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arXiv:2402.13203 · Physical review. B./Physical review. B

Quantum sensing of antiferromagnetic magnon two-mode squeezed vacuum

Anna-Luisa E. Römling, Akashdeep Kamra

Published May 6, 2024• 11 citations
arXivHTMLPDF

Abstract

N\'eel ordered antiferromagnets exhibit two-mode squeezing such that their ground state is a nonclassical superposition of magnon Fock states. Here we theoretically demonstrate that antiferromagnets can couple to spin qubits via direct dispersive interaction stemming from, e.g., interfacial exchange. We demonstrate that this kind of coupling induces a magnon number-dependent level splitting of the excited state resulting in multiple system excitation energies. This series of level splittings manifests itself as nontrivial excitation peaks in qubit spectroscopy thereby revealing the underlying nonclassical magnon composition of the antiferromagnetic quantum state. By appropriately choosing the drive or excitation energy, the magnonic state can be controlled via the qubit, suggesting that Fock states of magnon pairs can be generated deterministically. This enables achieving states useful for quantum computing and quantum information science protocols.

DOI
10.1103/physrevb.109.174410

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N'eel ordered antiferromagnets exhibit two-mode squeezing such that their ground state is a nonclassical superposition of magnon Fock states. Here we theoretically demonstrate that antiferromagnets can couple to spin qubits via direct dispersive interaction stemming from, e.g., interfacial exchange. We demonstrate that this kind of coupling induces a magnon number-dependent level splitting of the excited state resulting in multiple system excitation energies. This series of level splittings manifests itself as nontrivial excitation peaks in qubit spectroscopy thereby revealing the underlying nonclassical magnon composition of the antiferromagnetic quantum state. By appropriately choosing the drive or excitation energy, the magnonic state can be controlled via the qubit, suggesting that Fock states of magnon pairs can be generated deterministically. This enables achieving states useful for quantum computing and quantum information science protocols.
Recently gained insights into equilibrium squeezing and entanglement harbored by magnets point toward exciting opportunities for quantum science and technology, while concrete protocols for exploiting these are needed. Here, we theoretically demonstrate that a direct dispersive coupling between a qubit and a noneigenmode magnon enables detecting the magnonic number states' quantum superposition that forms the ground state of the actual eigenmode-squeezed magnon-via qubit excitation spectroscopy. Furthermore, this unique coupling is found to enable control over the equilibrium magnon squeezing and a deterministic generation of squeezed even Fock states via the qubit state and its excitation. Our work demonstrates direct dispersive coupling to noneigenmodes, realizable in spin systems, as a general pathway to exploiting the equilibrium squeezing and related quantum properties thereby motivating a search for similar realizations in other platforms.
Ordered magnets harbor intrinsically squeezed ground states and magnonic excitations characterized by entanglement between spins and nonclassical magnon number composition. A pathway to detecting the superpositions of noneigenmode magnon number states underlying these nonclassical magnetic ground states has recently been demonstrated by utilizing a qubit coupled to the magnon mode via a direct dispersive interaction. Here, we theoretically develop this qubit spectroscopy further delineating the capabilities and limitations of this qubit spectroscopy for sensing the quantum superpositions that underlie the excited states. We demonstrate that the spectroscopy lends itself naturally to unraveling the superpositions that underlie the various quantized squeezed-magnon number states. However, excited states comprising superpositions of multiple squeezed Fock states become increasingly hard due to the large number of possible transitions, and resulting peaks, in the qubit spectroscopy thereby requiring qubits with narrower linewidths. Along the same lines, we theoretically demonstrate the qubit spectroscopy of a low amplitude coherent squeezed-magnon state analyzing the tradeoff between frequency crowding due to multiple transitions and peak linewidths. Our work lays the groundwork and design equations for deploying high-quality qubits towards sensing the composite nature of spin excitations in magnetic systems.
