of the pairing theory of superconductivity. Although it is formally defined through a single-particle property, physically, it reflects the pairing correlations between opposite-spin fermions. Here, we exploit this physical connection and cast the gap equation in an alternative form which explicitly highlights these two-particle correlations by showing that it is equivalent to a Hugenholtz-Pines condition for fermion pairs. At a formal level, a direct connection is established in this way between the treatment of the condensate fraction in condensate systems of fermions and bosons. At a practical level, the use of this alternative form of the gap equation is expected to make easier the inclusion of pairing fluctuations beyond mean field. As a proof-of-concept of the new method, we apply the modified form of the gap equation to the long-pending problem about the inclusion of the Gorkov-Melik-Barkhudarov correction across the whole BCS-BEC crossover, from the BCS limit of strongly overlapping Cooper pairs to the BEC limit of dilute composite bosons, and for all temperatures in the superfluid phase. Our numerical calculations yield excellent agreement with the recently determined experimental values of the gap parameter for an ultracold Fermi gas in the intermediate regime between BCS and BEC, as well as with the available quantum Monte Carlo data in the same regime.
The problem of the evolution from BCS theory with cooperative Cooper pairing to the formation and condensation of composite bosons has attracted considerable attention for the past several decades. It has gained renewed impetus in the mid-eighties with the discovery of the high-Tc superconductors, which have a coherence length comparable to the interparticle spacing. More recently, this subject has spurred a great deal of research activity in connection with experiments involving dilute atomic gases of fermionic atoms. The initial objective of this work will be to use functional integral techniques to analyze the low-temperature BCS-to-BEC evolution of d-wave superconductors within the saddle point (mean field) approximation for a continuum model. Then, the same mathematical formalism will be applied to the problem of the BCS-to-BEC evolution of fully spin-polarized p-wave Fermi gases in two dimensions. We find that a quantum phase transition occurs for both systems as they are driven from the BCS-like regime of weakly interacting fermionic pairs to the opposite BEC-like regime of strongly interacting bosonic molecules. This is in contrast to the smooth crossover predicted and observed in systems that exhibit s-wave pairing symmetry. We calculate several spectroscopic and thermodynamic properties that signal the occurrence of this phase transition, and suggest some possible experimental realizations. Finally, fluctuations about the saddle point solution are included in the calculations, and the effects of such correction are analyzed in the low (T~0) and high (T~Tc) temperature limits. We conclude that, at high temperatures, the bosonic degrees of freedom that arise from two-particle bound states become essential to describe the strong coupling limit,\nas the saddle point approximation alone becomes unreliable.
The Josephson current-phase characteristics, that arise when a supercurrent flows across two fermionic superfluids separated by a potential barrier, can be controlled by varying either the interparticle coupling or the temperature. While the coupling dependence has been addressed in detail both theoretically and experimentally for an attractive Fermi gas undergoing the BCS-BEC crossover, a corresponding study of the temperature dependence of the Josephson characteristics is still lacking in this context. Here, we investigate the combined coupling and temperature dependence of the Josephson characteristics in a systematic way for a wide set of barriers, within ranges of height and width that can be experimentally explored. Our study smoothly connects the two limiting cases, of nonoverlapping composite bosons at low temperature described by the Gross-Piatevskii equation, and of strongly overlapping Cooper pairs near the critical temperature described by the Ginzburg-Landau equation. In this way, we are able to explore several interesting effects related to how the current-phase characteristics evolve along the BCS-BEC crossover as a function of temperature and of barrier shape. These effects include the coherence length outside the barrier and the pair penetration length inside the barrier (which is related to the proximity effect), as well as the temperature evolution of the Landau criterion in the limit of a vanishingly small barrier. A comparison is also presented between the available experimental data for the critical current and our theoretical results over a wide range of couplings along the BCS-BEC crossover.
We consider the problem of the crossover from BCS superconductivity to Bose-Einstein condensation in three dimensions for a system of fermions with a mutual attractive interaction, for which we adopt the simplifying assumption of a suitably regularized point-contact interaction. We examine in a critical way the fermionic (self-consistent) T-matrix approximation, which has been widely utilized in the literature to describe this crossover above the superconducting critical temperature, and show that it fails to yield the correct behavior of the system in the strong-coupling limit, where composite bosons form as tightly bound fermion pairs. We then set up the correct approximation for a ``dilute'' system of composite bosons and show that a class of diagrams has to be considered in the place of the fermionic T-matrix approximation for the self-energy. This class of diagrams correctly describes both the weak- and strong-coupling limits, and consequently results in an improved interpolation scheme for the intermediate (crossover) region. In this context, we provide also a systematic mapping between the corresponding diagrammatic theories for the composite bosons and the constituent fermions. As a preliminary result to demonstrate the numerical effect of our class of diagrams on physical quantities, we calculate the value of the scattering length for composite bosons in the strong-coupling limit and show that it is considerably modified with respect to the result obtained within the self-consistent fermionic T-matrix approximation.