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arXiv:2205.03910 · Physical Review Letters

Multipartite Entangled States in Dipolar Quantum Simulators

Tommaso Comparin, Fabio Mezzacapo, Tommaso Roscilde

Published Oct 7, 2022• 0 citations
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Abstract

The scalable production of multipartite entangled states in ensembles of qubits is a crucial function of quantum devices, as such states are an essential resource both for fundamental studies on entanglement, as well as for applied tasks. Here we focus on the U(1) symmetric Hamiltonians for qubits with dipolar interactions-a model realized in several state-of-the-art quantum simulation platforms for lattice spin models, including Rydberg-atom arrays with resonant interactions. Making use of exact and variational simulations, we theoretically show that the nonequilibrium dynamics generated by this Hamiltonian shares fundamental features with that of the one-axis-twisting model, namely, the simplest interacting collective-spin model with U(1) symmetry. The evolution governed by the dipolar Hamiltonian generates a cascade of multipartite entangled states-spin-squeezed states, Schrödinger's cat states, and multicomponent superpositions of coherent spin states. Investigating systems with up to N=144 qubits, we observe full scalability of the entanglement features of these states directly related to metrology, namely, scalable spin squeezing at an evolution time O(N^{1/3}) and Heisenberg scaling of sensitivity of the spin parity to global rotations for cat states reached at times O(N). Our results suggest that the native Hamiltonian dynamics of state-of-the-art quantum simulation platforms, such as Rydberg-atom arrays, can act as a robust source of multipartite entanglement.

