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arXiv:2503.17997 · Physical Review Research

Electromagnetically induced transparency spectroscopy of Rydberg levels dressed by linearly polarized rf fields: Complementary angular response for two types of transition ladders

Matthew Cloutman, Matthew Chilcott, Alexander Elliott, J. Susanne Otto, Amita B. Deb, Niels Kjærgaard

Published Jun 5, 2026• 1 citation
arXivHTMLPDF

Abstract

Rydberg atoms efficiently link photons between the radio-frequency (rf) and optical domains. They furnish a medium in which the presence of an rf field imprints on the transmission of a probe laser beam by altering the coherent coupling between atomic quantum states. The immutable atomic energy structure underpins quantum-metrological rf-field measurements and has driven intensive efforts to realize inherently self-calibrated sensing devices. Here, we investigate spectroscopic signatures owing to the quantization of atomic angular momentum. Using an electromagnetically induced transparency (EIT) sensing scheme, specific combinations of atomic terms are shown to give rise to universal, distinctive fingerprints in the detected optical fields upon rotating a linearly polarized rf field. Employing a dressed state picture, we identify two types of atomic angular momentum ladders that display strikingly disparate spectroscopic characteristics, including the distinctive absence or presence of a central spectral EIT peak. Our study adds important insights into the prospects of Rydberg atomic gases for quantum-metrological electric field characterization including polarimetry. In particular, it calls into question prevailing interpretations of SI-traceable Rydberg atom electrometers.

