Light beams offer many degrees of freedom to be explored in discrete and continuous domains. In addition to the possibility of entangling photons in these many degrees of freedom, it makes light a very useful and versatile tool for quantum information and quantum foundation purposes. In this thesis, we endorse its importance and versatility by presenting novel contributions that further explore both discrete and continuous degrees of freedom. It begins with two experiments that use classical light and explore its analogous behavior to quantum systems. The first one is a classical optics simulation of the dynamics of a relativistic quantum particle. The second work is related to the theory of mutually unbiased measurements that are effectively discrete but constructed from continuous variables systems. In the second part of the thesis, three works are presented that use the polarization and path discrete degrees of freedom. The first one is a redefinition of the quantum nonlocal correlation called steering in the multipartite scenario, based on an inconsistency in the previous definition, namely the creation of this correlation from scratch using operations that supposedly would not be able to do so. We call this exposure of quantum steering. Steering exposure is observed with entangled photons. The other two works are related to the experimental implementation of quantum channels of qubits, one of them is a particular channel for which we test for non-Markovianity using a operational measure called conditional past-future (CPF) correlation. The thesis finishes with a proposal for an experimental realization of any quantum channel of a single qubit, where the qubit is realized by the polarization of single photons. The functioning of all optical devices used is didactically explained.
Light beams offer many degrees of freedom to be explored in discrete and continuous domains. In addition to the possibility of entangling photons in these many degrees of freedom, it makes light a very useful and versatile tool for quantum information and quantum foundation purposes. In this thesis, we endorse its importance and versatility by presenting novel contributions that further explore both discrete and continuous degrees of freedom. It begins with two experiments that use classical light and explore its analogous behavior to quantum systems. The first one is a classical optics simulation of the dynamics of a relativistic quantum particle. The second work is related to the theory of mutually unbiased measurements that are effectively discrete but constructed from continuous variables systems. In the second part of the thesis, three works are presented that use the polarization and path discrete degrees of freedom. The first one is a redefinition of the quantum nonlocal correlation called steering in the multipartite scenario, based on an inconsistency in the previous definition, namely the creation of this correlation from scratch using operations that supposedly would not be able to do so. We call this exposure of quantum steering. Steering exposure is observed with entangled photons. The other two works are related to the experimental implementation of quantum channels of qubits, one of them is a particular channel for which we test for non-Markovianity using a operational measure called conditional past-future (CPF) correlation. The thesis finishes with a proposal for an experimental realization of any quantum channel of a single qubit, where the qubit is realized by the polarization of single photons. The functioning of all optical devices used is didactically explained.
We explore the concepts of coherence and entanglement as they apply to both the classical and quantum natures of light. In the classical domain, we take inspiration from the tools and concepts developed in foundational quantum mechanics and quantum information science to gain a better understanding of classical coherence theory of light with multiple degrees of freedom (DoFs). First, we use polarization and spatial parity DoFs to demonstrate the notion of classical entanglement, and show that Bell's measure can serve as a useful tool in distinguishing between classical optical coherence theory. Second, we establish a methodical yet versatile approach called 'optical coherency matrix tomography' for reconstructing the coherency matrix of an electromagnetic beam with multiple DoFs. This technique exploits the analogy between this problem in classical optics and that of tomographically reconstructing the density matrix associated with multipartite quantum states in quantum information science. Third, we report the first experimental measurements of the 4 x 4 coherency matrix associated with an electromagnetic beam in which polarization and a spatial DoF are relevant, ranging from the traditional two-point Young's double slit to spatial parity and orbital angular momentum modes. In the quantum domain, we use the modal structure of classical fields to develop qubits and structure Hilbert spaces for use in quantum information processing. Advancing to three-qubit logic gates is an important step towards the success of optical schemes for quantum computing. We experimentally implement a variety of two- and three- qubit, linear and deterministic, single-photon, controlled, quantum logic gates using polarization and spatial parity qubits. Lastly, we demonstrate the implementation of two-qubit single-photon logic using polarization and orbital angular momentum qubits.