DOI
10.1103/physrevlett.129.150503

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The scalable production of multipartite entangled states in ensembles of qubits is a crucial function of quantum devices, as such states are an essential resource both for fundamental studies on entanglement, as well as for applied tasks. Here we focus on the U(1) symmetric Hamiltonians for qubits with dipolar interactions-a model realized in several state-of-the-art quantum simulation platforms for lattice spin models, including Rydberg-atom arrays with resonant interactions. Making use of exact and variational simulations, we theoretically show that the nonequilibrium dynamics generated by this Hamiltonian shares fundamental features with that of the one-axis-twisting model, namely, the simplest interacting collective-spin model with U(1) symmetry. The evolution governed by the dipolar Hamiltonian generates a cascade of multipartite entangled states-spin-squeezed states, Schrödinger's cat states, and multicomponent superpositions of coherent spin states. Investigating systems with up to N=144 qubits, we observe full scalability of the entanglement features of these states directly related to metrology, namely, scalable spin squeezing at an evolution time O(N^{1/3}) and Heisenberg scaling of sensitivity of the spin parity to global rotations for cat states reached at times O(N). Our results suggest that the native Hamiltonian dynamics of state-of-the-art quantum simulation platforms, such as Rydberg-atom arrays, can act as a robust source of multipartite entanglement.
We study the generation of metrologically useful entanglement in a three-level (spin-1) system naturally realized in arrays of dipole-interacting Rydberg atoms confined in optical tweezers. In the spin-quadrupolar operator basis, the interaction Hamiltonian decomposes into effective SU(2) subspaces, within which quench dynamics from product initial states generate scalable spin-nematic squeezing. For symmetric interactions, we identify a mapping to effective one-axis twisting within bright and dark manifolds and demonstrate that the squeezing parameter scales as ξ2∝N−2/3ξ^{2}\propto N^{-2/3}ξ2∝N−2/3 (ξ2∝N−0.5ξ^{2}\propto N^{-0.5}ξ2∝N−0.5) with system size for all-to-all (two-dimensional dipolar) couplings. In both cases the quantum Fisher information reaches FQ∝N2F_Q\propto N^{2}FQ​∝N2. For antisymmetric interactions supplemented by a microwave drive we find a distinct two-axis countertwisting mechanism. This results in squeezing ξ2∝N−0.7ξ^{2}\propto N^{-0.7}ξ2∝N−0.7 for all-to-all interactions and moderate squeezing for dipolar interactions in 2D. Our results constitute a first theoretical step beyond the well-studied qubit setting toward scalable entanglement generation in qudit systems with dipolar interactions, directly relevant to current Rydberg tweezer experiments.
The production of large-scale entangled states is one of the main goals of next-generation quantum technologies, with an immediate potential for applications in the context of entanglement-assisted quantum sensing. A very promising platform to achieve this goal is offered by ultracold spinor gases, made of atoms with a large internal spin sensitive to magnetic fields. Here we show that the native spin-changing collisions in a spinor Bose-Einstein condensate, combined with an arbitrary quadratic Zeeman shift, can generate scalable spin squeezing in the collective spin of the ensemble, following the universal paradigm of the celebrated one-axis-twisting model. Squeezing dynamics is driven by the quadratic Zeeman shift when this shift is small; and by the spin-changing collisions for large shifts, in the form of stroboscopic squeezing. Turning off the Zeeman shift freezes out the collective-spin dynamics, so that the ensuing collective spin dynamics can be uniquely governed by an external field to be sensed. Our theoretical results pave the way for the use of spinor Bose gases with a large spin in fundamental studies of entanglement, as well as in advanced metrological applications.
Scalable spin squeezing in two-dimensional arrays of dipolar large-SSS spins
Controlling the quantum many-body state of arrays of qudits, possessing a large local Hilbert space, opens the path to a broad range of possibilities for many-particle entanglement, interesting both for fundamental quantum science, as well as for potential metrological applications. In this work we theoretically show that the spin-spin interactions realized in two-dimensional Mott insulators of large-spin magnetic atoms (such as Cr, Er or Dy) lead to scalable spin squeezing along the non-equilibrium unitary evolution initialized in a coherent spin state. An experimentally relevant perturbation to the collective squeezing dynamics is offered by a quadratic Zeeman shift, which leads instead to squeezing of individual spins. Making use of a truncated cumulant expansion for the quantum fluctuations of the spin array, we show that, for sufficiently small quadratic shifts, the spin squeezing dynamics is akin to that produced by the paradigmatic one-axis-twisting (OAT) model -- as expected from an effective separation between collective spin and spin-wave variables. Spin squeezing with OAT-like scaling is shown to be protected by the robustness of long-range ferromagnetic order to quadratic shifts in the equilibrium phase diagram of the system, that we reconstruct via quantum Monte Carlo and mean-field theory.
Spin squeezed entanglement enables metrological precision beyond the classical limit. Understood through the lens of continuous symmetry breaking, dipolar spin systems exhibit the remarkable ability to generate spin squeezing via their intrinsic quench dynamics. To date, this understanding has primarily focused on lattice spin systems; in practice however, dipolar spin systems$\unicode{x2014}$ranging from ultracold molecules to nuclear spin ensembles and solid-state color centers$\unicode{x2014}$often exhibit significant amounts of positional disorder. Here, we develop a theory for scalable spin squeezing in a two-dimensional randomly diluted lattice of quantum dipoles, which naturally realize a dipolar XXZ model. Via extensive quantum Monte Carlo simulations, we map out the phase diagram for finite-temperature XY order, and by extension scalable spin squeezing, as a function of both disorder and Ising anisotropy. As the disorder increases, we find that scalable spin squeezing survives only near the Heisenberg point. We show that this behavior is due to the presence of rare tightly-coupled dimers, which effectively heat the system post-quench. In the case of strongly-interacting nitrogen-vacancy centers in diamond, we demonstrate that an experimentally feasible strategy to decouple the problematic dimers from the dynamics is sufficient to enable scalable spin squeezing.
Quantum simulation platforms such as cold atoms, superconducting circuits, and trapped ions enable the experimental investigation of quantum many-body systems, with important implications for quantum technologies. In this thesis, we investigate how entanglement and correlations develop in such systems and how they can be harnessed both for the theoretical study of models relevant to condensed matter physics and for practical applications in quantum metrology. We begin by focusing on the adiabatic preparation of quantum many-body ground states. In particular, we show that quantum simulators can probe the link between spectral degeneracy and Spontaneous Symmetry Breaking, as pioneered by P.W. Anderson. We prove that odd-sized spin-½ systems exhibiting time-reversal symmetry sustain a net magnetization even away from the thermodynamic limit, thanks to an exact spectral degeneracy. Moreover, the symmetry-broken state exhibits scalable spin squeezing, a key resource for quantum metrology. We then turn to a different paradigm of evolution: quench dynamics. In particular, we show that monitoring the real-time evolution of correlations allows for the experimental measurement of the dispersion relation of fundamental excitations. In the case of two-dimensional long-range ordered systems, such as the dipolar XY model, these excitations are spin waves, leading to sharp features in the evolution of two-point correlation functions. Conversely, in one-dimensional systems, fundamental excitations have a fermionic nature, and their detection requires the measurement of non-local correlation functions. The latter, while inaccessible in condensed matter, are instead well suited to quantum simulators with individually addressable degrees of freedom.
The spin-squeezing protocols allow the dynamical generation of massively correlated quantum many-body states, which can be utilized in entanglement-enhanced metrology and technologies. We study a quantum simulator generating twisting dynamics realized in a two-component Bose-Hubbard model with dipolar interactions. We show that the interplay of contact and long-range dipolar interactions between atoms in the superfluid phase activates the anisotropic two-axis countertwisting mechanism, accelerating the spin-squeezing dynamics and allowing the Heisenberg-limited accuracy in spectroscopic measurements.