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arXiv:2105.12673 · Physical Review Letters

Active Frequency Measurement on Superradiant Strontium Clock Transitions

Yuan Zhang, Chongxin Shan, Klaus Mølmer

Published Jan 7, 2022• 15 citations
arXivHTMLPDF

Abstract

We develop a stochastic mean-field theory to describe active frequency measurements of pulsed superradiant emission, studied in a recent experiment with strontium-87 atoms trapped in an optical lattice inside an optical cavity [M. Norcia et al., Phys. Rev. X 8, 021036 (2018)PRXHAE2160-330810.1103/PhysRevX.8.021036]. Our theory reveals the intriguing dynamics of atomic ensembles with multiple transition frequencies, and it reproduces the superradiant beats signal, noisy power spectra, and frequency uncertainty in remarkable agreement with the experiments. Moreover, using longer superradiant pulses of similar strength and shortening the experimental duty cycle, we predict a short-term frequency uncertainty 7×10^{-17}/sqrt[τ/s], which makes active frequency measurements with superradiant transitions comparable with the record performance of current frequency standards [M. Schioppo et al., Nat. Photonics 11, 48 (2017)NPAHBY1749-488510.1038/nphoton.2016.231]. Our theory combines cavity quantum electrodynamics and quantum measurement theory, and it can be readily applied to explore conditional quantum dynamics and describe frequency measurements for other processes such as steady-state superradiance and superradiant Raman lasing.

DOI
10.1103/physrevlett.128.013604

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We develop a stochastic mean-field theory to describe active frequency measurements of pulsed superradiant emission, studied in a recent experiment with strontium-87 atoms trapped in an optical lattice inside an optical cavity [M. Norcia et al., Phys. Rev. X 8, 021036 (2018)PRXHAE2160-330810.1103/PhysRevX.8.021036]. Our theory reveals the intriguing dynamics of atomic ensembles with multiple transition frequencies, and it reproduces the superradiant beats signal, noisy power spectra, and frequency uncertainty in remarkable agreement with the experiments. Moreover, using longer superradiant pulses of similar strength and shortening the experimental duty cycle, we predict a short-term frequency uncertainty 7×10^{-17}/sqrt[τ/s], which makes active frequency measurements with superradiant transitions comparable with the record performance of current frequency standards [M. Schioppo et al., Nat. Photonics 11, 48 (2017)NPAHBY1749-488510.1038/nphoton.2016.231]. Our theory combines cavity quantum electrodynamics and quantum measurement theory, and it can be readily applied to explore conditional quantum dynamics and describe frequency measurements for other processes such as steady-state superradiance and superradiant Raman lasing.
A recent experiment demonstrated heterodyne detection-based frequency measurements with superradiant pulses from coherently pumped strontium atoms in an optical lattice clock system, while another experiment has analyzed the statistics of superradiant pulses from incoherently pumped calcium atoms in a similar system. In this article, we propose to perform heterodyne detection of the superradiant pulses from the calcium atoms, and analyze theoretically the corresponding atomic ensemble dynamics in terms of the rotation of a collective spin vector and the incoherent quantum jumps among superradiant Dicke states. We examine the effect of quantum measurement backaction on the emitted field and the collective spin vector dynamics, and we demonstrate that it plays an essential role in the modelling of the frequency measurements. We develop a stochastic mean field theory, which is also applicable to model frequency measurements with steady-state superradiance signals, and to explore quantum measurement effects in the dynamics of atomic ensembles.
Superradiant emission from long-lived excited states of an atomic ensemble confined in an optical cavity constitutes a practical source of light with narrow linewidth. In the pulsed regime, however, superradiance implies rapid emission and a broadening of the spectrum. Recent experiments have demonstrated constructive and destructive interference of superradiant emission by different strontium atomic transitions. In this article, we show that by modulating the atomic transition frequencies with a magnetic field, it is possible to control the release of the atomic excitation energy as a prolonged pulse or a train of superradiant pulses. By simulations, we show that heterodyne detection of the prolonged superradiance shows extremely sharp spectral features, which leads to significantly reduced frequency uncertainty and fluctuation.
We will describe a next-generation active atomic frequency reference based on super-radiant pulses of laser light from the ultra-narrow, 1 mHz linewidth, optical clock transition in an ensemble of cold 87Sr atoms. Light is stimulated from the millihertz linewidth transition by confining an ensemble of laser cooled atoms inside of a high finesse optical cavity. Such a light source has been proposed as a next-generation active atomic frequency reference, with the potential to enable high-precision optical frequency references to be used outside laboratory environments. We achieve a remarkable short term fractional frequency stability, 6.7 × 1016 at 1 s of averaging, absolute accuracy, 2 Hz (4 × 1015 fractional frequency), and high insensitivity to changes in the cavity length that limits the performance of todays more stable lasers. We will also discuss current work on cavity-enhanced dispersive measurements to perform high resolution spectroscopy and atom counting.
Recently, several theoretical proposals addressed the generation of an active optical frequency standard based on atomic ensembles trapped in an optical lattice potential inside an optical resonator. Using atoms with a narrow linewidth transition and population inversion together with a ``bad'' cavity allows us to realize the super-radiant photon emission regime. These schemes reduce the influence of mechanical or thermal vibrations of the cavity mirrors on the emitted optical frequency, overcoming current limitation in passive optical standards. The coherence time of the emitted light is ultimately limited by the lifetime of the atoms in the optical lattice potential. Therefore these schemes would produce one light pulse per atomic ensemble without a phase relation between pulses. Here we study how phase coherence between pulses can be maintained by using several inverted atomic ensembles, introduced into the cavity sequentially by means of a transport mechanism. We simulate the light emission process using the Heisenberg-Langevin approach and study the frequency noise of the intracavity field.
We demonstrate the state-of-the-art technique of an active clock to provide a continuous superradiant lasing signal using an ensemble of trapped Cs atoms in an optical lattice. A magic wavelength of the proposed $|7{S}_{1/2};F=4,{M}_{F}=0\ensuremath{\rangle}\ensuremath{\rightarrow}|6{P}_{3/2};F=3,{M}_{F}=0\ensuremath{\rangle}$ clock transition in Cs atoms is identified at 1181 nm for constructing the optical lattice. Pertinent optical lines are also found for pumping and repumping atoms from their ground states. A fractional uncertainty about ${10}^{\ensuremath{-}15}$ in the clock frequency has been predicted by carrying out rigorous calculations of several atomic properties. The bad-cavity operational mode of the active clock is anticipated to improve remarkably its short-term stability by suppressing intrinsic thermal fluctuations. Thus, a composite clock system with better short-term and long-term stabilities can be built by combining the proposed active clock with another high-accuracy passive optical clock.