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arXiv:2110.13322 · Photonics Research

Submegahertz spectral width photon pair source based on fused silica microspheres

Erasto Ortiz-Ricardo, Cesar Bertoni-Ocampo, Mónica Maldonado-Terrón, Arturo Garcia Zurita, Roberto Ramírez-Alarcón, Hector Cruz Ramirez, Rigoberto Castro‐Beltrán, Alfred B. U’Ren

Published Sep 1, 2021• 24 citations
arXivHTMLPDF

Abstract

High-efficiency submegahertz bandwidth photon pair generators will enable the field of quantum technology to transition from laboratory demonstrations to transformational applications involving information transfer from photons to atoms. While spontaneous parametric processes are able to achieve high-efficiency photon pair generation, the spectral bandwidth tends to be relatively large, as defined by phase-matching constraints. To solve this fundamental limitation, we use an ultrahigh quality factor ( Q ) fused silica microsphere resonant cavity to form a photon pair generator. We present the full theory for the spontaneous four-wave mixing (SFWM) process in these devices, fully taking into account all relevant source characteristics in our experiments. The exceptionally narrow (down to kilohertz-scale) linewidths of these devices result in a reduction in the bandwidth of the photon pair generation, allowing submegahertz spectral bandwidth to be achieved. Specifically, using a pump source centered around 1550 nm, photon pairs with the signal and idler modes at wavelengths close to 1540 and 1560 nm, respectively, are demonstrated. We herald a single idler-mode photon by detecting the corresponding signal photon, filtered via transmission through a wavelength division multiplexing channel of choice. We demonstrate the extraction of the spectral profile of a single peak in the single-photon frequency comb from a measurement of the signal–idler time of emission distribution. These improvements in device design and experimental methods enabled the narrowest spectral width ( Δ ν = 366 kHz ) to date in a heralded single-photon source based on SFWM.

DOI
10.1364/prj.435521

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Submegahertz spectral width photon-pair source based on fused silica microspheres

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We demonstrate, and characterize, a photon-pair source based on the process of spontaneous four wave mixing in fused-silica microspheres, with single heralded photon bandwidths down to 366kHz [1].

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Submegahertz spectral width photon-pair source based on fused silica microspheres

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Photonic quantum technologies require efficient sources of pure single photons. We present a heralded single-photon source based on spontaneous parametric down-conversion in a monolithic cavity optimized for high spectral and spatial purity. The source heralds single photons at a wavelength of 1540 nm and a spectral bandwidth of 168 MHz, with a maximum heralding efficiency of 70% including all transmission and detection losses, while keeping the multi-photon contamination below 3%. The cavity enhancement predominantly generates photons into the central cavity mode, with a theoretical upper bound on the spectral purity of 79.4% arising from nonzero overlap with adjacent cavity modes. Spectral isolation of the central cavity mode with an etalon yields an increased measured spectral purity of (96.2 $\pm$ 2.7)%.

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We demonstrate theoretically the direct (filter-free) generation of spectrally uncorrelated photon pairs, and consequently high-purity heralded single photons at telecommunication wavelengths, in SOI (silicon-on-insulator) nanowaveguides via spontaneous four-wave mixing (SFWM). The inherent strong waveguide dispersion in such high-index contrast structures is employed for discrete-band phase-matching in order to suppress the pair spectral correlations, and to produce photons in the fundamental spatial mode for easy in-out coupling to single-mode optical fibers. Additionally, by optimizing the source parameters like waveguide length, dispersion and pump bandwidth, the group-velocity of generated photons is also engineered to further eliminate spectral correlations. Extensive numerical mode simulations for various waveguide widths are used to design intrinsically pure photon sources via joint spectral amplitude (JSA) engineering. Purity$>$95% is shown to be achievable in a silica-clad SOI waveguide with a cross-section 220 × 600 nm$^{2}$for typical values of length and pump bandwidth. The wavelength of these heralded single photons can be tuned in the range of 1266–1363 nm ($\sim$O-band) by varying the pump wavelength. Considering the high accuracy provided by silicon nanofabrication techniques, the feasibility of generating single photons across the wavelength range 1333–1425 nm (E-band) and 1437–1510 nm (S-band) for slightly different waveguide widths (625 nm & 650 nm) is also demonstrated. These filter-free integrated photon sources could be important for large-scale linear optical quantum computation (LOQC) and long-distance fiber-optic quantum key distribution (QKD) networks.