The photon is a quantum system that is by nature robust against noise, and fast travelling, providing an ideal information carrier for quantum information science. The field of quantum information science has generated a great deal of interest for both researchers and the public due to the advantages it can have over classical technologies in areas including communication, computing and cryptography. In this thesis, I explore several different ways that photons can be used to realize quantum information advantages and enable quantum technologies, information tasks and fundamental studies of physics. A strong emphasis is placed on their practical implementation in optical experiments, where the challenges of noise, loss and device imperfections must be considered and combated. I utilize spontaneous parametric downconversion-based sources of high-quality single photons, and their polarization, path, and temporal degrees of freedom for encoding quantum information. In my first experimental project, I demonstrate the first violation of noncontextuality with time-polarization intraparticle entangled states encoded in a single photon by implementing a powerful interference-based measurement technique for photonic states. I perform a test of noncontextuality, acquiring a parameter |SCHSH| = 2.744 ± 0.006, which violates the classical bound of 2 by over 110 standard deviations, rigorously certifying both entanglement and contextuality of the system. We propose a new approach for preparing and measuring high-dimensional time-bin states, that overcomes many of the limitations of previous techniques, and demonstrate it for time-bin qubits and qutrits. In the next experimental project, I investigate the topic of universal cloning in quantum steering-with cloning and steering being two fundamental aspects of quantum physics deeply involved in the security of quantum protocols. I report the first experimental demonstration of cloned quantum steering, showing a simultaneous violation in a steering test by two clones made from one part of an entangled pair of photons. This provides a conclusive result on the question of whether the cloning of quantum steering is possible. We also present theoretical results that clarify our understanding of cloned steering for qubits: we find a no-go theorem where quantum steering can only be copied by a qubit universal cloning machine for 2 and 3 clones, and a monogamy relation where for N clones, steering is only possible if a minimum of N + 1 measurements are performed on each clone. I discuss the field of random number generation, and study how quantum physics allows for certifiably unpredictable random sequences, without needing complete trust in all of the physical devices, offering high levels of security over classical approaches. I report the first discrete-variable detection-loophole-free implementation of one-sided device-independent randomness expansion of certified random bits, based on the quantum steering task. These results illustrate an approach to secure randomness with greater tolerance to noise and loss compared to Bell test-based protocols. The final experimental project looks at quantum autoencoders, which are a quantum machine learning tool that we investigate for the purpose of denoising quantum states. I model and simulate a denoising quantum autoencoder which compresses ququarts into a qubit space and reconstructs noise-reduced ququart states. I construct an experimental apparatus that implements this device, and demonstrate quantum state tomography of ququart states, and the training of the autoencoder.
Quantum information can be processed in two fundamentally different ways, using either discrete or continuous variable implementations. Each one of them provides different practical advantages and drawbacks. In this thesis we study theoretical means allowing to implement quantum information protocols originally formulated for discrete quantum systems in physical objects characterized by continuous variables. At the heart of our considerations is the use of modular variables as helpful technique to reveal discrete structure in continuous-variable states, operations and observables. The present work is strongly guided by the experimental applicability of our ideas in quantum optics experiments, with a particular focus on the transverse degrees of freedom of single photons.One of the main themes of this thesis is the formulation of a framework for quantum information processing in phase-space based on the use of modular variables. The term modular variables refers to a specific class of observables that are periodic with respect to some pair of conjugate variables. In our framework we use these periodic observables in order to encode discrete quantum information in Hilbert spaces of infinite dimension. In particular, we consider protocols that involve measurements of judiciously chosen logical observables enabling the readout of the encoded discrete quantum information from the corresponding logical states. Using this framework we show how to perform tests of fundamental properties of quantum mechanics, such as entanglement, Bell nonlocality and contextuality, in Hilbert spaces of various dimensions. Particularly, we generalize known tests of each of these properties, that were originally formulated for measurements with discrete outcomes, to more general measurement contexts comprising the case of bounded continuous outcomes. Concerning experimental implementations of the presented theoretical elaborations we discuss the transverse degrees of freedom of single photons as a natural platform to manipulate and measure modular variables. In particular, we demonstrate how to process discrete quantum information encoded in the spatial distribution of single photons via the optical Talbot effect - a near-field interference effect. Finally, we show how to produce d-dimensional entangled Talbot photon pairs without post-selection, using spontaneous parametric down-conversion and linear optical elements only. As last topic we explore the nonlocal properties of a specific class of hybrid entanglement between particle-like and wave-like optical qubits. Using a hybrid measurement scheme of Pauli and displaced parity measurements we show that, even after including realistic experimental losses, a violation of local-realism is theoretically possible.
