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arXiv:2109.05862 · Physical Review A

Random-time quantum measurements

Markus Sifft, D. Hägele

Published May 5, 2023• 9 citations
arXivHTMLPDF

Abstract

The analysis of a continuous measurement record $z(t)$ poses a fundamental challenge in quantum measurement theory. Different approaches were used in the past as records can, e.g., exhibit predominantly Gaussian noise, telegraph noise, or clicks at random times. The last case may appear as photon clicks in an optical spin-noise measurement at very low probe laser power. Here we show that such random-time quantum measurements can, similarly to the first two cases, be analyzed in terms of higher-order temporal correlations of the detector output $z(t)$ and be related to the Liouvillian of the measured quantum system. Our analysis in terms of up to fourth-order spectra (quantum polyspectra) shows that this type of spectra reveals the same valuable information as previously studied higher-order spectra in the case of the usual continuous quantum measurements. Surprisingly, broadband system dynamics is revealed even for deliberately low average measurement rates. Many applications are envisioned in high-resolution spectroscopy, single-photon microscopy, circuit quantum electrodynamics, quantum sensing, and quantum measurements, in general.

DOI
10.1103/physreva.107.052203

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The analysis of a continuous measurement record z(t)z(t)z(t) poses a fundamental challenge in quantum measurement theory. Different approaches were used in the past as records can, e.g., exhibit predominantly Gaussian noise, telegraph noise, or clicks at random times. The last case may appear as photon clicks in an optical spin-noise measurement at very low probe laser power. Here we show that such random-time quantum measurements can, similarly to the first two cases, be analyzed in terms of higher-order temporal correlations of the detector output z(t)z(t)z(t) and be related to the Liouvillian of the measured quantum system. Our analysis in terms of up to fourth-order spectra (quantum polyspectra) shows that this type of spectra reveals the same valuable information as previously studied higher-order spectra in the case of the usual continuous quantum measurements. Surprisingly, broadband system dynamics is revealed even for deliberately low average measurement rates. Many applications are envisioned in high-resolution spectroscopy, single-photon microscopy, circuit quantum electrodynamics, quantum sensing, and quantum measurements, in general.
Random-time sampling of a quantum system is introduced as a new approach to continuous quantum measurements with prospects for ultra-low-perturbation measurements. Random sampling is, e.g., naturally realized in an optical spin noise experiment when weak probe-laser light exhibits random single-photon events in the detector. We show that a direct evaluation of these detector time-traces yields power spectra that are equivalent to those of the usual continuous measurement regime. Surprisingly, this holds true even for average sampling rates much lower than the typical frequency range of the measured quantum dynamics. The third-order quantum polyspectrum (bispectrum) also contains the same information as its continuous counterpart. Many applications of random-time sampling are envisioned for high-resolution spectroscopy, circuit quantum electrodynamics, quantum sensing, and quantum measurements in general.
We present general quantum mechanical expressions for higher-order moments, cumulants, and spectra of continuously measured quantum systems with applications in spin noise spectroscopy, quantum transport, and measurement theory in general. Starting from the so-called stochastic master equation of continuous measurement theory, we find that the leading orders of the fluctuating detector output z(t)z(t)z(t) with respect to the measurement strength $\ensuremath{\beta}$ are a white shot noise background, a constant measurement offset, and the leading order quantum noise of the measured operator AAA. Starting from quantum expressions for the multitime moments $\ensuremath{\langle}z({t}_{n})\ensuremath{\cdots}z({t}_{1})\ensuremath{\rangle}$ we derive three- and four-time cumulants that are valid in all orders of $\ensuremath{\beta}$ covering the full regime between the weak- and strong-measurement limit (Zeno limit). Intriguingly, quantum expressions for the cumulants were found that exhibit the same simple structure as those for the moments after introduction of only a slightly modified system propagator. Very compact expressions for the cumulant-based third- and fourth-order spectra (bispectrum and trispectrum) follow naturally. We illustrate the usefulness of higher-order spectra by treating a real-world two-spin system with strong hyperfine interaction. Moreover, spin noise spectroscopy is shown to have the potential for investigating the transition from weak measurements to the famous quantum Zeno regime for realistic probe laser intensities.