Journal of Lightwave Technology•Jul 5, 2022•12 citations
High-efficiency submegahertz bandwidth photon pair generators will enable the field of quantum technology to transition from laboratory demonstrations to transformational applications involving information transfer from photons to atoms. While spontaneous parametric processes are able to achieve high-efficiency photon pair generation, the spectral bandwidth tends to be relatively large, as defined by phase-matching constraints. To solve this fundamental limitation, we use an ultrahigh quality factor ( Q ) fused silica microsphere resonant cavity to form a photon pair generator. We present the full theory for the spontaneous four-wave mixing (SFWM) process in these devices, fully taking into account all relevant source characteristics in our experiments. The exceptionally narrow (down to kilohertz-scale) linewidths of these devices result in a reduction in the bandwidth of the photon pair generation, allowing submegahertz spectral bandwidth to be achieved. Specifically, using a pump source centered around 1550 nm, photon pairs with the signal and idler modes at wavelengths close to 1540 and 1560 nm, respectively, are demonstrated. We herald a single idler-mode photon by detecting the corresponding signal photon, filtered via transmission through a wavelength division multiplexing channel of choice. We demonstrate the extraction of the spectral profile of a single peak in the single-photon frequency comb from a measurement of the signal–idler time of emission distribution. These improvements in device design and experimental methods enabled the narrowest spectral width ( Δ ν = 366 kHz ) to date in a heralded single-photon source based on SFWM.
Summary form only given. Hybrid quantum technologies seek to combine the advantages of two individual quantum architectures by transferring the information between the two systems. We want to benefit from the high mobility and ease of transmission of photons for quantum communication and exploit the excellent readout and storage capabilities of atomic qubits as a quantum memory, which is essential to build up quantum repeater networks for quantum data processing. Efficient interaction of photons with atoms requires a match of the photons spectral properties to those of the resonances of the atomic species. The atomic transition usually has a much narrower bandwidth than single photons generated by spontaneous parametric down-conversion (SPDC), the current gold standard of producing high-purity heralded single photons at flexible wavelengths. To develop hybrid quantum technologies therefore requires significantly reducing the single photon emission spectra to fulfill these requirements. The way we try to achieve this is by using an optical cavity to enhance the probability of creating the photons in the spectral and spatial resonator mode.We report 100% duty cycle generation of sub-MHz single photon pairs at the Rubidium D1 line using cavityenhanced spontaneous parametric down-conversion [3]. The double exponential decay of the temporal intensity cross-correlation function exhibits a bandwidth of 666 ± 16 kHz for the single photons, an order of magnitude below the natural linewidth of the target transition. This is, to our knowledge, the narrowest bandwidth of single photons from SPDC to date. A new method of placing a half-wave plate inside the cavity helps to achieve triple resonance between pump, signal and idler photon, reducing the bandwidth and simplifying the locking scheme. Additionally, stabilisation of the cavity to the pump frequency enables the 100% duty cycle. The quantum nature of the source is confirmed by the idler-triggered second-order autocorrelation function at τ = 0 to be g(2) s,s (0) = 0.016 ± 0.002 for a heralding rate of 5 kHz and antibunching below 0.5 is observed up to heralding rates of 250 kHz [3]. The high purity of the source is matched by high indistinguishability of the photons demonstrated in a Hong-Ou-Mandel (HOM) interference experiment with a visibility V = 96.5 ± 0.5 %. Additionally, the modelocked two-photon state of the generated pairs leads to revivals of the HOM dip. We observe these revivals up to 100 m path difference between signal and idler photon, independently proofing the long coherence length of our photons.
