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arXiv:2105.10494 · Physical Review A

Optimal atomic quantum sensing using electromagnetically-induced-transparency readout

David H. Meyer, Christopher O’Brien, Donald P. Fahey, Kevin C. Cox, Paul D. Kunz

Published Oct 5, 2021• 66 citations
arXivHTMLPDF

Abstract

Quantum sensors offer the capability to reach unprecedented precision by operating at the standard quantum limit (SQL) or beyond by using quantum entanglement. But an emerging class of quantum sensors that use Rydberg electromagnetically induced transparency (EIT) to detect rf electric fields have yet to reach the SQL. In this work we prove that this discrepancy is due to fundamental limitations in the EIT probing mechanism. We derive the optimum sensitivity of a three-level quantum sensor based on EIT, or more generally coherent spectroscopy, and compare this to the SQL. We apply a minimal set of assumptions, while allowing strong probing fields, thermal broadening, and large optical depth. We derive the optimal laser intensities and optical depth, providing specific guidelines for sensitive operation under common experimental conditions. Clear boundaries of performance are established, revealing that ladder-EIT cannot achieve the SQL due to unavoidable absorption loss. The results may be applied to any EIT-based quantum sensor, but we particularly emphasize our results' importance to the growing field of Rydberg quantum sensing.

DOI
10.1103/physreva.104.043103

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Quantum sensors offer the capability to reach unprecedented precision by operating at the standard quantum limit (SQL) or beyond by using quantum entanglement. But an emerging class of quantum sensors that use Rydberg electromagnetically induced transparency (EIT) to detect rf electric fields have yet to reach the SQL. In this work we prove that this discrepancy is due to fundamental limitations in the EIT probing mechanism. We derive the optimum sensitivity of a three-level quantum sensor based on EIT, or more generally coherent spectroscopy, and compare this to the SQL. We apply a minimal set of assumptions, while allowing strong probing fields, thermal broadening, and large optical depth. We derive the optimal laser intensities and optical depth, providing specific guidelines for sensitive operation under common experimental conditions. Clear boundaries of performance are established, revealing that ladder-EIT cannot achieve the SQL due to unavoidable absorption loss. The results may be applied to any EIT-based quantum sensor, but we particularly emphasize our results' importance to the growing field of Rydberg quantum sensing.
Abstract Atom-based sensing with optical readout is fundamentally limited by photon shot noise. Squeezed light can effectively suppress this noise of optical readout, thereby enabling measurement sensitivities beyond the standard quantum limit, but their application in light–atom hybrid systems is often hindered by absorption losses of atomic medium. Here, we demonstrate the first realization of electromagnetically induced transparency spectrum in a Rydberg-atom system using a squeezed probe field that surpasses the photon shot noise limit. Our theoretical model identifies atomic transit and absorption-induced losses as the primary factors limiting squeezing preservation. Experimentally, we engineer the atomic ensemble as a medium with tunable transmittance by employing Doppler-matched velocity-selective excitation to suppress absorption, achieving a squeezing transmission of 90.4 %\%% % for -1.7 dB squeezed light through a cesium vapor cell. This work is a critical step towards quantum-enhanced Rydberg atom sensors.
Rydberg atoms efficiently link photons between the radio-frequency (rf) and optical domains. They furnish a medium in which the presence of an rf field imprints on the transmission of a probe laser beam by altering the coherent coupling between atomic quantum states. The immutable atomic energy structure underpins quantum-metrological rf-field measurements and has driven intensive efforts to realize inherently self-calibrated sensing devices. Here, we investigate spectroscopic signatures owing to the quantization of atomic angular momentum. Using an electromagnetically induced transparency (EIT) sensing scheme, specific combinations of atomic terms are shown to give rise to universal, distinctive fingerprints in the detected optical fields upon rotating a linearly polarized rf field. Employing a dressed state picture, we identify two types of atomic angular momentum ladders that display strikingly disparate spectroscopic characteristics, including the distinctive absence or presence of a central spectral EIT peak. Our study adds important insights into the prospects of Rydberg atomic gases for quantum-metrological electric field characterization including polarimetry. In particular, it calls into question prevailing interpretations of SI-traceable Rydberg atom electrometers.
