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Optica

Emergence of super-Poissonian light from indistinguishable single-photon emitters

Artem Kovalenko, D. Babjak, Adam Lešundák, Lukáš Podhora, Lukáš Lachman, Petr Obšil, T. Pham, Ondřej Čı́p, Radim Filip, L. Slodička

Published Feb 27, 2023• 5 citations
Publisher

Abstract

Photon indistinguishability constitutes an essential resource in modern physics. At the scale of individual atoms and photons, it is a diverse concept that causes different coherent phenomena. We present the experimental characterization of indistinguishable photons detected in a single mode from a finite and stable ensemble of single-photon emitters: trapped ions. We conclusively observe an increase of second-order correlation and super-Poissonian statistics of these photons with a number of contributing phase-incoherent independent emissions from the atoms, ranging from a single to up to several hundred. This optical emission regime provides insight into the emergence of super-Poissonian light at the atomic scale by photon indistinguishability. It constitutes a unique toolbox for its generation and control at the most microscopic level.

DOI
10.1364/optica.474897

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Photon indistinguishability constitutes an essential resource in modern physics. At the scale of individual atoms and photons, it is a diverse concept that causes different coherent phenomena. We present the experimental characterization of indistinguishable photons detected in a single mode from a finite and stable ensemble of single-photon emitters: trapped ions. We conclusively observe an increase of second-order correlation and super-Poissonian statistics of these photons with a number of contributing phase-incoherent independent emissions from the atoms, ranging from a single to up to several hundred. This optical emission regime provides insight into the emergence of super-Poissonian light at the atomic scale by photon indistinguishability. It constitutes a unique toolbox for its generation and control at the most microscopic level.
The optical interference constitutes a paramount resource in modern physics. At the scale of individual atoms and photons, it is a diverse concept that causes different coherent phenomena. We present the experimental characterization of both coherent and statistical properties of light emitted from ensembles of trapped ions increasing with a number of contributing phase-incoherent independent atomic particles ranging from a single to up to several hundreds. It conclusively demonstrates how super-Poissonian quantum statistics non-trivially arises purely from the finite number of indistinguishable single-photon emitters in the limit of a single detection mode. The achieved new optical emission regime in which these independent atoms contribute coherently to the super-Poissonian statistics provides a new perspective on the emergence of optical coherence at the atomic scale and constitutes a unique toolbox for its generation and control at the most microscopic level.
Photon-mediated interactions between atoms can arise via coupling to a common electromagnetic mode or by quantum interference. Here, we probe the role of coherence in cooperative emission arising from two distant but indistinguishable solid-state emitters because of path erasure. The primary signature of cooperative emission, the emergence of "bunching" at zero delay in an intensity correlation experiment, is used to characterize the indistinguishability of the emitters, their dephasing, and the degree of correlation in the joint system that can be coherently controlled. In a stark departure from a pair of uncorrelated emitters, in Hong-Ou-Mandel-type interference measurements, we observe photon statistics from a pair of indistinguishable emitters resembling that of a weak coherent state from an attenuated laser. Our experiments establish techniques to control and characterize cooperative behavior between matter qubits using the full quantum optics toolbox, a key step toward realizing large-scale quantum photonic networks.
If a beam of light is coherent, then the photons constituting the beam arrive at random moments in time. Consequently, the photon counting statistics in a given time interval below the coherence time, should in theory follow a Poissonian distribution. When the measurement interval exceeds the coherence time, the distribution should broaden and become a super-Poissonian distribution. The aim of this study is to experimentally demonstrate the Poissonian nature of light, as well as quantifying the transition to a super-Poissonian distribution. In the experiment, a low-intensity laser beam was measured with single-photon detectors, able to capture individual photons. The arrival time of the photons was detected with an oscilloscope, and the data further analysed with our own Python code. The probability distribution of the arrival time of photons was constructed and fitted with a Poissonian distribution for different time intervals. The results showed a clear Poissonian distribution for all intervals from 0.2 μs up to 2000 μs. We did however, observe tendencies of randomness for the longest measured intervals. A Poissonian distribution is defined by the variance being equal to the mean, whilst for a super-Poissonian distribution the variance is higher. The biggest measured ratio between the variance and the mean in our experiment was 1.06 for interval time 2000 μs, which is too small to infer super-Poissonian. Due to limited data memory, our dataset was restricted in length and resolution. Therefore, longer intervals could not be studied without statistical uncertainty. To cross-check the result we also calculated the probability distribution for the arrival time itself. The result perfectly fitted an exponential distribution which was in accordance with the theory of coherent light. Hence, within the given measurement accuracy and statistical uncertainty, it is safe to conclude that the laser beam is coherent for all tested time intervals. However, this does not allow us to conclude that it is a single-mode laser.
The vast majority of physical objects we are dealing with are almost exclusively made of atoms. Because of their discrete level structure, single atoms have proved to be emitters of light, which is incompatible with the classical description of electromagnetic waves. We demonstrate this incompatibility for atomic fluorescence when scaling up the size of the source ensemble, which consists of trapped atomic ions, by several orders of magnitude. The presented measurements of nonclassical statistics on light unconditionally emitted from ensembles containing up to more than a thousand ions promise further scalability to much larger emitter numbers. The methodology can be applied to a broad range of experimental platforms focusing on the bare nonclassical character of single isolated emitters.
Modification of spontaneous decay in space and time is a central topic of quantum physics. It has been predominantly investigated in the context of cavity quantum electrodynamics (QED), gaining new interest recently in the domain of nano-optics. Beyond cavity-QED, spontaneous emission may be modified also in free space due to correlations among the photon emitters, a phenomenon known as super- and sub-radiance. Correlations may stem either from direct interactions between the particles, from long-range exchange of photons, or by measuring single photons in a common mode. Yet, the genuine spatial spontaneous emission pattern of an atomic ensemble in an entangled quantum state has not been observed so far, due to the lack of ultra-fast cameras with high spatial resolution suited for recording single photons from single atoms. Preparing two trapped ions in free space in entangled Dicke states via photon detection, we study the resulting collective spontaneous emission patterns. Depending on the symmetry of the Dicke states, associated with the direction of detection of the first state-determining photon, we observe fundamentally different emission patterns for the subsequently scattered photon, including super- and sub-radiance. Our results demonstrate that the detection of a single photon can profoundly modify the collective emission of an atomic array, here represented by its most elementary building block of two atoms in free space.