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arXiv:2405.00411 · Physical Review Letters

Direct Detection of Down-Converted Photons Spontaneously Produced at a Single Josephson Junction

Dorian Fraudet, Izak Snyman, D. M. Basko, Sébastien Leger, Théo Sépulcre, Arpit Ranadive, Gwenael Le Gal, Alba Torras-Coloma, Wiebke Guichard, Serge Florens, Nicolas Roch

Published Jan 9, 2025• 11 citations
arXivHTMLPDF

Abstract

We study spontaneous photon decay into multiple photons triggered by strong nonlinearities in an experimental simulator of a bosonic quantum impurity model. Previously, spectroscopic signatures of photon conversion were reported and evidenced as resonances in the many-body spectrum of these systems. Here, we report on the observation of multimode fluorescence of a small Josephson junction embedded in a high impedance superconducting transmission line. Measurement of the down-converted photons is achieved using state-of-the-art broadband parametric amplifiers. Photon triplet emission is explicitly demonstrated at a given frequency as the counterpart of inelastic photon decay at 3× the emission frequency. These results open exciting prospects for the burgeoning field of many-body quantum optics and offer a direct signature of the ultrastrong light-matter coupling.

DOI
10.1103/physrevlett.134.013804

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We study spontaneous photon decay into multiple photons triggered by strong nonlinearities in an experimental simulator of a bosonic quantum impurity model. Previously, spectroscopic signatures of photon conversion were reported and evidenced as resonances in the many-body spectrum of these systems. Here, we report on the observation of multimode fluorescence of a small Josephson junction embedded in a high impedance superconducting transmission line. Measurement of the down-converted photons is achieved using state-of-the-art broadband parametric amplifiers. Photon triplet emission is explicitly demonstrated at a given frequency as the counterpart of inelastic photon decay at 3× the emission frequency. These results open exciting prospects for the burgeoning field of many-body quantum optics and offer a direct signature of the ultrastrong light-matter coupling.
Abstract The interaction between light and matter remains a central topic in modern physics despite decades of intensive research. Coupling an isolated emitter to a single mode of the electromagnetic field is now routinely achieved in the laboratory, and standard quantum optics provides a complete toolbox for describing such a setup. Current efforts aim to go further and explore the coherent dynamics of systems containing an emitter coupled to several electromagnetic degrees of freedom. Recently, ultrastrong coupling to a transmission line has been achieved where the emitter resonance broadens to a significant fraction of its frequency, and hybridizes with a continuum of electromagnetic (EM) modes. In this work we gain significantly improved control over this regime. We do so by combining the simplicity and robustness of a transmon qubit and a bespoke EM environment with a high density of discrete modes, hosted inside a superconducting metamaterial. This produces a unique device in which the hybridisation between the qubit and many modes (up to ten in the current device) of its environment can be monitored directly. Moreover the frequency and broadening of the qubit resonance can be tuned independently of each other in situ. We experimentally demonstrate that our device combines this tunability with ultrastrong coupling and a qubit nonlinearity comparable to the other relevant energy scales in the system. We also develop a quantitative theoretical description that does not contain any phenomenological parameters and that accurately takes into account vacuum fluctuations of our large scale quantum circuit in the regime of ultrastrong coupling and intermediate non-linearity. The demonstration of this new platform combined with a quantitative modelling brings closer the prospect of experimentally studying many-body effects in quantum optics. A limitation of the current device is the intermediate nonlinearity of the qubit. Pushing it further will induce fully developed many-body effects, such as a giant Lamb shift or nonclassical states of multimode optical fields. Observing such effects would establish interesting links between quantum optics and the physics of quantum impurities
We present the Josephson junction intersected superconducting transmission line resonator. In contrast to the Josephson parametric amplifier, Josephson bifurcation amplifier and Josephson parametric converter we consider the regime of few microwave photons. We review the derivation of eigenmode frequencies and zero point fluctuations of the nonlinear transmission line resonator and the derivation of the eigenmode Kerr nonlinearities. Remarkably these nonlinearities can reach values comparable to Transmon qubits rendering the device ideal for accessing the strongly correlated regime. This is particularly interesting for investigation of quantum many-body dynamics of interacting particles under the influence of drive and dissipation. We provide current profiles for the device modes and investigate the coupling between resonators in a network of nonlinear transmission line resonators.
