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arXiv:2110.14539 · Physical review. B./Physical review. B

Decoupling of the many-body effects from the electron mass in GaAs by means of reduced dimensionality

Pedro M. T. Vianez, Yizheng Jin, W. K. Tan, Q. Liu, Jonathan Griffiths, Ian A. Farrer, D. A. Ritchie, Oleksandr Tsyplyatyev, C. J. B. Ford

Published Mar 13, 2023• 2 citations
arXivHTMLPDF

Abstract

Determining the (bare) electron mass ${m}_{0}$ in crystals is often hindered by many-body effects since Fermi-liquid physics renormalizes the band mass, making the observed effective mass ${m}^{*}$ depend on density. Here, we use a one-dimensional (1D) geometry to amplify the effect of interactions, forcing the electrons to form a nonlinear Luttinger liquid with separate holon and spinon bands, therefore separating the interaction effects from ${m}_{0}$. Measuring the spectral function of gated quantum wires formed in GaAs by means of magnetotunnelling spectroscopy and interpreting them using the 1D Fermi-Hubbard model, we obtain ${m}_{0}=(0.0525\ifmmode\pm\else\textpm\fi{}0.0015){m}_{\text{e}}$ in this material, where ${m}_{\text{e}}$ is the free-electron mass. By varying the density in the wires, we change the interaction parameter ${r}_{\text{s}}$ in the range from $\ensuremath{\sim}1$--4 and show that ${m}_{0}$ remains constant. The determined value of ${m}_{0}$ is $\ensuremath{\sim}22%$ lighter than observed in GaAs in geometries of higher dimensionality $D$ ($D>1$), consistent with the quasiparticle picture of a Fermi liquid that makes electrons heavier in the presence of interactions.

