We study the dynamics of a quantum two state system driven through an avoided crossing under the influence of a super Ohmic environment, i.e. a longitudinal as well as a transversal one. The crossing time window, in which relaxation influences the dynamics, is centered around the avoided crossing. We determine the dynamics and the Landau-Zener probability employing the numerical exact quasi-adiabatic path integral. At weak coupling we show that the numerically less demanding nonequilibrium Bloch equations provide an accurate description. The crossing time depends strongly not only on the system-bath coupling strength but also on the bath spectral cut-off frequency in contrast to the situation in an Ohmic bath. Our results enable to design quantitative protocols which drive quantum systems out of the influence range of relaxation.
We study the dynamics of a quantum two state system driven through an avoided crossing under the influence of a super Ohmic environment, i.e. a longitudinal as well as a transversal one. The crossing time window, in which relaxation influences the dynamics, is centered around the avoided crossing. We determine the dynamics and the Landau-Zener probability employing the numerical exact quasi-adiabatic path integral. At weak coupling we show that the numerically less demanding nonequilibrium Bloch equations provide an accurate description. The crossing time depends strongly not only on the system-bath coupling strength but also on the bath spectral cut-off frequency in contrast to the situation in an Ohmic bath. Our results enable to design quantitative protocols which drive quantum systems out of the influence range of relaxation.
Abstract We study the dynamics of a quantum two-state system driven through an avoided crossing under the influence of a super-Ohmic environment. We determine the Landau–Zener probability employing the numerical exact quasi-adiabatic path integral and a Markovian weak coupling approach. Increasing the driving time in the numerical protocol, we find converged results which shows that super-Ohmic environments only influence the Landau Zener probability within a finite crossing time window. This crossing time is qualitatively determined by the environmental cut-off energy. At weak coupling, we show that the Markovian weak coupling approach provides an accurate description. Since pure dephasing of a super-Ohmic bath is non-Markovian, this highlights that pure dephasing hardly influences the Landau–Zener probability. The finite crossing time window, thus, results from the suppression of relaxation once the energy splitting exceeds the environmental cut-off energy. Graphical abstract
We investigate the dissipative influence of environmental fluctuations on the dynamics of driven quantum systems at an avoided crossing. We derive two simple approximative equations valid for weak system-bath coupling and compare results for the dissipative Landau-Zener problem with numerically exact results. Very good agreement is found for slow, i.e., adiabatic, driving. Specifically, the minimum in the Landau-Zener probability resulting from the competition of driving and dissipation is well described. For system-bath couplings and temperatures, where this minimum is observed in the adiabatic driving regime, good agreement is also observed for fast driving when the dynamics tends toward nonadiabatic behavior. Otherwise, however, for large temperatures and fast driving our approximation fails even for weak system-bath couplings, for which an undriven system is still accurately described by weak-coupling approximations.
We determine the Landau-Zener transition probability in a dissipative environment including both longitudinal as well as transversal quantum-mechanical noise originating from a single noise source. For this, we use the numerically exact quasiadiabatic path integral, as well as the approximative nonequilibrium Bloch equations. We find that transversal quantum noise in general influences the Landau-Zener probability much more strongly than longitudinal quantum noise does at a given temperature and system-bath coupling strength. In other words, transversal noise contributions become important even when the coupling strength of transversal noise is smaller than that of longitudinal noise. We furthermore reveal that transversal noise renormalizes the tunnel coupling independent of temperature. Finally, we show that the effect of mixed longitudinal and transversal noise originating from a single bath cannot be obtained from an incoherent sum of purely longitudinal and purely transversal noise.
Abstract We investigate the quantum dynamics of a multilevel bistable system coupled to a bosonic heat bath beyond the perturbative regime. We consider different spectral densities of the bath, in the transition from sub-Ohmic to super-Ohmic dissipation, and different cutoff frequencies. The study is carried out by using the real-time path integral approach of the Feynman–Vernon influence functional. We find that, in the crossover dynamical regime characterized by damped intrawell oscillations and incoherent tunneling, the short time behavior and the time scales of the relaxation starting from a nonequilibrium initial condition depend nontrivially on the spectral properties of the heat bath.
The stabilizing effect of quantum fluctuations on the escape process and the relaxation dynamics from a quantum metastable state are investigated. Specifically, the quantum dynamics of a multilevel bistable system coupled to a bosonic Ohmic thermal bath in strong dissipation regime is analyzed. The study is performed by a non-perturbative method based on the real-time path integral approach of the Feynman-Vernon influence functional. We consider a strongly asymmetric double well potential with and without a monochromatic external driving, and with an out-of-equilibrium initial condition. In the absence of driving we observe a nonmonotonic behavior of the escape time from the metastable region, as a function both of the system-bath coupling coefficient and the temperature. This indicates a stabilizing effect of the quantum fluctuations. In the presence of driving our findings indicate that, as the coupling coefficient γ increases, the escape time, initially controlled by the external driving, shows resonant peaks and dips, becoming frequency-independent for higher γ values. Moreover, the escape time from the metastable state displays a nonmonotonic behavior as a function of the temperature, the frequency of the driving, and the thermal-bath coupling, which indicates the presence of a quantum noise enhanced stability phenomenon. Finally, we investigate the role of different spectral densities, both in sub-Ohmic and super-Ohmic dissipation regime and for different cutoff frequencies, on the relaxation dynamics from the quantum metastable state. The results obtained indicate that, in the crossover dynamical regime characterized by damped intrawell oscillations and incoherent tunneling, the spectral properties of the thermal bath influence non-trivially the short time behavior and the time scales of the relaxation dynamics from the metastable state.
Dephasing in quantum systems is typically the result of their interaction with environmental degrees of freedom. We investigate within a spin-boson model the influence of a super-Ohmic environment on the dynamics of a quantum two-state system. A super-Ohmic environment thereby models typical bulk phonons which are a common disturbance for solid state quantum systems as, for example, nitrogen-vacancy centers. By applying the numerically exact quasiadiabatic path-integral approach we show that for strong system-bath coupling, pseudocoherent dynamics emerges, i.e., oscillatory dynamics at short times due to slaving of the quantum system to the bath dynamics. We extend the phase diagram known for sub-Ohmic and Ohmic environments into the super-Ohmic regime and observe a pronounced nonmonotonous behavior. Super-Ohmic purely dephasing fluctuations strongly suppress the amplitude of coherent dynamics at very short times with no subsequent further decay at later times. Nevertheless, they render the dynamics overdamped. The corresponding phase separation line shows also a nonmonotonous behavior, very similar to the pseudocoherent dynamics.