Precise environmental-noise characterisation in open quantum systems is a key step toward high-fidelity quantum control and targeted decoherence suppression in computing and sensing applications. Non-parametric quantum noise spectroscopy (QNS) provides a general-purpose, model-agnostic framework for estimating the spectral properties of an environment. The ability to perform such protocols under realistic constraints is key to their practical applicability. Notably, it is important to account for control constraints and understand how they limit the ability to learn about noise correlations as experiment-agnostic objects. We show how adopting a control-centric point of view allows one to recast the noise spectroscopy problem in such a way that (i) the central objects are now the time-ordered polyspectra, (ii) control filter functions are no longer encumbered by time-ordering. In particular, we show that this approach enables the seamless generalisation of frequency-comb QNS protocols to arbitrary control scenarios without introducing additional control symmetries that effectively remove time-ordering from filter functions, improving estimation in typically pathological scenarios. We demonstrate the targeted reconstruction of the time-ordered polyspectra across classical Gaussian and quantum non-Gaussian environments via simulations.
Precise environmental-noise characterisation in open quantum systems is a key step toward high-fidelity quantum control and targeted decoherence suppression in computing and sensing applications. Non-parametric quantum noise spectroscopy (QNS) provides a general-purpose, model-agnostic framework for estimating the spectral properties of an environment. The ability to perform such protocols under realistic constraints is key to their practical applicability. Notably, it is important to account for control constraints and understand how they limit the ability to learn about noise correlations as experiment-agnostic objects. We show how adopting a control-centric point of view allows one to recast the noise spectroscopy problem in such a way that (i) the central objects are now the time-ordered polyspectra, (ii) control filter functions are no longer encumbered by time-ordering. In particular, we show that this approach enables the seamless generalisation of frequency-comb QNS protocols to arbitrary control scenarios without introducing additional control symmetries that effectively remove time-ordering from filter functions, improving estimation in typically pathological scenarios. We demonstrate the targeted reconstruction of the time-ordered polyspectra across classical Gaussian and quantum non-Gaussian environments via simulations.
We introduce open-loop quantum control protocols for characterizing the spectral properties of non-Gaussian noise, applicable to both classical and quantum dephasing environments. By engineering a multidimensional frequency comb via repetition of suitably designed pulse sequences, the desired high-order spectra may be related to observable properties of the qubit probe. We prove that access to a high time resolution is key to achieving spectral reconstruction over an extended bandwidth, overcoming the limitations of existing schemes. Non-Gaussian spectroscopy is demonstrated for a classical noise model describing quadratic dephasing at an optimal point, as well as a quantum spin-boson model out of equilibrium. In both cases, we obtain spectral reconstructions that accurately predict the qubit dynamics in the non-Gaussian regime.
We introduce multipulse quantum noise spectroscopy protocols for spectral estimation of the noise affecting multiple qubits coupled to Gaussian dephasing environments including both classical and quantum sources. Our protocols are capable of reconstructing all the noise auto- and cross-correlation spectra entering the multiqubit dynamics, providing access, in particular, to the asymmetric spectra associated with nonclassical environments. Our result relies on (i) an exact analytic solution for the reduced multiqubit dynamics that holds in the presence of an arbitrary Gaussian environment and dephasing-preserving control; (ii) the use of specific timing symmetries, which allow for a frequency comb to be engineered for all filter functions of interest, and for the spectra to be related to experimentally accessible observables. We show that quantum spectra have distinctive dynamical signatures, which we explore in two paradigmatic open-system models describing spin and charge qubits coupled to bosonic environments. Complete noise spectroscopy is demonstrated numerically in a realistic setting consisting of two-exciton qubits coupled to a phonon bath. The estimated spectra allow us to accurately predict the exciton dynamics as well as extract the temperature and spectral density of the quantum environment.