This thesis fathoms the possibilities and limitations of measurements in quantum optics. After a short introduction to the general aspects of measurements in quantum mechanics, it presents three examples of a measurement process in concrete applications to quantum optics. For one, while operators describing quantities of interest might have a simple theoretical form, it is often hard to actually implement a measurement of their expectation values experimentally. This situation is encountered in the first part which is devoted to the measurement of quantum statistical properties of a light beam. In contrast to classical optics, these statistics are not fully determined by first- and second-order correlations. Instead, higher-order correlations, usually described by non-Hermitian operators, are necessary to characterize the quantum state completely. A particular example is the N-photon Fock state, for which only a measurement of the Nth-order correlations allows for a full characterization. Here, we present a new method how to measure an important class of Nth-order correlations for arbitrary N in a single spatial mode with two polarizations with limited experimental resources. The second part is again centered around the realization of specific measurement operators for photon correlation measurements. However, in contrast to the previous chapter, these measurements are not an end in their own, but are designed to create specific quantum states as a consequence of the measurement process: A suitable measurement of photons emitted by a number of atoms allows to transfer the atoms into long-lived entangled states. We find that with this method it is possible to entangle two remote atomic qubits to an arbitrary and well-defined degree. Furthermore, we show how to generate two families of quantum states in an arbitrary number of remote atomic qubits: one family consists of all -- symmetric and non-symmetric -- total angular momentum eigenstates in N remote qubits, the other is a family of cluster states. It is also systematically investigated whether the technique of quantum state engineering by projective measurements allows for the creation of any arbitrary state. We find explicit solutions for the case of two and three qubits, while it is shown that no solution exist for N > 6. We conclude the section by proving that with some changes in the setup, this measurement-based quantum state engineering technique allows to create the same states among the scattered photons themselves rather than among the emitting atoms. The last part is devoted to the amount of information one is able to gain about a given system when performing a measurement. The corresponding limits of information are investigated at the example of the duality that arises in a two-way interferometer between the visibility of the interference pattern and the knowledge about the path of the interfering object. We show that there exist correlations between the phase difference the interfering object acquires on its way through the interferometer and the amount of which-way information retrievable from certain observables of the which-way detector. In this way, the which-way information becomes a phase-dependent quantity. In particular, we find that for certain values of the phase shift, the amount of extractable which-way information can be larger than allowed by phase-independent measurement. This property is put to use to find the optimal observable for the which-way detector readout in dependence on the phase of the interfering object. Following this strategy, we are able to gain more which-way information than previously thought possible.
In the case of mixed states ρAB of the composite system A ⊗ B, the previous relation generalizes to ρAB = ∑ k pkρ A k ⊗ρk , where pk are probabilities and ρk ’s (ρk ’s) are generic density matrix of the system A (B). The entanglement derives from “subtle” nonlocal correlations between the parts of a quantum system and combines three basic structural elements of quantum theory: the superposition principle, the quantum non-separability property and the exponential scaling of the state space with the number of partitions. This unique resource can be used to perform computational and cryptographic tasks otherwise impossible with classical systems. An entangled state shared by two or more separated parties is a valuable resource for fundamental quantum protocols, such as quantum teleportation [2], quantum computing [3] and quantum cryptography. By using entangled states we can deeply investigate the nonlocal properties of the quantum world. In fact, an entangled system exhibits correlations between two (or more) parties, which cannot be reproduced by a classical theory or, in general, by a Local Hidden Variables Theory (LHVT). Quantum optics represents an excellent experimental test bench for various novel concepts introduced within the framework of quantum information theory. Quantum states of photons, generally produced by a probabilistic process, namely spontaneous parametric down conversion (SPDC), may be easily and accurately manipulated using linear and nonlinear optical devices and measured by efficient single-photon detectors. Photonic qubits represent the typical carrier of quantum information and can be distributed over long distances, either in free-space or in low-loss optical fibers. Two-particle experiments correspond to operate with qubits belonging to a (2 × 2) Hilbert space. Many quantum information tasks and fundamental tests of quantum mechanics, such as the simulation of properties of quantum systems, the realization of quantum algorithms of increasing complexity and the investigation of the quantum world at a mesoscopic level, deal with a large number of qubits. In order to take full advantage of the possibilities offered by quantum mechanics, more qubits must be added to a quantum state. Two approaches may be followed to increase the number of qubits. The first one consists of increasing the number of entangled particles. In this way, multi-qubit entangled states are created by distributing the qubits between the particles so that each particle carries one qubit. A second strategy consists of encoding more than one qubit in each particle, by exploiting different degrees of freedom (DOFs) of the photon such as the polarization, the path, the emission time, the orbital angular momentum. This has been used to create two-photon fourand six-qubit states and up to five-photon ten-qubit graph states. The entanglement of two particles in different DOFs corresponds to socalled hyperentanglement. It is worth noting that multi-qubit hyperentanglement allows to achieve higher
Quantum information science explores the foundational aspects of quantum mechanics and its ombination with information science for new information technologies. The underlying key resource is non-classical correlations. These counter-intuitive correlations between quantum systems can be used for encoding, transmitting and measuring information in quantum information tasks. Although quantum properties can be used in a variety of systems, here we explore photons. These information carriers are fast, easy to generate and manipulate and only interact weakly with the environment. These properties make them to excellent candidates to be employed in experiments. Developing quantum technology, such as single photon sources and single photon detectors, allows us to investigate the foundational aspects of quantum mechanics in quantum information tasks. These tasks use non-classical correlations, which form a hierarchy, from Bell nonlocality to Einstein-Podolsky-Rosen (EPR) steering to quantum nonseparability. Two systems are nonlocally correlated, when measuring one system affects the measurement results on the other system, hence the name `steering. In test for non-classical correlations, we share a quantum state between two observers which are trusted or untrusted. While observers are both untrusted or trusted in entanglement witness tests and Bell inequality violations, respectively, EPR-steering is distinct from these two classes by its fundamental asymmetry: one party is trusted while the other is untrusted.