Multiphoton emitters are a sought-after resource in quantum photonics. Nonlinear interactions between a multilevel atomic system and a coherent drive can lead to resonant two-photon emission, but harvesting light from this process has remained a challenge due to the small oscillator strengths involved. Here we present a study of two-photon resonance fluorescence at microwave frequencies, using a superconducting, ladder-type artificial atom, a transmon, strongly coupled to a waveguide. We drive the two-photon transition between the ground and second-excited states at increasingly high powers and observe a resonance fluorescence peak whose intensity becomes comparable to single-photon emission until it splits into a Mollow-like triplet. We measure photon correlations of frequency-filtered spectral lines and find that while emission at the fundamental frequency stays antibunched, the resonance fluorescence peak at the two-photon transition is superbunched. Our results provide a route towards the realization of multiphoton sources in the microwave domain.
Electromagnetic fields possess zero point fluctuations which lead to observable effects such as the Lamb shift and the Casimir effect. In the traditional quantum optics domain, these corrections remain perturbative due to the smallness of the fine structure constant. To provide a direct observation of non-perturbative effects driven by zero point fluctuations in an open quantum system we wire a highly non-linear Josephson junction to a high impedance transmission line, allowing large phase fluctuations across the junction. Consequently, the resonance of the former acquires a relative frequency shift that is orders of magnitude larger than for natural atoms. Detailed modeling confirms that this renormalization is non-linear and quantum. Remarkably, the junction transfers its non-linearity to about thirty environmental modes, a striking back-action effect that transcends the standard Caldeira-Leggett paradigm. This work opens many exciting prospects for longstanding quests such as the tailoring of many-body Hamiltonians in the strongly non-linear regime, the observation of Bloch oscillations, or the development of high-impedance qubits.
We investigate electromagnetic radiation emitted by a small voltage-biased Josephson junction connected to a superconducting transmission line. At frequencies below the well-known emission peak at the Josephson frequency (2eV/h), extra radiation is triggered by quantum fluctuations in the transmission line. For weak tunneling couplings and typical Ohmic transmission lines, the corresponding photon-flux spectrum is symmetric around half the Josephson frequency, indicating that the photons are predominately created in pairs. By establishing an input-output formalism for the microwave field in the transmission line, we give further evidence for this nonclassical photon pair production, demonstrating that it violates the classical Cauchy-Schwarz inequality for two-mode flux cross correlations. In connection to recent experiments, we also consider a stepped transmission line, where resonances increase the signal-to-noise ratio.
The realization of strong nonlinear coupling between single photons has been a long-standing goal in quantum optics and quantum information science, promising wide impact applications, such as all-optical deterministic quantum logic and single-photon frequency conversion. Here, we report an experimental observation of the strong coupling between a single-photon and a two-photon Fock state in an ultrastrongly-coupled circuit-QED system. This strong nonlinear interaction is realized by introducing a detuned flux qubit working as an effective coupler between two modes of a superconducting coplanar waveguide resonator. The ultrastrong light–matter interaction breaks the excitation number conservation, and an external flux bias breaks the parity conservation. The combined effect of the two enables the strong one–two-photon coupling. Quantum Rabi-like avoided crossing is resolved when tuning the two-photon resonance frequency of the first mode across the single-photon resonance frequency of the second mode. Within this new photonic regime, we observe the thresholdless second harmonic generation for a mean photon number below one. Our results represent a key step towards a new regime of quantum nonlinear optics, where individual photons can deterministically and coherently interact with each other in the absence of any stimulating fields. Systems with strong photon-photon interactions enable advanced quantum optical applications as well as the study of highly correlated light-matter states. Here the authors report strong coupling between single- and two-photon states in a superconducting circuit, enabling a new regime of nonlinear quantum optics.