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arXiv:2111.14852 · Physical review. B./Physical review. B

Thermodynamics of an exactly solvable model for superconductivity in a doped Mott insulator

Jinchao Zhao, Luke Yeo, Edwin W. Huang, Philip Phillips

Published May 12, 2022• 22 citations
arXivHTMLPDF

Abstract

Computing superconducting properties starting from an exactly solvable model for a doped Mott insulator stands as a grand challenge. We have recently shown that this can be done starting from the Hatsugai-Kohmoto (HK) model, which can be understood generally as the minimal model that breaks the nonlocal ${\mathbb{Z}}_{2}$ symmetry of a Fermi liquid, thereby constituting a new quartic fixed point for Mott physics [Phillips et al., Nat. Phys. 16, 1175 (2020); Huang et al., Nat. Phys. (2022)]. In the current paper, we compute the thermodynamics, condensation energy, and electronic properties such as the NMR relaxation rate $1/{T}_{1}$ and ultrasonic attenuation rate. Key differences arise with the standard BCS analysis from a Fermi liquid: (1) the free energy exhibits a local minimum at ${T}_{p}$ where the pairing gap turns on discontinuously above a critical value of the repulsive HK interaction, thereby indicating a first-order transition; (2) a tricritical point emerges, thereby demarcating the boundary between the standard second-order superconducting transition and the novel first-order regime; (3) Mottness changes the sign of the quartic coefficient in the Landau-Ginzburg free-energy functional relative to that in BCS; (4) as this obtains in the strongly interacting regime, it is Mott physics that underlies the generic first-order transition; (5) the condensation energy exceeds that in BCS theory suggesting that multiple Mott bands might be a way of enhancing superconducting; (6) the heat-capacity jump is nonuniversal and increases with the Mott scale; (7) Mottness destroys the Hebel-Slichter peak in NMR; and (8) Mottness enhances the fall-off of the ultrasonic attenuation at the pairing temperature ${T}_{p}$. As several of these properties are observed in the cuprates, our analysis here points a way forward in computing superconducting properties of strongly correlated electron matter.

