Spontaneous decay of a single photon is a notoriously inefficient process in nature irrespective of the frequency range. We report that a quantum phase-slip fluctuation in high-impedance superconducting waveguides can split a single incident microwave photon into a large number of lower-energy photons with a near unit probability. The underlying inelastic photon-photon interaction has no analogs in nonlinear optics. Instead, the measured decay rates are explained without adjustable parameters in the framework of a new model of a quantum impurity in a Luttinger liquid. Our result connects circuit quantum electrodynamics to critical phenomena in two-dimensional boundary quantum field theories, important in the physics of strongly correlated systems. The photon lifetime data represent a rare example of verified and useful quantum many-body simulation.
Spontaneous decay of a single photon is a notoriously inefficient process in nature irrespective of the frequency range. We report that a quantum phase-slip fluctuation in high-impedance superconducting waveguides can split a single incident microwave photon into a large number of lower-energy photons with a near unit probability. The underlying inelastic photon-photon interaction has no analogs in nonlinear optics. Instead, the measured decay rates are explained without adjustable parameters in the framework of a new model of a quantum impurity in a Luttinger liquid. Our result connects circuit quantum electrodynamics to critical phenomena in two-dimensional boundary quantum field theories, important in the physics of strongly correlated systems. The photon lifetime data represent a rare example of verified and useful quantum many-body simulation.
Light does not typically scatter light, as witnessed by the linearity of Maxwell’s equations. In this work, we demonstrate two superconducting circuits, in which microwave photons have well-defined energy and momentum, but their lifetime is finite due to decay into lower energy photons. The circuits we present are formed with Josephson junction arrays where strong quantum phase-slip fluctuations are present either in all of the junctions or in only a single junction. The quantum phase-slip fluctuations are shown to result in the strong inelastic photon-photon interaction observed in both circuits. The phenomenon of a single photon decay provides a new way to study multiple long-standing many-body problems important for condensed matter physics. The examples of such problems, which we cover in this work include superconductor to insulator quantum phase transition in one dimension and a general quantum impurity problem. The photon lifetime data can be treated as a rare example of a verified and useful quantum many-body simulation.
A hallmark of integrable systems is the purely elastic scattering of their excitations. Such systems possess an extensive number of locally conserved charges, leading to the conservation of the number of scattered excitations, as well as their set of individual momenta. In this work, we show that inelastic decay can nevertheless be observed in circuit-QED realizations of integrable boundary models. We consider the scattering of microwave photons off impurities in superconducting circuits implementing the boundary sine-Gordon and Kondo models, which are both integrable. We show that not only is inelastic decay possible for the microwave photons, in spite of integrability, and due to a nonlinear relation between them and the elastically scattered excitations, but also that integrability in fact provides powerful analytical tools allowing us to obtain exact expressions for response functions describing the inelastic decay. Using the framework of form factors, we calculate the total inelastic decay rate and elastic phase shift of the microwave photons, extracted from a two-point response function. We then go beyond linear response and obtain the exact energy-resolved inelastic decay spectrum, using a novel method to evaluate form-factor expansions of three-point response functions, which could prove useful in other applications of integrable quantum field theories. Our results could be relevant to several recent photon-splitting experiments and, in particular, to recent experimental works that provide evidence for the elusive Schmid-Bulgadaev dissipative quantum phase transition. Published by the American Physical Society 2024
Instantons, spacetime-localized quantum field tunneling events, are ubiquitous in correlated condensed matter and high-energy systems. However, their direct observation through collisions with conventional particles has not been considered possible. We show how recent advances in circuit quantum electrodynamics, specifically, the realization of galvanic coupling of a transmon qubit to a high-impedance transmission line, allows the observation of inelastic collisions of single microwave photons with instantons (phase slips). We develop a formalism for calculating the photon-instanton cross section, which should be useful in other quantum field theoretical contexts. In particular, we show that the inelastic scattering probability can significantly exceed the effect of conventional Josephson quartic anharmonicity and reach order-unity values.
Instantons, semiclassical trajectories of quantum tunneling in imaginary time, have long been used to study thermodynamic and transport properties in a myriad of condensed matter and high-energy systems. A recent experiment in superconducting circuits [R. Kuzmin et al., Phys. Rev. Lett. 126, 197701 (2021)] provided first evidence for direct dynamical signatures of instantons (phase slips), manifested by order-unity inelastic decay probabilities for photons with which they interact, motivating the development of a scattering theory of instantons [A. Burshtein et al., Phys. Rev. Lett. 126, 137701 (2021)]. While this framework successfully predicted the measured inelastic decay rates of the photons for several experimental devices, it is valid only if the tunneling time of the instantons is much shorter than the relaxation time due to the environment in which they are embedded, and requires a closed analytical expression for the instanton trajectory. Here, we alleviate these restrictions by incorporating numerical methods that eliminate some of the previously applied approximations. Our results improve the agreement with the experimental measurements, also for devices with lower impedances and thus shorter relaxation times, without fitting parameters. This framework should be useful in many other quantum field theoretical contexts.
Inducing interactions between individual photons is key for photonic quantum information and studying many-body photon states. Superconducting circuits are well suited to combine strong interactions with low losses. Typically, microwave photons are stored in an LC oscillator shunted by a Josephson junction, where the zero-point phase fluctuations across the junction determine the strength and order of photon interactions. Most superconducting nonlinear oscillators operate with small phase fluctuations, where two-photon Kerr interactions dominate. In our experiment, we shunt a high-impedance LC oscillator with a dipole element favoring the tunneling of paired Cooper pairs. This leads to large phase fluctuations of 3.4, accessing a regime where transition frequencies shift non-monotonically with excitation number. From spectroscopy, we extract two-, three-, and four-photon interaction energies, all of similar strength and exceeding the photon loss rate. Our results open a new regime of high-order photon interactions in microwave quantum optics. In superconducting circuits, the nonlinearity of Josephson junctions mediates photon interactions, but they are typically dominated by two-photon processes. Here the authors observe multi-photon interactions in a superconducting circuit with Cooper-pair pairing, revealing a new regime of microwave quantum optics.
We study spontaneous photon decay into multiple photons triggered by strong nonlinearities in an experimental simulator of a bosonic quantum impurity model. Previously, spectroscopic signatures of photon conversion were reported and evidenced as resonances in the many-body spectrum of these systems. Here, we report on the observation of multimode fluorescence of a small Josephson junction embedded in a high impedance superconducting transmission line. Measurement of the down-converted photons is achieved using state-of-the-art broadband parametric amplifiers. Photon triplet emission is explicitly demonstrated at a given frequency as the counterpart of inelastic photon decay at 3× the emission frequency. These results open exciting prospects for the burgeoning field of many-body quantum optics and offer a direct signature of the ultrastrong light-matter coupling.