Qubit noise spectroscopy (QNS) is a valuable tool for both the characterization of a qubit's environment and as a precursor to more effective qubit control to improve qubit fidelities. Existing approaches to QNS are what the classical spectrum estimation literature would call "non-parametric" approaches, in that a series of probe sequences are used to estimate noise power at a set of points or bands. In contrast, model-based approaches to spectrum estimation assume additional structure in the form of the spectrum and leverage this for improved statistical accuracy or other capabilities, such as superresolution. Here, we derive model-based QNS approaches using inspiration from classical signal processing, primarily though the recently developed Schrodinger wave autoregressive moving-average (SchWARMA) formalism for modeling correlated noise. We show, through both simulation and experimental data, how these model-based QNS approaches maintain the statistical and computational benefits of their classical counterparts, resulting in powerful new estimation approaches. Beyond the direct application of these approaches to QNS and quantum sensing, we anticipate that the flexibility of the underlying models will find utility in adaptive feedback control for quantum systems, in analogy with their role in classical adaptive signal processing and control.
Quantum-enabled technologies promise advancements across a huge range of industrial, metrological and medical applications and are already demonstrating significant impacts, especially in the realm of sensing and metrology. While the extreme sensitivity of quantum systems to their environment is fueling those applications, it also represents a major hurdle to technologies which require long-term stability such as quantum computing and quantum simulations. In addition to the inherent decoherence phenomenon, the challenge associated with controlling a quantum system accurately and precisely, does in fact impede all of the aforementioned applications. Such techniques have therefore been subject to extensive research in both the academic and industrial sector and as a result, sophisticated quantum control techniques are emerging in order to understand, characterize and mitigate errors in quantum systems. This thesis presents how quantum control techniques can be employed to characterize and suppress both control imperfections and environmental noise in quantum systems, using experiments with trapped ions as a model quantum platform. We demonstrate two distinct but interrelated approaches that leverage either time-domain or frequency-domain information about the noise. In the first approach, we show how supervised learning algorithms can efficiently extract time-domain correlations from time-stamped sequences of projective measurements on a qubit. This information can then be used to perform real-time predictive control in which we autonomously pre-compensate anticipated qubit noise in order to stabilize the system. The second approach deploys provably optimal narrowband controls in order to characterize the specific spectral components of noise experienced by a qubit. Here, frequency-shifted Slepian functions permit reconstruction of system noise with maximum out-of-band rejection, and full spectrum reconstruction is enabled using techniques based on multitaper and Bayesian methods.
Resolving signals with closely spaced frequencies is central to applications in communications, spectroscopy and sensing. Recent results have shown that quantum sensing protocols can exhibit superresolution, the ability to discriminate between spectral lines with arbitrarily small frequency separation. Here, we revisit this problem from the perspective of quantum control theory, utilizing the filter function formalism to derive general, analytic conditions on quantum control protocols for achieving superresolution. Building on these conditions, we develop an optimal control framework, the utility of which is demonstrated through numerical identification of superresolution control protocols in the presence of realistic, experimentally-relevant constraints. We further extend our results to entangled initial states and assess their potential advantage. Our approach is broadly applicable to a wide variety of quantum sensing platforms, and it provides a systematic path to discover novel protocols that surpass conventional resolution limits in these systems.
Mitigating noise-induced decoherence is the central challenge in controlling open quantum systems. While existing robust protocols often require precise noise models, we introduce a universal framework for noise-agnostic quantum control that achieves high-fidelity operations without prior environmental noise characterization. This framework capitalizes on the dynamical modification of the system-environment coupling through control drives, an effect rigorously encoded in the dynamical equation. Since the derived noise sensitivity metric remains independent of the coupling details between the system and the environment, our protocol demonstrates robustness against arbitrary Markovian noises within the first-order weak coupling approximation. Numerical validation through quantum state transfer and gate operations reveals near-unity fidelity across diverse noise regimes, achieving orders-of-magnitude error suppression compared to target-only approaches. This framework bridges critical gaps between theoretical control design and experimental constraints, establishing a broadly applicable strategy for high-fidelity quantum information processing across platforms such as superconducting circuits, trapped ions, and solid-state qubits.