DOI
10.1103/physrevb.105.184509

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Computing superconducting properties starting from an exactly solvable model for a doped Mott insulator stands as a grand challenge. We have recently shown that this can be done starting from the Hatsugai-Kohmoto (HK) model, which can be understood generally as the minimal model that breaks the nonlocal Z2{\mathbb{Z}}_{2}Z2​ symmetry of a Fermi liquid, thereby constituting a new quartic fixed point for Mott physics [Phillips et al., Nat. Phys. 16, 1175 (2020); Huang et al., Nat. Phys. (2022)]. In the current paper, we compute the thermodynamics, condensation energy, and electronic properties such as the NMR relaxation rate 1/T11/{T}_{1}1/T1​ and ultrasonic attenuation rate. Key differences arise with the standard BCS analysis from a Fermi liquid: (1) the free energy exhibits a local minimum at Tp{T}_{p}Tp​ where the pairing gap turns on discontinuously above a critical value of the repulsive HK interaction, thereby indicating a first-order transition; (2) a tricritical point emerges, thereby demarcating the boundary between the standard second-order superconducting transition and the novel first-order regime; (3) Mottness changes the sign of the quartic coefficient in the Landau-Ginzburg free-energy functional relative to that in BCS; (4) as this obtains in the strongly interacting regime, it is Mott physics that underlies the generic first-order transition; (5) the condensation energy exceeds that in BCS theory suggesting that multiple Mott bands might be a way of enhancing superconducting; (6) the heat-capacity jump is nonuniversal and increases with the Mott scale; (7) Mottness destroys the Hebel-Slichter peak in NMR; and (8) Mottness enhances the fall-off of the ultrasonic attenuation at the pairing temperature Tp{T}_{p}Tp​. As several of these properties are observed in the cuprates, our analysis here points a way forward in computing superconducting properties of strongly correlated electron matter.
We establish the Hatsugai-Kohmoto model as a stable quartic fixed point (distinct from Wilson-Fisher) by computing the $\ensuremath{\beta}$ function in the presence of perturbing local interactions. In vicinity of the half-filled doped Mott state, the $\ensuremath{\beta}$ function vanishes for all local interactions regardless of their sign. The only flow away from the HK model is through the superconducting channel which lifts the spin degeneracy as does any ordering tendency. The superconducting instability is identical to that established previously [Phillips et al., Nat. Phys. 16, 1175 (2020)]. A corollary of this work is that any system in which the spectral weight bifurcates into lower and upper bands such as the Hubbard model with repulsive interactions flows into the HK stable fixed point in the vicinity of half-filling. Consequently, although the HK model has all-to-all interactions, the bifurcation of the spectral weight is stable as nothing local destroys it. The consilience with Hubbard arises because both models break the Z2{Z}_{2}Z2​ symmetry on a Fermi surface, the HK model being the simplest to do so. Indeed, the simplicity of the HK model belies its robustness and generality.
This pedagogic review aims to give a gentle introduction to an exactly solvable model, the Hatsugai-Kohmoto (HK) model, which has infinite-ranged interaction but conserves the center of mass. Although this model is invented in 1992, intensive studies on its properties ranging from unconventional superconductivity, topological ordered states to non-Fermi liquid behaviors are made since 2020. We focus on its emergent non-Fermi liquid behavior and provide discussion on its thermodynamics, single-particle and two-particle correlation functions. Perturbation around solvable limit has also been explored with the help of perturbation theory, renormalization group and exact diagonalization calculation. We hope the present review will be helpful for graduate students or researchers interested in HK-like models or more generic strongly correlated electron systems.
Abstract Superconductivity in strongly correlated electrons can emerge out from a normal state that is beyond the Landau’s Fermi liquid paradigm, often dubbed as ‘non-Fermi liquid’. While the theory for non-Fermi liquid is still not yet conclusive, a recent study on the exactly-solvable Hatsugai–Kohomoto (HK) model has suggested a non-Fermi liquid ground state whose Green’s function resembles the Yang–Rice–Zhang ansatz for cuprates (2020 Phillips et al Nat. Phys. 16 1175). Similar to the effect of on-site Coulomb repulsion in the Hubbard model, the repulsive interaction in the HK model divides the momentum space into three parts: empty, single-occupied and double-occupied regions, that are separated from each other by two distinct Fermi surfaces. In the presence of an additional Bardeen–Cooper–Schrieffer-type pairing interaction of a moderate strength, we show that the system exhibits a ‘two-stage superconductivity’ feature as temperature decreases: a first-order superconducting transition occurs at a temperature T c that is followed by a sudden increase of the superconducting order parameter at a lower temperature T c ′ < T c . At the first stage, T c ′ < T < T c , the pairing function arises and the entropy is released only in the vicinity of the two Fermi surfaces; while at the second stage, T < T c ′ , the pairing function becomes significant and the entropy is further released in deep (single-occupied) region in the Fermi sea. The phase transitions are analyzed within the Ginzburg–Landau theory. Our work sheds new light on unconventional superconductivity in strongly correlated electrons.
