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arXiv:2108.01942 · Physical review. B./Physical review. B

Theory of quantum entanglement and structure of the two-mode squeezed antiferromagnetic magnon vacuum

Dennis Wuhrer, Niklas Rohling, Wolfgang Belzig

Published Feb 8, 2022• 21 citations
arXivHTMLPDF

Abstract

Recently, investigations of the quantum properties of an antiferromagnet in the spin wave approximation have identified the eigenstates as two-mode squeezed sublattice-magnon states. The uniform magnon states were shown to display a massive sublattice entanglement. Here we extend this idea and study the squeezing properties of all sublattice Fock states throughout the magnetic Brillouin zone. We derive the full statistics of the sublattice magnon number with wave number $\stackrel{P\vec}{k}$ in the ground state and show that sublattice magnons occur in pairs with opposite wave vectors, hence, resulting in entanglement of both modes. To quantify the degree of entanglement we apply the Duan-Giedke-Cirac-Zoller inequality and show that it can be violated for all modes. The degree of entanglement decreases towards the corners of the Brillouin zone. We relate the entanglement to measurable correlations of components of the N\'eel and the magnetization vectors, thus allowing one to experimentally test the quantum nature of the squeezed vacuum. The distinct $k$-space structure of the entanglement shows that the squeezed vacuum has a nonuniform shape that is revealed through the $\stackrel{P\vec}{k}$-dependent correlators for the magnetization and the N\'eel vectors.

