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arXiv:2102.04749 · Optica

Chiral light–matter interactions in hot vapor-cladded waveguides

Roy Zektzer, Eliran Talker, Yefim Barash, Noa Mazurski, Uriel Levy

Published Dec 20, 2018• 23 citations
arXivHTMLPDF

Abstract

Recently, there is growing interest in integrating alkali vapors with nanoscale photonic structures, such as nano-waveguides, resonators and nanoantennas. Nanoscale confinement of electromagnetic fields may introduce a longitudinal electric field component, giving rise to circularly polarized modes which are essential for diverse applications involving vapor and light, such as chirality and non-reciprocity. Hereby, we have designed, fabricated and characterized a miniaturized vapor cell that is integrated with optical waveguides that are designed to generate a peculiar circular-like polarization. Taking advantage of this phenomenon, we demonstrate a spectral shift in the atomic absorption signatures at varying magnetic fields, and significant isolation between forward and backward propagating waves in our atomic-cladded waveguide. Our results pave the way for the utilization of chip-scale integrated atomic devices in applications such as optical isolation and high spatial resolution magnetometry.

DOI
10.1364/optica.6.000015

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Alkali vapours, such as rubidium, are being used extensively in several important fields of research such as slow and stored light nonlinear optics quantum computation, atomic clocks and magnetometers. Recently, there is a growing effort towards miniaturizing traditional centimetre-size vapour cells. Owing to the significant reduction in device dimensions, light–matter interactions are greatly enhanced, enabling new functionalities due to the low power threshold needed for nonlinear interactions. Here, taking advantage of the mature platform of silicon photonics, we construct an efficient and flexible platform for tailored light–vapour interactions on a chip. Specifically, we demonstrate light–matter interactions in an atomic cladding waveguide, consisting of a silicon nitride nano-waveguide core with a rubidium vapour cladding. We observe the efficient interaction of the electromagnetic guided mode with the rubidium cladding and show that due to the high confinement of the optical mode, the rubidium absorption saturates at powers in the nanowatt regime. Alkali vapours are increasingly useful in photonic research and metrology applications, and they provide a useful test bed for investigating light–matter interaction. Stern et al. integrate silicon nitride waveguides with alkali vapours to study light–matter interactions on a chip-scale platform.
Abstract Optical magnetometers based on alkali vapors, such as rubidium, are among the most sensitive technologies for detecting and characterizing magnetic fields. Following the recent effort in miniaturizing atomic-based quantum technologies, the last years were marked by a growing interest in developing integrated quantum nanophotonic circuits for a vast range of applications. Motivated by the attractiveness of such chip-scale integration, we present and experimentally demonstrate an integrated magnetic sensing platform, based on a nanophotonic-chip interfaced to a microfabricated alkali vapor cell. Magnetically induced circular dichroism in rubidium vapor is measured using a planar structure that spatially resolves the handedness of incoming photons depending on their spin. The presented approach paves the way toward further integration of highly sensitive magnetometers, with potential for future applications, such as in high-spatial resolution magnetic vectorial imaging.
Following the efforts of size reduction and the integration of light and vapor systems, great promise is held in the integration of vapor and confined electromagnetic waves. By confining light to nanoscale dimensions, fundamental properties of light-vapor interactions may vary significantly. For example, the state of polarization may be modified as compared with weakly focused beams. Specifically, in transverse magnetic modes, the existence of a longitudinal field component, which is in quadrature to the transverse field, generates a "circular-like" polarized light. Here, by taking advantage of this very property, we study the interaction of confined light and vapor in a coupled system of plasmons and atomic vapors in the presence of magnetic fields. Our results show that the spectroscopic nature and Fano resonances of the hybrid plasmonic-atomic system are greatly altered. In parallel, we also exploit the existence of the atoms in proximity to the plasmonic mode to probe the polarization state of the electromagnetic field and reveal the longitudinal-to-transverse ratio between the plasmonic modes components in the near field. Interestingly, our system maps the amplitude and phase information of the electromagnetic modes to the spectral domain. As such, combining magnetic fields with the coupled plasmonic-atomic system has the potential for future applications in high spatial resolution magnetometry, near-field vectorial imaging, and magnetically induced switching and tuning.
Accurate and stable frequency sources can be realized by locking lasers to well-known transitions between energy levels in isolated quantum systems such as alkali atoms. Unfortunately, current implementations of such frequency standards typically involve bulky optical setups and discrete optical components. Furthermore, the common transitions of alkali atoms are in the near-infrared, hindering their use as frequency references in the telecom regime. Our current work is focused on mitigating these deficiencies. In particular, we demonstrate the design, fabrication, and experimental characterization of an on-chip telecom frequency reference that is based on a ladder transition of rubidium atoms integrated with nanoscale optical waveguides. These atomic cladded waveguides are implemented in a serpentine geometry in order to optimize the chip area and maximize the interaction of light with the alkali atoms. Following its fabrication, the device is used to stabilize a telecom laser around a 1.5 μm wavelength to a precision better than 200 kHz at ∼250 s. Moreover, in spite of the fact that the natural lifetime of the excited state of the atom corresponding to only a few megahertz line widths, the nanoscale confinement of the optical mode dictates ultrashort interaction times and extreme photonic energy densities allowing us to demonstrate low power and faster (∼200 MHz) all-optical modulation of a near-infrared light with a telecom light. The results presented in this paper push forward the efforts toward fully integrated chip-scale stabilization system and provide an extremely efficient link between atomic based devices and silicon photonics platform in the telecom.
Atom-light interactions in nano-scale systems hold great promise for novel technologies based on integrated emitters and optical modes. We present the design architecture, construction method, and characterization of an all-glass alkali-metal vapor cell with nanometer-scale internal structure. Our cell has a glue-free design which allows versatile optical access, in particular with high numerical aperture optics. By performing spectroscopy in different illumination and detection schemes, we investigate atomic densities and velocity distributions in various nanoscopic landscapes. We apply a two-photon excitation scheme to atoms confined in one dimension within our cells, achieving a resonance line-width of 32 MHz in a counter-propagating geometry, and 57.5 MHz in a co-propagating geometry. Both of these are considerably narrower than the Doppler width (GHz), and are limited by transit time broadening and velocity selection. We also demonstrate sub-Doppler line-widths for atoms confined in two dimensions to micron-sized channels. Furthermore, we illustrate control over vapor density within our cells through nano-scale confinement alone, which could offer a scalable route towards room-temperature devices with single atoms within an interaction volume. Our design offers a robust platform for miniaturized devices that could easily be combined with integrated photonic circuits.