Quantum polyspectra of up to fourth order are introduced for modeling and evaluating quantum transport measurements offering a powerful alternative to methods of the traditional full counting statistics. Experimental time traces of the occupation dynamics of a single quantum dot are evaluated via simultaneously fitting their second-, third-, and fourth-order spectra. The scheme recovers the same electron tunneling and spin relaxation rates as previously obtained from an analysis of the same data in terms of factorial cumulants of the full counting statistics and waiting-time distributions. Moreover, the evaluation of time traces via quantum polyspectra is demonstrated to be feasible also in the weak measurement regime even when quantum jumps can no longer be identified from time traces and methods related to the full counting statistics cease to be applicable. A numerical study of a double dot system shows strongly changing features in the quantum polyspectra for the transition from the weak measurement regime to the Zeno regime where coherent tunneling dynamics is suppressed. Quantum polyspectra thus constitute a general unifying approach to the strong and weak regime of quantum measurements with possible applications in diverse fields as nanoelectronics, circuit quantum electrodynamics, spin noise spectroscopy, or quantum optics.
Quantum polyspectra of up to fourth order are introduced for modeling and evaluating quantum transport measurements offering a powerful alternative to methods of the traditional full counting statistics. Experimental time traces of the occupation dynamics of a single quantum dot are evaluated via simultaneously fitting their second-, third-, and fourth-order spectra. The scheme recovers the same electron tunneling and spin relaxation rates as previously obtained from an analysis of the same data in terms of factorial cumulants of the full counting statistics and waiting-time distributions. Moreover, the evaluation of time traces via quantum polyspectra is demonstrated to be feasible also in the weak measurement regime even when quantum jumps can no longer be identified from time traces and methods related to the full counting statistics cease to be applicable. A numerical study of a double dot system shows strongly changing features in the quantum polyspectra for the transition from the weak measurement regime to the Zeno regime where coherent tunneling dynamics is suppressed. Quantum polyspectra thus constitute a general unifying approach to the strong and weak regime of quantum measurements with possible applications in diverse fields as nanoelectronics, circuit quantum electrodynamics, spin noise spectroscopy, or quantum optics.
The analysis of a continuous measurement record z(t) poses a fundamental challenge in quantum measurement theory. Different approaches were used in the past as records can, e.g., exhibit predominantly Gaussian noise, telegraph noise, or clicks at random times. The last case may appear as photon clicks in an optical spin-noise measurement at very low probe laser power. Here we show that such random-time quantum measurements can, similarly to the first two cases, be analyzed in terms of higher-order temporal correlations of the detector output z(t) and be related to the Liouvillian of the measured quantum system. Our analysis in terms of up to fourth-order spectra (quantum polyspectra) shows that this type of spectra reveals the same valuable information as previously studied higher-order spectra in the case of the usual continuous quantum measurements. Surprisingly, broadband system dynamics is revealed even for deliberately low average measurement rates. Many applications are envisioned in high-resolution spectroscopy, single-photon microscopy, circuit quantum electrodynamics, quantum sensing, and quantum measurements, in general.
We present general quantum mechanical expressions for higher-order moments, cumulants, and spectra of continuously measured quantum systems with applications in spin noise spectroscopy, quantum transport, and measurement theory in general. Starting from the so-called stochastic master equation of continuous measurement theory, we find that the leading orders of the fluctuating detector output z(t) with respect to the measurement strength $\ensuremath{\beta}$ are a white shot noise background, a constant measurement offset, and the leading order quantum noise of the measured operator A. Starting from quantum expressions for the multitime moments $\ensuremath{\langle}z({t}_{n})\ensuremath{\cdots}z({t}_{1})\ensuremath{\rangle}$ we derive three- and four-time cumulants that are valid in all orders of $\ensuremath{\beta}$ covering the full regime between the weak- and strong-measurement limit (Zeno limit). Intriguingly, quantum expressions for the cumulants were found that exhibit the same simple structure as those for the moments after introduction of only a slightly modified system propagator. Very compact expressions for the cumulant-based third- and fourth-order spectra (bispectrum and trispectrum) follow naturally. We illustrate the usefulness of higher-order spectra by treating a real-world two-spin system with strong hyperfine interaction. Moreover, spin noise spectroscopy is shown to have the potential for investigating the transition from weak measurements to the famous quantum Zeno regime for realistic probe laser intensities.
Precise environmental-noise characterisation in open quantum systems is a key step toward high-fidelity quantum control and targeted decoherence suppression in computing and sensing applications. Non-parametric quantum noise spectroscopy (QNS) provides a general-purpose, model-agnostic framework for estimating the spectral properties of an environment. The ability to perform such protocols under realistic constraints is key to their practical applicability. Notably, it is important to account for control constraints and understand how they limit the ability to learn about noise correlations as experiment-agnostic objects. We show how adopting a control-centric point of view allows one to recast the noise spectroscopy problem in such a way that (i) the central objects are now the time-ordered polyspectra, (ii) control filter functions are no longer encumbered by time-ordering. In particular, we show that this approach enables the seamless generalisation of frequency-comb QNS protocols to arbitrary control scenarios without introducing additional control symmetries that effectively remove time-ordering from filter functions, improving estimation in typically pathological scenarios. We demonstrate the targeted reconstruction of the time-ordered polyspectra across classical Gaussian and quantum non-Gaussian environments via simulations.
