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arXiv:2105.09399 · Science Advances

Coherence in cooperative photon emission from indistinguishable quantum emitters

Zhe Xian Koong, Moritz Cygorek, Eleanor Scerri, Ted Silva Santana, Suk In Park, Jin Dong Song, Erik M. Gauger, Brian D. Gerardot

Published Mar 18, 2022• 42 citations
arXivHTMLPDF

Abstract

Photon-mediated interactions between atoms can arise via coupling to a common electromagnetic mode or by quantum interference. Here, we probe the role of coherence in cooperative emission arising from two distant but indistinguishable solid-state emitters because of path erasure. The primary signature of cooperative emission, the emergence of "bunching" at zero delay in an intensity correlation experiment, is used to characterize the indistinguishability of the emitters, their dephasing, and the degree of correlation in the joint system that can be coherently controlled. In a stark departure from a pair of uncorrelated emitters, in Hong-Ou-Mandel-type interference measurements, we observe photon statistics from a pair of indistinguishable emitters resembling that of a weak coherent state from an attenuated laser. Our experiments establish techniques to control and characterize cooperative behavior between matter qubits using the full quantum optics toolbox, a key step toward realizing large-scale quantum photonic networks.

DOI
10.1126/sciadv.abm8171

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Photon-mediated interactions between atoms can arise via coupling to a common electromagnetic mode or by quantum interference. Here, we probe the role of coherence in cooperative emission arising from two distant but indistinguishable solid-state emitters because of path erasure. The primary signature of cooperative emission, the emergence of "bunching" at zero delay in an intensity correlation experiment, is used to characterize the indistinguishability of the emitters, their dephasing, and the degree of correlation in the joint system that can be coherently controlled. In a stark departure from a pair of uncorrelated emitters, in Hong-Ou-Mandel-type interference measurements, we observe photon statistics from a pair of indistinguishable emitters resembling that of a weak coherent state from an attenuated laser. Our experiments establish techniques to control and characterize cooperative behavior between matter qubits using the full quantum optics toolbox, a key step toward realizing large-scale quantum photonic networks.
Photon-mediated interactions between atomic systems are the cornerstone of quantum information transfer. They can arise via coupling to a common electromagnetic mode or by quantum interference. This can manifest in cooperative light-matter coupling, yielding collective rate enhancements such as those at the heart of superradiance, or remote entanglement via measurement-induced path erasure. Here, we report coherent control of cooperative emission arising from two distant but indistinguishable solid-state emitters due to path erasure. The primary signature of cooperative emission, the emergence of bunching at zero-delay in an intensity correlation experiment, is used to characterise the indistinguishability of the emitters, their dephasing, and the degree of correlation in the joint system which can be coherently controlled. In a stark departure from a pair of uncorrelated emitters, we observe photon statistics resembling that of a weak coherent state in Hong-Ou-Mandel type interference measurements. Our experiments establish new techniques to control and characterize cooperative behaviour between matter qubits using the full quantum optics toolbox, a key stepping stone on the route to realising large-scale quantum photonic networks.
Quantum interference of indistinguishable photons is the foundation of photonic quantum technologies, yet scaling from a few to many identical quantum light sources remains a major challenge. In solid-state platforms, spatial and spectral inhomogeneity and resource-intensive architectures impede scaling. As a result, interference between remote, independent quantum emitters has been thus far limited to pairs. Here we introduce a wavefront-shaping approach that enables scalable interference from multiple indistinguishable quantum dots on the same chip. Using programmable spatial light modulators, we independently excite, collect, and route emission from spatially distinct, yet spectrally degenerate dots. Scaling from two to five indistinguishable emitters, we verify interference through cooperative-emission phenomena and Hong-Ou-Mandel two-photon interference, thereby establishing a route towards large-scale, programmable quantum photonic architectures.
Quantum emitters such as quantum dots, defects in diamond or in silicon have emerged as efficient single-photon sources that are progressively exploited in quantum technologies. In 2019, it was shown that the emitted single-photon states often include coherence with the vacuum component. Here we investigate how such photon-number coherence alters quantum interference experiments that are routinely implemented both for characterizing or exploiting the generated photons. We show that it strongly modifies intensity correlation measurements in a Hong–Ou–Mandel experiment and leads to errors in indistinguishability estimations. It also results in additional entanglement when performing partial measurements. We illustrate the impact on quantum protocols by evidencing modifications in heralding efficiency and fidelity of two-qubit gates.
Indistinguishable quantum emitters confined to length scales smaller than the wavelength of the light become superradiant. Compared to uncorrelated and distinguishable emitters, superradiance results in qualitative modifications of optical signals such as photon coincidences. However, recent experiments revealed that similar signatures can also be obtained in situations where emitters are too far separated to be superradiant if correlations between emitters are induced by the wave-function collapse during an emission-angle-selective photon detection event. Here, we compare two sources for cooperative emission, superradiance and measurement-induced cooperativity, and analyze their impact on time-dependent optical signals. We find that an antidip in photon coincidences at zero time delay is a signature of interemitter correlations in general but does not unambiguously prove the presence of superradiance. This suggests that photon coincidences at zero time delay alone are not sufficient and time-dependent data are necessary to clearly demonstrate a superradiant enhancement of the spontaneous radiative decay rate.
Photon indistinguishability constitutes an essential resource in modern physics. At the scale of individual atoms and photons, it is a diverse concept that causes different coherent phenomena. We present the experimental characterization of indistinguishable photons detected in a single mode from a finite and stable ensemble of single-photon emitters: trapped ions. We conclusively observe an increase of second-order correlation and super-Poissonian statistics of these photons with a number of contributing phase-incoherent independent emissions from the atoms, ranging from a single to up to several hundred. This optical emission regime provides insight into the emergence of super-Poissonian light at the atomic scale by photon indistinguishability. It constitutes a unique toolbox for its generation and control at the most microscopic level.
The ability to entangle distant quantum nodes is essential for the construction of quantum networks and for quantum information processing. For solid-state quantum emitters used as qubits, it can be achieved by photon interference. When the emitter is subject to spectral diffusion, this process can become highly inefficient, impeding the achievement of scalable quantum technologies. We study two-photon interference in the context of a Hong-Ou-Mandel (HOM)-type experiment for two separate quantum emitters, with different detunings with respect to a specific target frequency. We evaluate the second order coherences that characterize photon indistinguishability between the two emitters. We find that the two-photon interference operation that is inefficient in the absence of a control protocol, when the two detunings are different and spectral overlap is lessened, can be highly improved by a periodic sequence of $\ensuremath{\pi}$ pulses at a set target frequency. Photon indistinguishability in solid state and other quantum emitters subject to spectral diffusion can thus be enhanced by the proposed pulse sequence and similar external control protocols despite the fluctuations in the environment.