Rydberg atoms are neutral atoms excited to high principal quantum number states, which endows them with exaggerated properties such as large electric dipole moments, long lifetimes, and extreme sensitivity to external electromagnetic fields. These characteristics form the foundation of Rydberg atom-based sensors, an emerging class of quantum devices capable of optically detecting electric fields across frequencies from DC to the terahertz regime. Rydberg-based electrometry operates through both Autler–Townes (AT) splitting of resonant Rydberg transitions and Stark-shift measurements for high-frequency or far-detuned fields, enabling broadband field sensing from DC to the THz regime. Using ladder-type electromagnetically induced transparency (EIT) and AT splitting, these sensors enable non-invasive, SI-traceable measurements of field amplitude, frequency, phase, and polarization. Recent developments have demonstrated broadband electric field probes, voltage calibration standards, and compact RF receivers based on thermal vapor cells and integrated photonic architectures. Furthermore, innovations in multi-photon EIT, superheterodyne readout, and multi wave mixing have expanded the dynamic range and bandwidth of Rydberg-based electrometry. Despite challenges related to environmental perturbations, linewidth broadening, and laser stabilization, ongoing advances in atomic control, hybrid photonic integration, and EIT-based readout promise scalable, chip-compatible sensors. This review summarizes the physical principles, experimental progress, and emerging applications of Rydberg atom-based sensing, emphasizing their potential for next generation quantum metrology, wireless communication, and precision field mapping.
Abstract Quantum electrometric sensing properties of a four-level system are theoretically investigated for microwave (MW) field measurement in thermal Rydberg atoms. In the considered system, the phenomenon of electromagnetically induced transparency (EIT) is invoked to study the impact of microwave (MW) field strength on its optical response. The amplitude of the MW electric field is obtained directly by measuring the height and frequency of EIT peaks. Further, for MW frequency measurement, the probe spectra are examined for red and blue MW detuned cases. It is found that the responsiveness of 133Cs for MW electric field as well as frequency is relatively higher than 87Rb. The overall sensitivity of both these atoms can be enhanced by the convenient setting of the system and field parameters.
The Rydberg-based microwave detection is an all-optical technology that uses the strong coherent interaction between Rydberg atoms and microwave field. Different from the traditional microwave meter, the Rydberg atomic sensing is a new-type microwave detector that transforms the microwave spectrum into a coherent optical spectrum, and arouses increasingly the interests due to its high sensibility. For this kind of sensor, the coherence effect induced by coupling atoms with microwave plays a key role, and the decoherence may reduce the sensitivity. A multi-level Rydberg atomic scheme with optimized quantum coherence, which enhances both the bandwidth and the sensitivity for 4 GHz microwave sensing, is demonstrated experimentally in this work. The enhanced quantum coherence of Rydberg electromagnetically induced transparency (EIT) and microwave induced Autler-Townes (AT) splitting in EIT windows are shown using optical pumping at D1 line. The enhanced sensitivity at 3.4 GHz with 0.3 GHz bandwidth can be realized, based on the enhanced EIT-AT spectrum. The experimental results show that in the stepped Rydberg EIT system, the spectral width of EIT and microwave field EIT-AT can be narrowed by optical pumping (OP), so the sensitivity of microwave electric field measurement can be improved. After optimizing the EIT amplitude and adding single-frequency microwaves, the sensitivity of the microwave electric field measurement observed by the AT splitting interval is improved by 1.3 times. This work provides a reference for utilizing atomic microwave detection.
Rydberg-atom electrometry is a core technique in the development of highly sensitive quantum electric-field sensors. Its sensitivity based on atom-photon interaction is typically limited by photon shot-noise (PSN) and spectral broadenings. Here, we experimentally demonstrate a near PSN-limited Rydberg electrometry from a 85Rb atomic vapor cell. By engineering atomic coherence through control of residual magnetic fields and laser frequency noise, we achieve the Rydberg electromagnetically induced transparency (EIT) with the narrow linewidth of 1.6 MHz, yielding an enhanced spectral slope for high-sensitivity Rydberg-EIT electrometry. Under optimized superheterodyne detection conditions, we obtain an electric-field sensitivity of 12.5(8) nV cm^-1 Hz^-1/2 at 37 GHz, in close agreement with the calculated PSN limit. These results provide direct experimental evidence of the high-sensitive quantum electrometry and establish a practical route toward quantum-noise-limited Rydberg electrometry.