Random-time sampling of a quantum system is introduced as a new approach to continuous quantum measurements with prospects for ultra-low-perturbation measurements. Random sampling is, e.g., naturally realized in an optical spin noise experiment when weak probe-laser light exhibits random single-photon events in the detector. We show that a direct evaluation of these detector time-traces yields power spectra that are equivalent to those of the usual continuous measurement regime. Surprisingly, this holds true even for average sampling rates much lower than the typical frequency range of the measured quantum dynamics. The third-order quantum polyspectrum (bispectrum) also contains the same information as its continuous counterpart. Many applications of random-time sampling are envisioned for high-resolution spectroscopy, circuit quantum electrodynamics, quantum sensing, and quantum measurements in general.
A general theoretical formulation for the effect of a strong on-site Coulomb interaction on the time-dependent electron transport through a quantum dot under the influence of arbitrary time-varying bias voltages and/or external fields is presented, based on slave bosons and the Keldysh nonequilibrium Green's function (GF) techniques. To avoid the difficulties of computing double-time GFs, we generalize the propagation scheme recently developed by Croy and Saalmann to combine the auxiliary-mode expansion with the celebrated Lacroix's decoupling approximation in dealing with the second-order correlated GFs and then establish a closed set of coupled equations of motion, called second-order quantum rate equations (SOQREs), for an exact description of transient dynamics of electron correlated tunneling. We verify that the stationary solution of our SOQREs is able to correctly describe the Kondo effect on a qualitative level. Moreover, a comparison with other methods, such as the second-order von Neumann approach and Hubbard-I approximation, is performed. As illustrations, we investigate the transient current behaviors in response to a step voltage pulse and a harmonic driving voltage, and linear admittance as well, in the cotunneling regime.
The development of solid-state quantum technologies requires the understanding of quantum measurements in interacting, nonisolated quantum systems.In general, a permanent coupling of detectors to a quantum system leads to memory effects that have to be taken into account in interpreting the measurement results.In this thesis we develop a microscopic framework for correlations in non-Markovian weak measurements.A special point of interest are the different orders of quantum mechanical operators that appear naturally in such a scheme.First, we analyze a generic setup of two detectors coupled to a quantum system and derive a compact formula in the weak-measurement limit that interpolates between an instantaneous (text-book type) and almost continuous -detector dynamics-dependent -measurement.A quantum memory effect that we term system-mediated detector-detector interaction is crucial to observe noncommuting observables simultaneously.A response function of the observed system variables introduces an antisymmetric operator order to the total result.We propose a mesoscopic double-dot detector setup in which the memory effect is tunable and that can be used to explore the transition to non-Markovian quantum measurements experimentally.The response and noise functions which we find to describe the system-mediated detector-detector interaction are analyzed in detail.They are compared to the phenomenological "equilibrium order" approach for non-Markovian measurements which was introduced in Ref. [1].We give an overview of the broad spectrum of results beyond "equilibrium order" in the microscopic model in a compendium of different detectors and discuss general mathematical properties of the detector functions.As the quantum measurement problem is not banned from our theory by operation in the weak measurement limit, but deferred from the system of interest to the detectors, we comment on the influence of the detector readout procedure on the results.Finally, we combine the phenomenological proposal for nonsymmetrized correlations in quantum noninvasive measurements [1] and our microscopic derivation of the systemmediated detector-detector interaction of second order to investigate higher-order correlations of non-Markovian weak quantum measurements.The general third-order correlator is introduced and the underlying physical processes are identified and discussed.We find a more complex behavior than in second-order correlations with four types of system operator orders which we denote third cumulant, noise susceptibility I and II and second-order susceptibility.We introduce a convenient diagrammatic description which we illustrate by an example of measuring the third-order correlations of the tunnel current through a barrier.v I would like to express my deep gratitude to all the people who contributed to this thesis.Special thanks to my supervisor Wolfgang Belzig for offering me the opportunity to work in his research group, for the numerous helpful discussions in which I learned a lot and which gave impetus to this work again and again, for being always patient and an excellent guidance during my studies.I also wish to express great thanks to my other collaborators, Adam Bednorz, whose ideas are an important part of the foundation of this work and who was always ready to comment new results and bring things forward, and Christoph Bruder, who was a great help in thinking through results and formulating them in an understandable manner while preparing parts of this work for publication.Many thanks to Maxim Trushin, who was willing to discuss our weak measurement formalism with the example of a graphene coherence measurement, and who contributed the initial idea of a optical detection of pseudospin superposition states as well as the description of the carrier statistics using the Liouville-von Neumann equation and very important parts of the discussion of the results.In this context I also want to acknowledge valuable discussions with Daniele Brida about the optical detection scheme and with Bertrand Reulet about third-order current correlations.Finally, I wish to thank the current and former members of the Quantum Transport Group