DOI
10.1103/physrevb.107.115128

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Determining the (bare) electron mass m0{m}_{0}m0​ in crystals is often hindered by many-body effects since Fermi-liquid physics renormalizes the band mass, making the observed effective mass m∗{m}^{*}m∗ depend on density. Here, we use a one-dimensional (1D) geometry to amplify the effect of interactions, forcing the electrons to form a nonlinear Luttinger liquid with separate holon and spinon bands, therefore separating the interaction effects from m0{m}_{0}m0​. Measuring the spectral function of gated quantum wires formed in GaAs by means of magnetotunnelling spectroscopy and interpreting them using the 1D Fermi-Hubbard model, we obtain m0=(0.0525\ifmmode±\else\textpm\fi0.0015)me{m}_{0}=(0.0525\ifmmode\pm\else\textpm\fi{}0.0015){m}_{\text{e}}m0​=(0.0525\ifmmode±\else\textpm\fi0.0015)me​ in this material, where me{m}_{\text{e}}me​ is the free-electron mass. By varying the density in the wires, we change the interaction parameter rs{r}_{\text{s}}rs​ in the range from \ensuremath∼1\ensuremath{\sim}1\ensuremath∼1--4 and show that m0{m}_{0}m0​ remains constant. The determined value of m0{m}_{0}m0​ is \ensuremath∼22\ensuremath{\sim}22%\ensuremath∼22 lighter than observed in GaAs in geometries of higher dimensionality DDD (D>1D>1D>1), consistent with the quasiparticle picture of a Fermi liquid that makes electrons heavier in the presence of interactions.
One-dimensional electronic fluids are peculiar conducting systems, where the fundamental role of interactions leads to exotic, emergent phenomena, such as spin-charge (spinon-holon) separation. The distinct low-energy properties of these 1D metals are successfully described within the theory of linear Luttinger liquids, but the challenging task of describing their high-energy nonlinear properties has long remained elusive. Recently, novel theoretical approaches accounting for nonlinearity have been developed, yet the rich phenomenology that they predict remains barely explored experimentally. Here, we probe the nonlinear spectral characteristics of short GaAs quantum wires by tunnelling spectroscopy, using an advanced device consisting of 6000 wires. We find evidence for the existence of an inverted (spinon) shadow band in the main region of the particle sector, one of the central predictions of the new nonlinear theories. A (holon) band with reduced effective mass is clearly visible in the particle sector at high energies.
The properties of fermions in one dimension are markedly different from those in higher dimensions. In two or three dimensions, the many-body behaviour of fermions is described by the Fermi liquid model, whose most prominent result is that, instead of studying the behaviour of individual particles, it is better to describe the emergent phenomena of the whole system, known as quasiparticles. These are collective modes of excitations born out of particle-particle interactions, which resemble the constituent single particles, albeit with renormalised mass. In one dimension, however, the formation of such a correlated state is unfavourable and the quasiparticles are completely absent. Instead, 1D fermions are described by a model known as the Tomonaga-Luttinger liquid. Central to this model is the process of bosonisation, a mathematical technique which maps the excitation of fermions to bosonic modes of spin-density and charge-density waves. As a prerequisite of the bosonisation technique, the fermionic single-particle dispersion is approximated as a linear function. Consequently, the Luttinger liquid model is limited in its scope of applicability. Specifically, it is valid only in the vicinity of the Fermi points, where the excitation energy is low. Recent advancement in the theoretical field has expanded our understanding of 1D interacting fermions beyond the limit of linearity. The mobile-impurity model, proposed by L. Glazman and his co-authors, is a generalised model of 1D fermions which extends the scope of applicability of the Tomanaga-Luttinger model, accounting for the curvature of single-particle dispersion relations. It extends the region of validity of the tradition TLL theory from the neighbourhood of the Fermi points to a band which follows the single-particle dispersion. This thesis presents the results of an experimental work which provides direct evidence of non-linear behaviour predicted by the new model. It revolves around the measurement of the spectral function of electrons in surface-gate-defined quantum wires on a double-quantum-well, GaAs/AlGaAs device, and the comparison and fitting of the result to the non-linear theory. The spectral function is a theoretical concept frequently used in discussions on many-body problems. Its physical interpretation makes it closely related to experimental observables, such as the tunnelling current between the double quantum wells in this work. This thesis consists of three parts. Part one concerns the theories of the various many-body models and the experimental technique: Chapter 1 briefly introduces the concept of Fermi liquid, before focusing on a detailed account of the Luttinger-liquid model. The mobile-impurity model will be introduced in the framework of the Luttinger liquid model afterwards, followed by a review of experimental works reported in the literature on the study of TLL physics. In Chapter 2, the principles of the experimental tunnelling spectroscopy technique are described. The second part of the thesis details the structure of the test device used in the experiment and its fabrication. In particular, we will discuss the intricacies of the three-dimensional EBL fabrication process developed specifically for this project. The setup and running of the measurement circuit will also be discussed in this part of the thesis, in the context of a prerequisite sample characterisation measurement. In the final part of the work, data from the main experiment will be presented and analysed, in search for the electron-electron interaction effects which are predicted by the theoretical discussions in the first chapter.
