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arXiv:2303.18213 · Physical Review A

Dephasing and pseudocoherent quantum dynamics in super-Ohmic environments

Ph. Nacke, Florian Otterpohl, Michael Thorwart, P. Nalbach

Published Jun 28, 2023• 9 citations
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Abstract

Dephasing in quantum systems is typically the result of their interaction with environmental degrees of freedom. We investigate within a spin-boson model the influence of a super-Ohmic environment on the dynamics of a quantum two-state system. A super-Ohmic environment thereby models typical bulk phonons which are a common disturbance for solid state quantum systems as, for example, nitrogen-vacancy centers. By applying the numerically exact quasiadiabatic path-integral approach we show that for strong system-bath coupling, pseudocoherent dynamics emerges, i.e., oscillatory dynamics at short times due to slaving of the quantum system to the bath dynamics. We extend the phase diagram known for sub-Ohmic and Ohmic environments into the super-Ohmic regime and observe a pronounced nonmonotonous behavior. Super-Ohmic purely dephasing fluctuations strongly suppress the amplitude of coherent dynamics at very short times with no subsequent further decay at later times. Nevertheless, they render the dynamics overdamped. The corresponding phase separation line shows also a nonmonotonous behavior, very similar to the pseudocoherent dynamics.

DOI
10.1103/physreva.107.062218

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Dephasing in quantum systems is typically the result of their interaction with environmental degrees of freedom. We investigate within a spin-boson model the influence of a super-Ohmic environment on the dynamics of a quantum two-state system. A super-Ohmic environment thereby models typical bulk phonons which are a common disturbance for solid state quantum systems as, for example, nitrogen-vacancy centers. By applying the numerically exact quasiadiabatic path-integral approach we show that for strong system-bath coupling, pseudocoherent dynamics emerges, i.e., oscillatory dynamics at short times due to slaving of the quantum system to the bath dynamics. We extend the phase diagram known for sub-Ohmic and Ohmic environments into the super-Ohmic regime and observe a pronounced nonmonotonous behavior. Super-Ohmic purely dephasing fluctuations strongly suppress the amplitude of coherent dynamics at very short times with no subsequent further decay at later times. Nevertheless, they render the dynamics overdamped. The corresponding phase separation line shows also a nonmonotonous behavior, very similar to the pseudocoherent dynamics.
We report exact results for the influence of purely sub-Ohmic dephasing on the dynamics of a quantum two-level system. From response functions, we determine a crossover coupling strength between oscillatory coherent and overdamped dynamics. Surprisingly, we find no overdamping even at arbitrary large dephasing for spectra with spectral exponent s<scs<{s}_{c}s<sc​. For ${s}_{c}<s\ensuremath{\le}1$ we observe a crossover to overdamped dynamics but a reemergence of oscillatory behavior at very large couplings. Thus experimentally tuning the character of fluctuations from relaxational to dephasing should allow us to suppress the dephasing character of sub-Ohmic and thus 1/f1/f1/f noise.
A quantum two-level system immersed in a sub-Ohmic bath experiences enhanced low-frequency quantum statistical fluctuations which render the nonequilibrium quantum dynamics highly non-Markovian. Upon using the numerically exact time-evolving matrix product operator approach, we investigate the phase diagram of the polarization dynamics. In addition to the known phases of damped coherent oscillatory dynamics and overdamped decay, we identify a new third region in the phase diagram for strong coupling showing an aperiodic behavior. We determine the corresponding phase boundaries. The dynamics of the quantum two-state system herein is not coherent by itself but slaved to the oscillatory bath dynamics.