Employing the concept of two-mode squeezed states from quantum optics, we demonstrate a revealing physical picture for the antiferromagnetic ground state and excitations. Superimposed on a N\'eel ordered configuration, a spin-flip restricted to one of the sublattices is called a sublattice magnon. We show that an antiferromagnetic spin-up magnon is composed of a quantum superposition of states with n+1n+1n+1 spin-up and nnn spin-down sublattice magnons and is thus an enormous excitation despite its unit net spin. Consequently, its large sublattice spin can amplify its coupling to other excitations. Employing von Neumann entropy as a measure, we show that the antiferromagnetic eigenmodes manifest a high degree of entanglement between the two sublattices, thereby establishing antiferromagnets as reservoirs for strong quantum correlations. Based on these insights, we outline strategies for exploiting the strong quantum character of antiferromagnetic (squeezed) magnons and give an intuitive explanation for recent experimental and theoretical findings in antiferromagnetic magnon spintronics.
We propose an efficient method for dissipative generation of magnonic cat states in a cavity-magnon-qubit hybrid system by exploiting a two-magnon driving and dissipation mechanism. When both the magnon and qubit are driven, a coherent nonlinear two-magnon interaction is induced, wherein the qubit and the magnon mode exchange energy through magnon pairs. The dissipation of the qubit is exploited to steer the magnon mode into a quantum superposition of distinct coherent states, where the magnon mode evolves into either an even or odd cat state, depending on the parity of the magnon initial state. For the case where the magnon initial state is a superposition state, e.g., of $|0\ensuremath{\rangle}$ and $|1\ensuremath{\rangle}$, the magnon mode can evolve into a weighted mixture of the even and odd cat states. We also find that magnon squeezed states may emerge during the short-time evolution, showcasing the capability of our mechanism in preparing diverse magnon nonclassical states. Magnonic cat and squeezed states are macroscopic quantum states and have applications in macroscopic quantum studies and quantum sensing, e.g., in the dark-matter search using ferromagnetic axion haloscopes.
Hybrid systems based on magnons in ferromagnetic materials, such as yttrium iron garnet, have achieved remarkable development in the last decade. These include the coupling of magnons to microwave and optical photons, superconducting qubits, phonons, spins, the center-of-mass motion of a ferromagnet, etc. Here, we review both the experimental and theoretical progress in this field, focusing on the generation of magnonic quantum states and their applications in a broad range of fields. Since the strong coupling is a prerequisite for achieving coherent quantum control of magnons and preparing magnonic quantum states, we start by introducing representative strong-coupling experiments in cavity magnonics, then review a series of protocols for creating various magnonic quantum states, such as Fock, cat, squeezed, and entangled states, and discuss their potential applications in macroscopic quantum studies, quantum information science, quantum sensing, magnonic quantum devices, dark matter detection, and so on. Finally, we summarize the review and give an outlook for the future study of quantum magnonics.
Recently, investigations of the quantum properties of an antiferromagnet in the spin wave approximation have identified the eigenstates as two-mode squeezed sublattice-magnon states. The uniform magnon states were shown to display a massive sublattice entanglement. Here we extend this idea and study the squeezing properties of all sublattice Fock states throughout the magnetic Brillouin zone. We derive the full statistics of the sublattice magnon number with wave number $\stackrel{P\vec}{k}$ in the ground state and show that sublattice magnons occur in pairs with opposite wave vectors, hence, resulting in entanglement of both modes. To quantify the degree of entanglement we apply the Duan-Giedke-Cirac-Zoller inequality and show that it can be violated for all modes. The degree of entanglement decreases towards the corners of the Brillouin zone. We relate the entanglement to measurable correlations of components of the N\'eel and the magnetization vectors, thus allowing one to experimentally test the quantum nature of the squeezed vacuum. The distinct kkk-space structure of the entanglement shows that the squeezed vacuum has a nonuniform shape that is revealed through the $\stackrel{P\vec}{k}$-dependent correlators for the magnetization and the N\'eel vectors.