We study trajectories of collective spin states of an ensemble of spinors. The spinors considered here are either trapped ions in free space or atoms confined in a cavity, both systems of which are engineered through their interactions with light fields to obey an effective Dicke model. In an appropriate limit of the Dicke model, one obtains one-axis twisting dynamics of the collective spin and evolution after a finite time to a spin cat state or, in the long-time limit, the Dicke state ${|S,0\ensuremath{\rangle}}_{x}$, conditioned upon there being no photon emissions from the system (i.e., no quantum jumps). If there is a jump, however, the system evolves probabilistically into one of a finite number of entangled-state cycles, where the system then undergoes a persistent sequence of jumps between two Dicke-state superpositions in a rotated basis. The different cycles can be distinguished by the frequency at which jumps occur.
We study trajectories of collective spin states of an ensemble of spinors. The spinors considered here are either trapped ions in free space or atoms confined in a cavity, both systems of which are engineered through their interactions with light fields to obey an effective Dicke model. In an appropriate limit of the Dicke model, one obtains one-axis twisting dynamics of the collective spin and evolution after a finite time to a spin cat state or, in the long-time limit, the Dicke state ∣S,0\ensuremath⟩x, conditioned upon there being no photon emissions from the system (i.e., no quantum jumps). If there is a jump, however, the system evolves probabilistically into one of a finite number of entangled-state cycles, where the system then undergoes a persistent sequence of jumps between two Dicke-state superpositions in a rotated basis. The different cycles can be distinguished by the frequency at which jumps occur.
We study quantum trajectories of collective atomic spin states of N effective two-level atoms driven with laser and cavity fields. We show that interesting ``entangled-state cycles'' arise probabilistically when the (Raman) transition rates between the two atomic levels are set equal. For odd (even) N, there are (N+1)/2(N/2) possible cycles. During each cycle the N-qubit state switches, with each cavity photon emission, between the states $(|N/2,m⟩\ifmmode\pm\else\textpm\fi{}|N/2,\ensuremath{-}m⟩)/\sqrt{2}$, where ∣N/2,m⟩ is a Dicke state in a rotated collective basis. The quantum number m(>0), which distinguishes the particular cycle, is determined by the photon counting record and varies randomly from one trajectory to the next. For even N it is also possible, under the same conditions, to prepare probabilistically (but in steady state) the Dicke state ∣N/2,0⟩, i.e., an N-qubit state with N/2 excitations, which is of particular interest in the context of multipartite entanglement.
We propose a method for engineering spin dynamics in ensembles of integer-spin atoms confined within a high-finesse optical cavity. Our proposal uses cavity-assisted Raman transitions to engineer a Dicke model for integer-spin atoms, which, in a dispersive limit, reduces to effective atom-atom interactions within the ensemble. This scheme offers a promising and flexible new avenue for the exploration of a wide range of spinor many-body physics. As an example of this, we present results showing that this method can be used to generate spin-nematic squeezing in an ensemble of spin-1 atoms. With realistic parameters, the scheme should enable substantial squeezing on time scales much shorter than current experiments with spin-1 Bose-Einstein condensates.
In this thesis a theoretical framework for a spin-1 exchange dynamics is developed by the use of effective Hamiltonian theory. We develop this framework through several applications beginning with the standard Jaynes-Cummings model, which under the method of time-averaging leads to the Hamiltonian described by one-axis twisting in a more efficient manner than standard adiabatic elimination. The process of developing effective many-body spin Hamiltonian’s is then applied in several contexts. The robustness of the systems we studied are demonstrated through the generation of entangled states under various constraints.\nWe find that when fixed within a sub-manifold of the collective angular momentum states the time evolution of minimally uncertain atomic states results in atomic cat states, which have been utilized in a variety of contexts for precision measurements. More so, when the initial state is given freedom to evolve between all angular momentum sub-manifolds large degrees of entanglement results. We give analytic results for the case of two-atoms where the entanglement quantification is given through the fidelity, and Schmidt number. This gives implications for measurement protocols through Ramsey pulses, quantum simulators, and creation of spin-1 Bell states for teleportation.\nUnder different operating conditions, we demonstrate the emergence of electromagnetically induced transparency(EIT) which provides a platform for quantum memory, polarization conversion, and state transfer. A limitation of photonic processes is the short optical resonance lifetime, however, our system is free of this issue due to the dispersive approximation constraining the system to a decoherence free ground state manifold. As a result our EIT scheme can result in longer storage times, and more efficient state transfer as decoherence due to spontaneous emission is not the limiting factor.
