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arXiv:2607.06842

Universal spin-squeezing dynamics in spinor condensates

Nikolaos Giovanoudis, Navid Kazemiseresht, Fabio Mezzacapo, Emilia Witkowska, Tommaso Roscilde

quant-phcond-mat.quant-gasSubmitted Jul 7, 2026• Announced Jul 9, 2026• 0 citations
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Abstract

The production of large-scale entangled states is one of the main goals of next-generation quantum technologies, with an immediate potential for applications in the context of entanglement-assisted quantum sensing. A very promising platform to achieve this goal is offered by ultracold spinor gases, made of atoms with a large internal spin sensitive to magnetic fields. Here we show that the native spin-changing collisions in a spinor Bose-Einstein condensate, combined with an arbitrary quadratic Zeeman shift, can generate scalable spin squeezing in the collective spin of the ensemble, following the universal paradigm of the celebrated one-axis-twisting model. Squeezing dynamics is driven by the quadratic Zeeman shift when this shift is small; and by the spin-changing collisions for large shifts, in the form of stroboscopic squeezing. Turning off the Zeeman shift freezes out the collective-spin dynamics, so that the ensuing collective spin dynamics can be uniquely governed by an external field to be sensed. Our theoretical results pave the way for the use of spinor Bose gases with a large spin in fundamental studies of entanglement, as well as in advanced metrological applications.

Comments
4.5+2 pages, 3+2 figures

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The production of large-scale entangled states is one of the main goals of next-generation quantum technologies, with an immediate potential for applications in the context of entanglement-assisted quantum sensing. A very promising platform to achieve this goal is offered by ultracold spinor gases, made of atoms with a large internal spin sensitive to magnetic fields. Here we show that the native spin-changing collisions in a spinor Bose-Einstein condensate, combined with an arbitrary quadratic Zeeman shift, can generate scalable spin squeezing in the collective spin of the ensemble, following the universal paradigm of the celebrated one-axis-twisting model. Squeezing dynamics is driven by the quadratic Zeeman shift when this shift is small; and by the spin-changing collisions for large shifts, in the form of stroboscopic squeezing. Turning off the Zeeman shift freezes out the collective-spin dynamics, so that the ensuing collective spin dynamics can be uniquely governed by an external field to be sensed. Our theoretical results pave the way for the use of spinor Bose gases with a large spin in fundamental studies of entanglement, as well as in advanced metrological applications.
Scalable spin squeezing in two-dimensional arrays of dipolar large-SSS spins
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We theoretically show that the spin-spin interactions realized in two-dimensional Mott insulators of large-spin magnetic atoms (such as Cr, Er, or Dy) lead to scalable spin squeezing along the nonequilibrium unitary evolution initialized in a coherent spin state. An experimentally relevant perturbation to the collective squeezing dynamics is offered by a quadratic Zeeman shift, which leads instead to squeezing of individual spins. Making use of a truncated cumulant expansion for the quantum fluctuations of the spin array, we show that, for sufficiently small quadratic shifts, the spin squeezing dynamics is akin to that produced by the paradigmatic one-axis-twisting model-as expected from an effective separation between collective-spin and spin-wave variables. Scalable spin squeezing is shown to be protected by the robustness of long-range ferromagnetic order to quadratic shifts in the equilibrium phase diagram of the system that we reconstruct via quantum Monte Carlo and mean-field theory.
We study spin-nematic squeezing in a spinor Bose-Einstein condensate and use it to probe dynamical quantum phase transitions. We show that the quench dynamics of the spin-nematic squeezing exhibits a nonanalytical change with respect to a final quadratic Zeeman energy, and demonstrate that the squeezing detects not only the ground state phase diagram, but also the excited state quantum phase transition. We further analyze the dynamic stabilization of the system and present its relation to the dynamical quantum phase transitions. Our results are applicable to the spinor condensates with both of the sodium and rubidium atoms.
The quantum many-body problem, and especially the study of dynamical properties of a multipartite quantum system, is one of the hardest problems of modern physics. There exist only a few analytical results and exact numerical simulations require an amount of resources that grow exponentially with the system size.In this thesis, we studied correlations and entanglement properties for systems composed of magnetic atoms on a lattice, for instance via the generation of spin squeezing. For this purpose we have developed new approximate numerical methods that allow us to study large system sizes. This enabled us to propose protocols to generate an amount of spin squeezing that scales with the system size. The advantage is twofold. Since spin squeezing is an entanglement witness, this would allow for entanglement detection in a system of magnetic atoms - which has yet to be realized experimentally. Moreover, spin squeezing offers an important metrological advantage, asspin-squeezed states can be used for extremely precise measurements of external magnetic fields, far beyond what one can achieve within dependent atoms.Finally, we studied the generation of other forms of entanglement, namely Dicke squeezing (of spin or momentum), in systems of Bose condensed atoms. This form of entanglement is well-known in spin-1 atomic condensates. Here, we propose a protocol to generalize it to the case of momentum modes, using a time-dependent Hamiltonian. The entangled states generated during the dynamics are potentially useful for the precision measurements of inertial forces.
Spin squeezing generated via inter-atom entanglement in multilevel atomic ensembles provides a powerful resource for quantum-enhanced metrology. Existing schemes that harness internal atomic degrees of freedom to boost squeezing typically encode the collective squeezing in complex superpositions of magnetic sublevels, which complicates state control and limits practical applications. Here, we propose a coherent control scheme that simultaneously enhances collective spin squeezing and maps the resulting atom-atom entanglement onto two well-defined magnetic sublevels suitable for subsequent metrology experiments. Our protocol sandwiches a quantum non-demolition measurement between two internal one-axis-twisting interactions arranged in an echo sequence. We show that this approach can optimally leverage internal states to boost the inter-atom entanglement and, at the same time, encode it in two magnetic sublevels, which is readily convertible into metrologically useful spin squeezing. Our results offer a straightforward and efficient strategy for generating highly entangled yet readily accessible quantum states in multilevel atomic systems.
Spin squeezing inequalities (SSI) represent a major tool to probe quantum entanglement among a collection of few-level atoms, and are based on collective spin measurements and their fluctuations. Yet, for atomic ensembles of spin- j atoms and ultracold spinor gases, many experiments can image the populations in all Zeeman sublevels s=−j,−j+1,…,j , potentially revealing finer features of quantum entanglement not captured by SSI. Here we present a systematic approach which exploits Zeeman-sublevel population measurements in order to construct novel entanglement criteria, and illustrate our approach on ground states of spin-1 and spin-2 Bose-Einstein condensates. Beyond these specific examples, our approach allows one to infer, in a systematic manner, the optimal permutationally-invariant entanglement witness for any given set of collective measurements in an ensemble of d -level quantum systems.