The decoherence of a two-state system coupled with a sub-Ohmic bath is investigated theoretically by means of the perturbation approach based on a unitary transformation. It is shown that the decoherence depends strongly and sensitively on the structure of environment. Nonadiabatic effect is treated through the introduction of a function ${\ensuremath{\xi}}_{k}$ which depends on the boson frequency and renormalized tunneling. The results are as follows: (i) the nonequilibrium correlation function P(t)P(t)P(t), the dynamical susceptibility ${\ensuremath{\chi}}^{\ensuremath{''}}(\ensuremath{\omega})$, and the equilibrium correlation function C(t)C(t)C(t) are analytically obtained for $s\ensuremath{\leqslant}1$; (ii) the phase diagram of thermodynamic transition shows the delocalized-localized transition point ${\ensuremath{\alpha}}_{l}$ which agrees with exact results and numerical data from the numerical renormalization group; (iii) the dynamical transition point ${\ensuremath{\alpha}}_{c}$ between coherent and incoherent phase is explicitly given. A crossover from the coherent oscillation to incoherent relaxation appears with increasing coupling (for $\ensuremath{\alpha}>{\ensuremath{\alpha}}_{c}$, the coherent dynamics disappear); (iv) the Shiba's relation and sum rule are exactly satisfied when $\ensuremath{\alpha}\ensuremath{\leqslant}{\ensuremath{\alpha}}_{c}$; (v) an underdamping-overdamping transition point ${\ensuremath{\alpha}}_{c}^{*}$ exists in the function $S(\ensuremath{\omega})$. Consequently, the dynamical phase diagrams in both ohmic and sub-Ohmic case are mapped out. For $\ensuremath{\Delta}⪡{\ensuremath{\omega}}_{c}$, the critical couplings (${\ensuremath{\alpha}}_{l},{\ensuremath{\alpha}}_{c}$, and ${\ensuremath{\alpha}}_{c}^{*}$) are proportional to ${\ensuremath{\Delta}}^{1\ensuremath{-}s}$.
Quantum mechanics describes the unitary time evolution of closed systems. In practice, every quantum system interacts with the environment, leading to an irreversible loss of coherence. The spin-boson model (SBM) is central to the understanding of the fundamental process of decoherence of a two-state quantum system interacting with a bosonic heat bath, but the nature of transient dynamics in the presence of hybrid diagonal and off-diagonal system-bath interactions remains much less explored. Here, we investigate how the hybrid system-bath interactions of an Ohmic environment induce localization in the bias-free SBM. For strong coupling to the environment, localization is strongly affected by a dynamically generated bias via the renormalization of the tunneling amplitude. We find that counteracting effects of Hamiltonian parameters on non-exponential short-time dynamics and long-time population equilibration can lead to a separation of timescales and transient quantum coherent dynamics that can persist even for ultra-strong system-bath interaction. The findings offer novel insight into the equilibration behavior of quantum devices operating in the ultra-strong coupling regime.
Quantum mechanics describes the unitary time evolution of closed systems. In practice, every quantum system interacts with the environment leading to an irreversible loss of coherence. The Spin-Boson model (SBM) is central to the understanding of the fundamental process of decoherence of a two-state quantum system interacting with a bosonic heat bath but the nature of transient dynamics in the presence of hybrid diagonal and off-diagonal system-bath interactions remains largely unexplored. Here, we investigate how the hybrid system-bath interactions of an Ohmic environment induce localization in the bias-free SBM. For strong coupling to the environment, localization is strongly affected by a dynamically generated bias via the renormalization of the tunneling amplitude. We find that counteractive effects of Hamiltonian parameters on non-exponential short-time dynamics and long-time population equilibration can lead to a separation of timescales and non-equilibrium quantum coherent dynamics that can persist even for ultra-strong system-bath interaction. The findings offer novel opportunities to exploit coherence as a resource in quantum devices operating in the ultra-strong coupling regime.
We study the dissipative quantum dynamics and the asymptotic behavior of a particle in a bistable potential interacting with a sub-Ohmic broadband environment. The reduced dynamics, in the intermediate to strong dissipation regime, is obtained beyond the two-level system approximation by using a real-time path integral approach. We find a crossover dynamic regime with damped intra-well oscillations and incoherent tunneling and a completely incoherent regime at strong damping. Moreover, a nonmonotonic behavior of the left/right well population difference is found as a function of the damping strength.