DOI
10.1103/gcms-2yhg

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Rydberg atoms efficiently link photons between the radio-frequency (rf) and optical domains. They furnish a medium in which the presence of an rf field imprints on the transmission of a probe laser beam by altering the coherent coupling between atomic quantum states. The immutable atomic energy structure underpins quantum-metrological rf-field measurements and has driven intensive efforts to realize inherently self-calibrated sensing devices. Here, we investigate spectroscopic signatures owing to the quantization of atomic angular momentum. Using an electromagnetically induced transparency (EIT) sensing scheme, specific combinations of atomic terms are shown to give rise to universal, distinctive fingerprints in the detected optical fields upon rotating a linearly polarized rf field. Employing a dressed state picture, we identify two types of atomic angular momentum ladders that display strikingly disparate spectroscopic characteristics, including the distinctive absence or presence of a central spectral EIT peak. Our study adds important insights into the prospects of Rydberg atomic gases for quantum-metrological electric field characterization including polarimetry. In particular, it calls into question prevailing interpretations of SI-traceable Rydberg atom electrometers.
Rydberg atomic electrometry leverages the extreme sensitivity of highly excited atoms for calibration-free electric field measurements. The technique uses a non-metallic vapor cell to link properties of an RF field to a spectroscopic readout in the optical domain. Most demonstrations have so far focused on detecting linearly-polarized fields, for which the induced splitting of dressed atomic levels is rotationally invariant. Here we report on Rydberg atomic measurements of RF fields in a general state of polarization (SOP) which we map onto the Poincaré sphere through spectroscopic fingerprints. For a Stokes vector circumnavigating a Poincaré sphere meridian, we witness a continuous transformation of the atomic eigenenergy spectrum. Because the relative positions of eigenenergies are locked in place by quantization of angular momentum, the framework is universal and calibration free. We provide a specific demonstration in rubidium, which generalizes to all systems with a single valence electron.
The large electric dipole moment of the Rydberg atom allows for strong coupling with weak electric fields, and is widely used in electric field measurements because of its reproducibility, precision and stability. The combination of Rydberg atoms and electromagnetically induced transparency (EIT) technology has been used for detecting and characterizing radio-frequency (RF) electric fields. In this work, by selecting probe light (852 nm), dressed light (1470 nm), and coupled light (780 nm), the Rydberg state (49P3/2) of Cs atom is prepared by using a three-photon excitation scheme through using all-infrared light excitation of Rydberg atoms. We experimentally observe the EIT spectra of the Rydberg states decorated by radio-frequency electric fields, which optically detects Rydberg atoms. The effect of the amplitude and frequency of the RF electric field on the spectrum is explored in light of changes in the EIT spectrum. The results show that in the region of weak electric field, only the ac Stark energy shift and spectral broadening occur. As the electric field is further enhanced, the sideband phenomenon occurs in both the primary peak and secondary peak of the EIT. In the region of strong field, the Rydberg energy level produces a series of Floquet states with higher-order terms, as well as state shifting and mixing, resulting in asymmetry in the spectra of the EIT sideband peaks. The effect of frequency on the shielding effect of the Cs vapor cell is further discussed based on the shift of the main peak of the EIT. The demodulation of the electric field in a range of 50 Hz–1 kHz with a fidelity of 95% is achieved by modulating the low-frequency electric field to the RF electric field. The results can provide valuable references for spectral detection and traceable measurements of low-frequency electric fields.
Abstract We study electromagnetically induced transparency (EIT) in a room-temperature cesium vapor cell using wavelength-modulated probe laser light. In the utilized cascade level scheme, the probe laser drives the lower transition 6 S 1 / 2 ( F = 4) → 6 P 3 / 2 ( F ’ = 5), while the coupling laser drives the Rydberg transition 6 P 3 / 2 → 57 S 1 / 2 . The probe laser has a fixed average frequency and is modulated at a frequency of a few kHz, with a variable modulation amplitude in the range of tens of MHz. The probe transmission is measured as a function of the detuning of the coupling laser from the Rydberg resonance. The first-harmonic demodulated EIT signal has two peaks that are, in the case of large modulation amplitude, separated by the peak-to-peak modulation amplitude of the probe laser times a scaling factor λ p / λ c , where λ p and λ c are the probe- and coupling-laser wavelengths. The scaling factor is due to Doppler shifts in the EIT geometry. Second-harmonic demodulated EIT signals, obtained with small modulation amplitudes, yield spectral lines that are much narrower than corresponding lines in the modulation-free EIT spectra. The resultant spectroscopic resolution enhancement is conducive to improved measurements of radio-frequency (RF) fields based on Rydberg-atom EIT, an approach in which the response of Rydberg atoms to RF fields is exploited to characterize RF fields. Here, we employ wavelength modulation spectroscopy to reduce the uncertainty of atom-based frequency and field measurement of an RF field in the VHF radio band.
We present experimental results on the influence of magnetic fields and laser polarization on electromagnetically induced transparency (EIT) using Rydberg levels of ^{87} 87 Rb atoms. The measurements are performed in a room temperature vapor cell with two counter-propagating laser beams at 480 m and 780 m in a ladder-type energy level scheme. We measure the EIT spectrum of a range of ns_{1/2} n s 1 / 2 Rydberg states for n=19-27 n = 19 − 27 , where the hyperfine structure can still be resolved. Our measurements span the range of magnetic fields from the low field linear Zeeman regime to the high field Paschen-Back regimes. The observed spectra are very sensitive to small changes in magnetic fields and the polarization of the laser beams. We model our observations using optical Bloch equations that take into account the full multi-level structure of the atomic states involved and the decoupling of the electronic J J and nuclear I I angular momenta in the Breit-Rabi regime. The numerical model yields excellent agreement with the observations. In addition to EIT related experiments, our results are relevant for experiments involving coherent excitation to Rydberg levels in the presence of magnetic fields.
In this work, Electromagnetically Induced Transparency (EIT) has been studied in a RF-driven four-level ladder85Rb atomic model. Rb atomic cell is simultaneously driven by three fields; two lasers, namely control and probe and one microwave. This spectroscopic technique of exposing atomic vapors to three energies may get established as a quantum primary standard for the RF electric-field amplitude metrology due to its dependency only on universal Plank's constant. It is observed that when right resonant frequency is achieved the absorption spectrum gives a transition to EIT by inducing a window in middle of the curve cancelling the absorption. In addition, two-dimensional localization of an atom is also studied in various field scenarios. The maxima of absorption spectrum can be modified by making slight modifications in the electromagnetic fields driving the system. Next step in the metrology would be of measuring vector E-field for which finding the position of an atom may play a crucial role. This may add one extra degree of freedom in the evaluation of SI traceable E-field.
We prepare and analyze Rydberg states with orbital quantum numbers ℓ≤6 using three-optical-photon electromagnetically induced transparency (EIT) and radio frequency (rf) dressing, and employ the high- ℓ states in electric-field sensing. Rubidium-85 atoms in a room-temperature vapor cell are first promoted into the 25F5/2 state via Rydberg-EIT with three infrared laser beams. Two rf dressing fields then (near-)resonantly couple the 25F, 25H(ℓ=5) , and 25I(ℓ=6) Rydberg states. The dependence of the rf-dressed Rydberg-state level structure on rf powers, rf and laser frequencies is characterized using EIT. Furthermore, we discuss the principles of dc-electric-field sensing using high- ℓ Rydberg states and experimentally demonstrate the method using test electric fields of ≲50 V/m induced via photo-illumination of the vapor-cell wall. We measure the highly nonlinear dependence of the dc-electric-field strength on the power of the photo-illumination laser. Numerical calculations, which reproduce our experimental observations well, elucidate the underlying physics. Our paper is relevant to high-precision spectroscopy of high- ℓ Rydberg states, Rydberg-atom-based electric-field sensing, and plasma electric-field diagnostics. Published by the American Physical Society 2024