We investigate the Hatsugai-Kohmoto (HK) model on a square lattice, which describes both a Mott insulator at half-filling and a non-Fermi liquid phase on doping. Through the solution of this exactly solvable model with the inclusion of pairing interactions, we demonstrate the emergence of strong pair-density-wave (PDW) fluctuations associated with center-of-mass momentum $\mathbf{Q}=(\ensuremath{\pi},\ensuremath{\pi})$ at finite temperatures for low dopings up to a critical doping and intermediate UUU interaction. Furthermore, we also confirm that a superconducting instability appears in the model within a wide regime of interaction UUU and doping parameter xxx. In view of the fact that it has been recently put forward that the metal-insulator transition of the HK model belongs to the same universality class as the Mott transition of the paradigmatic Hubbard model [Huang et al., Nat. Phys. 18, 511 (2022)], our work may thus shed light on an interesting scenario regarding the emergence of a fluctuating PDW phase on doping a Mott insulator, which has been argued to be relevant for understanding the physics of the cuprate superconductors in the underdoped regime.
Though most fermionic Mott insulators order at low temperatures, ordering is ancillary to their insulating behavior. Our emphasis here is on disentangling ordering from the intrinsic strongly correlated physics of a doped half-filled band. To this end, we focus on the two-dimensional Hubbard model. Because the charge gap arises from on-site correlations, we have been refining the nonperturbative approach of Matsumoto and Mancini [Phys. Rev. B 55, 2095 (1997)] which incorporates local physics. Crucial to this method is a self-consistent two-site dynamical cluster expansion which builds in the nearest-neighbor energy scale J. At half-filling, we find that the spectral function possesses a gap of order U and is devoid of any coherent quasiparticle peaks although ordering or charge fractionalization are absent. At low temperatures, local antiferromagnetic correlations emerge. In the doped case, we find that the Fermi surface exceeds the Luttinger volume. The breakdown of Luttinger's theorem in the underdoped regime is traced both to the dynamically generated Mott gap as well to a nonvanishing of the imaginary part of the self-energy at the Fermi level. Spectral weight transfer across the Mott gap also emerges as a ubiquitous feature of a doped Mott insulator and suggests that high- and low-energy scales are inseparable. Additionally in the underdoped regime, we find that a pseudogap exists in the single-particle density of states as well as in the heat capacity. The pseudogap (which is set by the energy scale t2/U){t}^{2}/U)t2/U) is argued to be a ubiquitous feature of a lightly doped Mott state and simply represents the fact that hole transport involves double occupancy. In analogy with the Mott gap and antiferromagnetism, we propose that ordering may also accompany the formation of a pseudogap. We suggest a current pattern within a one-band model that preserves translational but breaks time-reversal symmetry along the canonical x and y axes but not along $x=\ifmmode\pm\else\textpm\fi{}y$ that is consistent with the experimental observations. Finally, we show that the Hall coefficient in a doped Mott insulator must change sign at a doping level x<1/3.x<1/3.x<1/3. The sign change is tied to a termination of strong correlation physics in the doped Mott state.
Abstract We present a T = 0 K renormalization group (RG) phase diagram for the hole-doped 2D Hubbard model on the square lattice. The RG method employed is nonperturbative in treating quantum fluctuations of the single-particle occupation number via the unitarily decoupling of one electronic state at every RG step. As a result, the RG phase diagram possesses the quantum fluctuation energy scale (ω) as one of its axes. Using effective Hamiltonians and wavefunctions for the low-energy many-body eigenstates for the doped Mott liquid obtained from the stable fixed point of the RG flows, we demonstrate the collapse of the pseudogap for charge excitations (Mottness) at a quantum critical point (QCP) possessing a nodal non-Fermi liquid with superconducting fluctuations, and spin-pseudogapping near the antinodes. The QCP is characterised using both thermodynamic and quantum information-theoretic measures. d-wave superconducting order is shown to arise from this quantum critical state of matter. The pseudogap phase possesses a variety of fluctuations that lead to several symmetry-broken phases at low-energies. Benchmarking of the ground state energy per particle and the double-occupancy fraction obtained from a finite-size scaling analysis against existing numerical results yields excellent agreement. We present detailed insight into the T = 0 origin of several experimentally observed findings in the cuprates, including Homes law and Planckian dissipation. We also establish that the heirarchy of temperature scales for the pseudogap (T PG), onset temperature for pairing (T ons), formation of the Mott liquid (T ML) and superconductivity (T C) obtained from our analysis is quantitatively consistent with that observed experimentally for some members of the cuprates. Our results offer insight on the ubiquitous origin of superconductivity in doped Mott insulating states, and pave the way towards a systematic search for higher superconducting transition temperatures in such systems.