Present-day experiments have started to couple traditional simulations of ultracold atom experiments with quantum light-fields in cavities. This has provided a wealth of op- portunities to enlarge the number of interaction potentials: cavity mediated long-range interactions compete with kinetic energies, longitudinal fields, short-ranged collisional or magnetic spin-spin interactions. The intracavity many-body lattice models often have to be maintained far from equilibrium through the presence of external driving lasers that help to boost and engineer the various interaction potentials. The steady influx of energy is compensated by a steady stream of energy out of the atom-cavity system for example by photon losses or atomic spontaneous emission. Several experiments have demonstrated that such environments can give rise to new competing quantum phases. \nBut this long-standing ambition to push for models with tailorable interaction potentials can bring with it also considerable challenges in their theoretical description, since sponta- neous symmetry breaking transitions in many body lattice systems coupled to dynamical light-fields with single-photon character occur in the presence of drive and dissipation for the photonic force carriers. This clearly calls for model systems where the above men- tioned interplay of interactions, drive, dissipation and cooperative many-body behaviour can be theoretically studied to provide simple, experimentally verifiable predictions. \nThe Dicke model is, through its simplicity (an exactly solved ferromagnet with infinite range atom-atom interactions mediated by a single cavity mode), an exceptionally well- suited candidate. As the generic model for atom-light interactions, it has been experimen- tally realized in a variety of modern quantum optical systems, highlighting its relevance for present-day research. The Dicke model is also highly versatile itself. It has been extended into the dissipative realm, was promoted to account for multiple optical light modes and was used to describe multiple, coupled single-mode cavity structures. It was adapted to treat spin-selective coupling to a cavity to describe superradiance phase tran- sitions in multi-level atomic systems. Moreover, it was realised in electronic circuits where the dipole coupling of real atoms to single mode fields is replaced by a capacitive cou- pling of artificial atoms to a resonator mode. This illustrates that the Dicke model and its extended variants are ’future-proof’ and continue to be of relevance for fundamental light-matter interactions and for driven-dissipative phase transitions. \nIn this thesis, we investigate magnetic phase transitions in driven-dissipative atomic en- sembles interacting with quantum light. We present three research projects on variants of cooperative radiation of an ensemble of laser driven two-level atoms in a single mode optical cavity, as described by the Dicke model. \nThroughout the chapters 2,3 and 4 that contain the main body of research of this thesis, we investigate phase transitions between non-equilibrium stationary states in engineered quantum-optical systems each of which extends the conventional Dicke model physics. As a starting point, we map the quantum equations of motion onto a set of semiclassical nonlinear stochastic equations and analyse their stationary states and instabilities with master equations for atomic spin and photon mean-field amplitudes. These are used to obtain experimentally relevant parameters such as critical atom-light couplings for phase transitions, phase diagrams and properties of stationary non-equilibrium states in addition to cavity output spectra that identify the imprint of magnetic correlations in the light-field. \nIn chapter 2, we help resolve a discrepancy between earlier experimental investigations of the critical atom-light coupling strength for the superradiance transition in the Dicke model: higher external pumping strengths than theoretically predicted were needed to observe a coherent, superradiant state of the light field in an optical cavity. By including incoherent spontaneous emission of atomic excitations, we extend the dissipative Dicke model to a two loss channel variant containing both photon leakage and atomic decay that reproduces the experimentally observed critical atom-light coupling. \nRecent experiments have started to interface quantum many body lattice models with coherent cavity fields, thereby allowing to realize new quantum phases through