The stochastic detector output z(t)z(t)z(t) of a general continuously measured quantum system is calculated using a stochastic master equation approach. The resulting continuous quantum noise formula (CQNF) is valid in all orders of the measurement strength. The CQNF provides a rigorous route to the calculation of higher order noise spectra of quantum systems with applications in spin noise spectroscopy and quantum measurement theory in general.
Classical time-resolved optical spectroscopy experiments are performed using sequences of ultrashort light pulses, with photon fluxes incident on the sample which are many orders of magnitude higher than real-world conditions corresponding to sunlight illumination. Here we overcome this paradigm by exploiting quantum correlations to perform time-resolved spectroscopy with entangled photons. Starting from spontaneous parametric down-conversion driven by a continuous-wave laser, we exploit the temporal entanglement between randomly generated signal/idler pairs to obtain temporal resolution, and their spectral entanglement to select the excitation frequency. We also add spectral resolution in detection, using a Fourier transform approach which employs a common-path interferometer. We demonstrate the potential of our entangled-photon streak camera by resolving, at the single-photon level, excitation energy transfer cascades from LH2 to LH1 in the photosynthetic membrane and disentangling the lifetimes of two dyes in a mixture. We show that time-resolved spectroscopy with quantum light can be performed without compromising measurement time, recording a fluorescence time trace in less than a minute even for samples with low quantum yield, which can be reduced to sub-second times with acceptable signal-to-noise ratio. Our results provide a new approach to ultrafast optical spectroscopy, where experiments are performed under conditions comparable to real-world sunlight illumination.
Quantum polyspectra of up to fourth order are introduced for modeling and evaluating quantum transport measurements offering a powerful alternative to methods of the traditional full counting statistics. Experimental time traces of the occupation dynamics of a single quantum dot are evaluated via simultaneously fitting their second-, third-, and fourth-order spectra. The scheme recovers the same electron tunneling and spin relaxation rates as previously obtained from an analysis of the same data in terms of factorial cumulants of the full counting statistics and waiting-time distributions. Moreover, the evaluation of time traces via quantum polyspectra is demonstrated to be feasible also in the weak measurement regime even when quantum jumps can no longer be identified from time traces and methods related to the full counting statistics cease to be applicable. A numerical study of a double dot system shows strongly changing features in the quantum polyspectra for the transition from the weak measurement regime to the Zeno regime where coherent tunneling dynamics is suppressed. Quantum polyspectra thus constitute a general unifying approach to the strong and weak regime of quantum measurements with possible applications in diverse fields as nanoelectronics, circuit quantum electrodynamics, spin noise spectroscopy, or quantum optics.
Classical time-resolved optical spectroscopy experiments are performed using sequences of ultrashort light pulses, with photon fluxes incident on the sample which are many orders of magnitude higher than real-world conditions corresponding to sunlight illumination. Spectroscopy and microscopy schemes that use quantum states of light have been widely described theoretically with fewer experimental demonstrations that typically require very long measurements that can extend for hours or more. Here, we show that time-resolved spectroscopy with quantum light can be performed without compromising measurement time or wavelength tunability, recording a fluorescence lifetime trace in biological samples in less than a second with acceptable signal-to-noise ratio. Starting from spontaneous parametric down-conversion driven by a continuous-wave laser, we exploit the temporal correlation between randomly generated signal/idler pairs to obtain temporal resolution, and their spectral correlation to select the excitation frequency. We also add spectral resolution in detection, using a 'photon-efficient' Fourier transform approach which employs a common-path interferometer. We demonstrate the potential of this approach by resolving, at the single-photon level, excitation energy transfer cascades from LH2 to LH1 in the photosynthetic membrane and disentangling the lifetimes of two dyes in a mixture. Our results provide a new approach to ultrafast optical spectroscopy, where experiments are performed under illumination intensity conditions comparable to real-world sunlight illumination.