DOI
10.1103/physrevb.105.054406

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Recently, investigations of the quantum properties of an antiferromagnet in the spin wave approximation have identified the eigenstates as two-mode squeezed sublattice-magnon states. The uniform magnon states were shown to display a massive sublattice entanglement. Here we extend this idea and study the squeezing properties of all sublattice Fock states throughout the magnetic Brillouin zone. We derive the full statistics of the sublattice magnon number with wave number \stackrel{P\vec}{k} in the ground state and show that sublattice magnons occur in pairs with opposite wave vectors, hence, resulting in entanglement of both modes. To quantify the degree of entanglement we apply the Duan-Giedke-Cirac-Zoller inequality and show that it can be violated for all modes. The degree of entanglement decreases towards the corners of the Brillouin zone. We relate the entanglement to measurable correlations of components of the N'eel and the magnetization vectors, thus allowing one to experimentally test the quantum nature of the squeezed vacuum. The distinct kkk-space structure of the entanglement shows that the squeezed vacuum has a nonuniform shape that is revealed through the \stackrel{P\vec}{k}-dependent correlators for the magnetization and the N'eel vectors.
Employing the concept of two-mode squeezed states from quantum optics, we demonstrate a revealing physical picture for the antiferromagnetic ground state and excitations. Superimposed on a N\'eel ordered configuration, a spin-flip restricted to one of the sublattices is called a sublattice magnon. We show that an antiferromagnetic spin-up magnon is composed of a quantum superposition of states with n+1n+1n+1 spin-up and nnn spin-down sublattice magnons and is thus an enormous excitation despite its unit net spin. Consequently, its large sublattice spin can amplify its coupling to other excitations. Employing von Neumann entropy as a measure, we show that the antiferromagnetic eigenmodes manifest a high degree of entanglement between the two sublattices, thereby establishing antiferromagnets as reservoirs for strong quantum correlations. Based on these insights, we outline strategies for exploiting the strong quantum character of antiferromagnetic (squeezed) magnons and give an intuitive explanation for recent experimental and theoretical findings in antiferromagnetic magnon spintronics.
N\'eel ordered antiferromagnets exhibit two-mode squeezing such that their ground state is a nonclassical superposition of magnon Fock states. Here we theoretically demonstrate that antiferromagnets can couple to spin qubits via direct dispersive interaction stemming from, e.g., interfacial exchange. We demonstrate that this kind of coupling induces a magnon number-dependent level splitting of the excited state resulting in multiple system excitation energies. This series of level splittings manifests itself as nontrivial excitation peaks in qubit spectroscopy thereby revealing the underlying nonclassical magnon composition of the antiferromagnetic quantum state. By appropriately choosing the drive or excitation energy, the magnonic state can be controlled via the qubit, suggesting that Fock states of magnon pairs can be generated deterministically. This enables achieving states useful for quantum computing and quantum information science protocols.
Quantum magnonics is an emerging research field, with great potential for applications in magnon based hybrid systems and quantum information processing. Quantum correlation, such as entanglement, is a central resource in many quantum information protocols that naturally comes about in any study toward quantum technologies. This applies also to quantum magnonics. Here, we investigate antiferromagnetic coupling of two ferromagnetic sublattices that can have two different magnon modes. We show how this may lead to experimentally measurable bipartite continuous-variable magnon-magnon entanglement. The entanglement can be fully characterized via a single squeezing parameter or, equivalently, entanglement parameter. The clear relation between the entanglement parameter and the Einstein, Podolsky, and Rosen (EPR) function of the ground state opens up for experimental quantification magnon-magnon continuous-variable entanglement and EPR nonlocality. We propose a practical experimental realization to measure the EPR function of the ground state, in a setting that relies on magnon-photon interaction in a microwave cavity.
Abstract These two accompanying papers are concerned with entanglement for systems of identical massive bosons and the relationship to spin squeezing and other quantum correlation effects. The main focus is on two mode entanglement, but multi-mode entanglement is also considered. The bosons may be atoms or molecules as in cold quantum gases. The previous paper I dealt with the general features of quantum entanglement and its specific definition in the case of systems of identical bosons. Entanglement is a property shared between two (or more) quantum sub-systems. In defining entanglement for systems of identical massive particles, it was concluded that the single particle states or modes are the most appropriate choice for sub-systems that are distinguishable, that the general quantum states must comply both with the symmetrization principle and the super-selection rules (SSR) that forbid quantum superpositions of states with differing total particle number (global SSR compliance). Further, it was concluded that (in the separable states) quantum superpositions of sub-system states with differing sub-system particle number (local SSR compliance) also do not occur. The present paper II determines possible tests for entanglement based on the treatment of entanglement set out in paper I. Several inequalities involving variances and mean values of operators have been previously proposed as tests for entanglement between two sub-systems. These inequalities generally involve mode annihilation and creation operators and include the inequalities that define spin squeezing. In this paper, spin squeezing criteria for two mode systems are examined, and spin squeezing is also considered for principle spin operator components where the covariance matrix is diagonal. The proof, which is based on our SSR compliant approach shows that the presence of spin squeezing in any one of the spin components requires entanglement of the relevant pair of modes. A simple Bloch vector test for entanglement is also derived. Thus we show that spin squeezing becomes a rigorous test for entanglement in a system of massive bosons, when viewed as a test for entanglement between two modes. In addition, other previously proposed tests for entanglement involving spin operators are considered, including those based on the sum of the variances for two spin components. All of the tests are still valid when the present concept of entanglement based on the symmetrization and SSR criteria is applied. These tests also apply in cases of multi-mode entanglement, though with restrictions in the case of sub-systems each consisting of pairs of modes. Tests involving quantum correlation functions are also considered and for global SSR compliant states these are shown to be equivalent to tests involving spin operators. A new weak correlation test is derived for entanglement based on local SSR compliance for separable states, complementing the stronger correlation test obtained previously when this is ignored. The Bloch vector test is equivalent to one case of this weak correlation test. Quadrature squeezing for single modes is also examined but not found to yield a useful entanglement test, whereas two mode quadrature squeezing proves to be a valid entanglement test, though not as useful as the Bloch vector test. The various entanglement tests are considered for well-known entangled states, such as binomial states, relative phase eigenstates and NOON states—sometimes the new tests are satisfied while than those obtained in other papers are not. The present paper II then outlines the theory for a simple two mode interferometer showing that such an interferometer can be used to measure the mean values and covariance matrix for the spin operators involved in entanglement tests for the two mode bosonic system. The treatment is also generalized to cover multi-mode interferometry. The interferometer involves a pulsed classical field characterized by a phase variable and an area variable defined by the time integral of the field amplitude, and leads to a coupling between the two modes. For simplicity the center frequency was chosen to be resonant with the inter-mode transition frequency. Measuring the mean and variance of the population difference between the two modes for the output state of the interferometer for various choices of interferometer variables is shown to enable the mean values and covariance matrix for the spin operators for the input quantum state of the two mode system to be determined. The paper concludes with a discussion of several key experimental papers on spin squeezing.
Ultrastrong light-matter coupling opens exciting possibilities to generate squeezed quantum states and entanglement. We propose achieving this regime in superconducting hybrid nanostructures with ferromagnetic interlayers. Strong confinement of the electromagnetic field between superconducting plates results in the existence of magnon-polariton (MP) modes with ultrastrong magnon-photon coupling, ultrahigh cooperativity, and colossal group velocities. These modes provide a numerically accurate explanation of recent experiments and have intriguing quantum properties. The MP quantum vacuum consists of the squeezed magnon and photon states with the degree of squeezing controlled in wide limits by the external magnetic field. The ground-state population of virtual photons and magnons is vast and can be used for generating correlated magnon and photon pairs. MP excitations contain bipartite entanglement between magnons and photons. Our results indicate that superconducting/ferromagnet nanostructures are very promising for quantum magnonics.
We investigate the second-order photon correlation function in cavity-magnon systems, focusing on ferromagnetic and antiferromagnetic cavities within the ultrastrong coupling regime, and extending beyond the rotating-wave approximation. By deriving exact integral solutions for the second-order correlation function, we demonstrate that counter-rotating magnon-photon interactions induce quadrature squeezing in the cavity mode. Furthermore, we show that tuning the anisotropic magnon-cavity couplings enhances the squeezing effect by changing the level repulsion of the magnon-cavity photon hybrid mode without increasing the cavity photon occupation number. Our study reveals distinct quantum correlation behaviors in ferromagnetic and antiferromagnetic cavities: For ferromagnetic cavities, we show that squeezing increases with coupling strength asymmetry, whereas in the antiferromagnetic case, magnon modes with opposite chirality suppress quantum effects and impose a lower bound on correlation functions. These findings provide a pathway to optimize photon blockade for quantum information technology in magnon-cavity systems in the ultrastrong coupling limit.