competing atom-cavity and atom-atom interactions. In chapter 3, we consider a simplified model for such a set-up where a single quantized mode of the light-field interacts with an ensemble of Rydberg-dressed atoms inside a high finesse optical cavity. This model provides a base case for further studies of quantum magnets in optical cavities. At the heart of this model is a competition of short- (dipolar atom-atom) and long-range (atom-light) interactions at the Hamiltonian level in the presence of both spontaneous emission and photon leak- age through the cavity mirrors. We show that different magnetic phases can coexist with coherent atomic radiation and provide clear experimental signatures to identify the mag- netic structure and intra-cavity dynamics. We suggest an experimental level-scheme for a quantum optical implementation of our model. \nIn chapter 4 we consider a generic, collective decay for many-body excitations in the paradigmatic Dicke model. This extension drastically enriches the dynamics as it induces a bicritical point and a bistable regime dominated by true non-equilibrium fluctuations that induce a dissipative first-order phase transition that can only be resolved by including finite fluctuation corrections with the help of stochastic Langevin equations. We investigate the hysteretic response to time-dependent ramps of the atom-light coupling. Discontinuous first-order phase transitions where metastable states coexist in a hysteresis domain have been investigated in recent dissipative quantum-optical experiments. We review noise- activation far from thermal equilibrium in chapter 5.
Superradiance is an extensive cooperative spontaneous emission phenomenon, exhibited by some atomic collective-spin states. However, distinct initial states differ in their decay dynamics. Dicke states ∣j,m⟩ with distinct numbers of excitations n=m+j, driven by vacuum fluctuations, have their peak emission intensity shifted in time. Rotating Dicke states relative to the decay axis introduces an interesting parity structure that affects the pulse profile and photon correlations. Squeezed-bath prepared states undergo a squeezing-controlled crossover to the rotated Dicke states, making the emission character dependent on the amount of squeezing transferred from light to the atomic state. For semiclassical states with a macroscopic dipole moment, like the atomic coherent state, the emission intensity depends on their polarization. We present detailed results on the superradiant dynamics of a representative selection of states expanded in Dicke states to highlight the initial state as an independent dynamical control parameter. For large-N, we are able to predict fairly accurately the pulse profile in each case using the mean-field approximation, an approach based on the Fokker--Planck equation. We also present comparative results on the intensity correlation function, quantify the coherent and incoherent contributions of the emission, and contrast between small and large ensembles.
The scalable production of multipartite entangled states in ensembles of qubits is a crucial function of quantum devices, as such states are an essential resource both for fundamental studies on entanglement, as well as for applied tasks. Here we focus on the U(1) symmetric Hamiltonians for qubits with dipolar interactions-a model realized in several state-of-the-art quantum simulation platforms for lattice spin models, including Rydberg-atom arrays with resonant interactions. Making use of exact and variational simulations, we theoretically show that the nonequilibrium dynamics generated by this Hamiltonian shares fundamental features with that of the one-axis-twisting model, namely, the simplest interacting collective-spin model with U(1) symmetry. The evolution governed by the dipolar Hamiltonian generates a cascade of multipartite entangled states-spin-squeezed states, Schrödinger's cat states, and multicomponent superpositions of coherent spin states. Investigating systems with up to N=144 qubits, we observe full scalability of the entanglement features of these states directly related to metrology, namely, scalable spin squeezing at an evolution time O(N^{1/3}) and Heisenberg scaling of sensitivity of the spin parity to global rotations for cat states reached at times O(N). Our results suggest that the native Hamiltonian dynamics of state-of-the-art quantum simulation platforms, such as Rydberg-atom arrays, can act as a robust source of multipartite entanglement.