Experiments on quasi-one-dimensional systems such as quantum wires and metallic chains on surfaces suggest the existence of electron-electron interactions of substantial range and hence physics beyond the Hubbard model. We therefore investigate one-dimensional, quarter-filled chains with a Coulomb potential with variable screening length by quantum Monte Carlo methods and exact diagonalization. The Luttinger liquid interaction parameter ${K}_{\ensuremath{\rho}}$ decreases with increasing interaction strength and range. Experimentally observed values close to 1/4 require strong interactions and/or large screening lengths. As predicted by bosonization, we find a metal-insulator transition at ${K}_{\ensuremath{\rho}}=1/4$. Upon increasing the screening length, the charge and spin correlation functions reveal the crossover from dominant 2kF2{k}_{\mathrm{F}}2kF​ spin correlations to dominant 4kF4{k}_{\mathrm{F}}4kF​ charge correlations, and a strong enhancement of the charge velocity. In the metallic phase, the signatures of spin-charge separation in the single-particle spectrum, spinon and holon bands, remain robust even for rather long-ranged interactions. The charge-density-wave state exhibits backfolded shadow bands.
The natural excitations of an interacting one-dimensional system at low energy are the hydrodynamic modes of a Luttinger liquid, protected by the Lorentz invariance of the linear dispersion. We show that beyond low energies, where the quadratic dispersion reduces the symmetry to Galilean, the main character of the many-body excitations changes into a hierarchy: calculations of dynamic correlation functions for fermions (without spin) show that the spectral weights of the excitations are proportional to powers of R2/L2{\mathcal{R}}^{2}/{L}^{2}R2/L2, where R\mathcal{R}R is a length-scale related to interactions and LLL is the system length. Thus only small numbers of excitations carry the principal spectral power in representative regions on the energy-momentum planes. We have analyzed the spectral function in detail and have shown that the first-level (strongest) excitations form a mode with parabolic dispersion, like that of a renormalized single particle. The second-level excitations produce a singular power-law line shape to the first-level mode and multiple power laws at the spectral edge. We have illustrated a crossover to a Luttinger liquid at low energy by calculating the local density of states through all energy scales: from linear to nonlinear, and to above the chemical potential energies. In order to test this model, we have carried out experiments to measure the momentum-resolved tunneling of electrons (fermions with spin) from/to a wire formed within a GaAs heterostructure. We observe a well-resolved spin-charge separation at low energy with appreciable interaction strength and only a parabolic dispersion of the first-level mode at higher energies. We find a structure resembling the second-level excitations, which dies away rapidly at high momentum in line with the theoretical predictions here.
A system of one-dimensional electrons interacting via a short-range potential described by Hubbard model is considered in the regime of strong coupling using the Bethe ansatz approach. We study its momentum distribution function at zero temperature and find one additional singularity at the 3kF3{k}_{\mathrm{F}}3kF​ point. We identify that the second singularity is of the same Luttinger liquid type as the low-energy one at kF{k}_{\mathrm{F}}kF​. By calculating the spectral function simultaneously, we show that the second Luttinger liquid at 3kF3{k}_{\mathrm{F}}3kF​ is formed by charge modes only, unlike the known one around kF{k}_{\mathrm{F}}kF​ consisting of both spin and charge modes. This result reveals the ability of the spin-charge separation effect to split the Fermi point of free electrons into two, demonstrating its robustness beyond the low-energy limit of Luttinger liquid where it was originally found.
The low-energy properties of a homogeneous one-dimensional electron system are completely specified by two Tomonaga-Luttinger parameters ${K}_{\ensuremath{\rho}}$ and ${v}_{\ensuremath{\sigma}}.$ In this paper we discuss microscopic estimates of the values of these parameters in semiconductor quantum wires that exploit their relationship to thermodynamic properties. Motivated by the recognized similarity between correlations in the ground state of a one-dimensional electron liquid and correlations in a Wigner crystal, we evaluate these thermodynamic quantities in a self-consistent Hartree-Fock approximation. According to our calculations, the Hartree-Fock approximation ground state is a Wigner crystal at all electron densities and has antiferromagnetic order that gradually evolves from spin-density wave to localized in character as the density is lowered. Our results for ${K}_{\ensuremath{\rho}}$ are in good agreement with weak-coupling perturbative estimates ${K}_{\ensuremath{\rho}}^{\mathrm{pert}}$ at high densities, but deviate strongly at low densities, especially when the electron-electron interaction is screened at long distances. ${K}_{\ensuremath{\rho}}^{\mathrm{pert}}\ensuremath{\sim}{n}^{1/2}$ vanishes at small carrier density n, whereas we conjecture that ${K}_{\ensuremath{\rho}}\ensuremath{\rightarrow}1/2$ when $\stackrel{\ensuremath{\rightarrow}}{n}0,$ implying that ${K}_{\ensuremath{\rho}}$ should pass through a minimum at an intermediate density. Observation of this nonmonotonic dependence could be used to measure the effective interaction range in a realistic semiconductor quantum wire geometry. In the spin sector we find that the spin velocity decreases with increasing interaction strength or decreasing n. Strong correlation effects make it difficult to obtain fully consistent estimates of ${v}_{\ensuremath{\sigma}}$ from Hartree-Fock calculations. We conjecture that ${v}_{\ensuremath{\sigma}}{/v}_{\mathrm{F}}\ensuremath{\propto}{n/V}_{0},$ where V0{V}_{0}V0​ is the interaction strength, in the limit $\stackrel{\ensuremath{\rightarrow}}{n}0.$