Summary form only given. Single-photon sources are key components in applications of photonic quantum technologies such as quantum key distribution (QKD) [1]. One way of realizing single-photon sources is generation of photon pairs (PP) using spontaneous four-wave mixing (FWM): two photons from a pump p annihilate and create two side-band photons at frequencies determined partly by the energy conservation 2ωρ= ω1+ ω2, where ωp,ω1,ω2are the frequencies of the pump and the two side-bands, respectively, and partly by the phase-matching condition. PP generated spontaneously arrive at indeterministic times but even so, they are useful for QKD because one of the photons can be heralded by detecting the other. The heralded photons are then used for transmitting the quantum key.We propose a higher order mode scheme for generating PP in silica fibers; the side-band photons are generated at center wavelength λ1 = 810 nm in the linearly polarized LP02-mode and at λ2 = 1550 nm in the LP01mode, respectively, by pumping in the LP11-mode at λ7, = 1064 nm, where laser sources are readily available. The 810 nm photon is detectable with relatively cheap and efficient silicon-based single-photon detectors, and the heralded 1550 nm photon is mode-matched with transmission fibers in the low-loss spectral window. We design a silica fiber that phase matches these modes and wavelengths while it also reduces the impacts of core radius fluctuations (CRF) caused by fabrication imperfections; the fiber design is inspired by B. P.-P. Kuo et al. [3] and a sketch of the refractive index profile is shown in Fig. 1(a). The scalar wave equation is solved using appropriate Sellmeier data for Germanium-doped silica and the calculated effective indexes for the three modes versus wavelength are shown in Fig. 1(b) together with the core and cladding refractive indexes; the inset shows the wavelength configuration of the pump and two side-bands; phase matching is achieved when the effective indexes of the three modes lie on a straight line [2]. The nonlinear overlap of the waves in this configuration is approximately 18% of the corresponding overlap where all waves are in the LP01-mode.
Photonic quantum technologies require efficient sources of pure single photons. We present a heralded single-photon source based on spontaneous parametric down-conversion in a monolithic cavity optimized for high spectral and spatial purity. The source heralds single photons at a wavelength of 1540 nm and a spectral bandwidth of 168 MHz, with a maximum heralding efficiency of 70% including all transmission and detection losses, while keeping the multi-photon contamination below 3%. The cavity enhancement predominantly generates photons into the central cavity mode, with a theoretical upper bound on the spectral purity of 79.4% arising from nonzero overlap with adjacent cavity modes. Spectral isolation of the central cavity mode with an etalon yields an increased measured spectral purity of (96.2 ±\pm± 2.7)%.
We demonstrate theoretically the direct (filter-free) generation of spectrally uncorrelated photon pairs, and consequently high-purity heralded single photons at telecommunication wavelengths, in SOI (silicon-on-insulator) nanowaveguides via spontaneous four-wave mixing (SFWM). The inherent strong waveguide dispersion in such high-index contrast structures is employed for discrete-band phase-matching in order to suppress the pair spectral correlations, and to produce photons in the fundamental spatial mode for easy in-out coupling to single-mode optical fibers. Additionally, by optimizing the source parameters like waveguide length, dispersion and pump bandwidth, the group-velocity of generated photons is also engineered to further eliminate spectral correlations. Extensive numerical mode simulations for various waveguide widths are used to design intrinsically pure photon sources via joint spectral amplitude (JSA) engineering. Purity$>9595% is shown to be achievable in a silica-clad SOI waveguide with a cross-section 220 × 600 nm95^{2}fortypicalvaluesoflengthandpumpbandwidth.Thewavelengthoftheseheraldedsinglephotonscanbetunedintherangeof1266–1363nm(for typical values of length and pump bandwidth. The wavelength of these heralded single photons can be tuned in the range of 1266–1363 nm (fortypicalvaluesoflengthandpumpbandwidth.Thewavelengthoftheseheraldedsinglephotonscanbetunedintherangeof1266–1363nm(\sim$O-band) by varying the pump wavelength. Considering the high accuracy provided by silicon nanofabrication techniques, the feasibility of generating single photons across the wavelength range 1333–1425 nm (E-band) and 1437–1510 nm (S-band) for slightly different waveguide widths (625 nm & 650 nm) is also demonstrated. These filter-free integrated photon sources could be important for large-scale linear optical quantum computation (LOQC) and long-distance fiber-optic quantum key distribution (QKD) networks.