Instantons, spacetime-localized quantum field tunneling events, are ubiquitous in correlated condensed matter and high-energy systems. However, their direct observation through collisions with conventional particles has not been considered possible. We show how recent advances in circuit quantum electrodynamics, specifically, the realization of galvanic coupling of a transmon qubit to a high-impedance transmission line, allows the observation of inelastic collisions of single microwave photons with instantons (phase slips). We develop a formalism for calculating the photon-instanton cross section, which should be useful in other quantum field theoretical contexts. In particular, we show that the inelastic scattering probability can significantly exceed the effect of conventional Josephson quartic anharmonicity and reach order-unity values.
Instantons, spacetime-localized quantum field tunneling events, are ubiquitous in correlated condensed matter and high-energy systems. However, their direct observation through collisions with conventional particles has not been considered possible. We show how recent advances in circuit quantum electrodynamics, specifically, the realization of galvanic coupling of a transmon qubit to a high-impedance transmission line, allows the observation of inelastic collisions of single microwave photons with instantons (phase slips). We develop a formalism for calculating the photon-instanton cross section, which should be useful in other quantum field theoretical contexts. In particular, we show that the inelastic scattering probability can significantly exceed the effect of conventional Josephson quartic anharmonicity and reach order-unity values.
Instantons, semiclassical trajectories of quantum tunneling in imaginary time, have long been used to study thermodynamic and transport properties in a myriad of condensed matter and high-energy systems. A recent experiment in superconducting circuits [R. Kuzmin et al., Phys. Rev. Lett. 126, 197701 (2021)] provided first evidence for direct dynamical signatures of instantons (phase slips), manifested by order-unity inelastic decay probabilities for photons with which they interact, motivating the development of a scattering theory of instantons [A. Burshtein et al., Phys. Rev. Lett. 126, 137701 (2021)]. While this framework successfully predicted the measured inelastic decay rates of the photons for several experimental devices, it is valid only if the tunneling time of the instantons is much shorter than the relaxation time due to the environment in which they are embedded, and requires a closed analytical expression for the instanton trajectory. Here, we alleviate these restrictions by incorporating numerical methods that eliminate some of the previously applied approximations. Our results improve the agreement with the experimental measurements, also for devices with lower impedances and thus shorter relaxation times, without fitting parameters. This framework should be useful in many other quantum field theoretical contexts.
Spontaneous decay of a single photon is a notoriously inefficient process in nature irrespective of the frequency range. We report that a quantum phase-slip fluctuation in high-impedance superconducting waveguides can split a single incident microwave photon into a large number of lower-energy photons with a near unit probability. The underlying inelastic photon-photon interaction has no analogs in nonlinear optics. Instead, the measured decay rates are explained without adjustable parameters in the framework of a new model of a quantum impurity in a Luttinger liquid. Our result connects circuit quantum electrodynamics to critical phenomena in two-dimensional boundary quantum field theories, important in the physics of strongly correlated systems. The photon lifetime data represent a rare example of verified and useful quantum many-body simulation.
We address recent advances in quantum optics with propagating microwaves\nin superconducting circuits. This research field exploits on the fact that the coupling between a superconducting artificial atom and propagating microwave photons in a one-dimensional (1D) open transmission line can be made strong enough to observe quantum effects, without using any cavity to confine the microwave photons.\nWe embed an artificial atom, a superconducting transmon qubit, in a 1D open\ntransmission line and investigate the scattering properties of coherent microwaves. When an input coherent state, with an average photon number much less than 1, is on resonance with the artificial atom, we observe extinction of up to 99% in the forward propagating field. We observe the strong nonlinearity of the artificial atom and under strong driving we observe the Mollow triplet. We also study the statistics of the reflected and transmitted beams, which are predicted to be nonclassical states. In particular, we demonstrate photon antibunching in the reflected beam by measuring the second-order correlation function. By applying a second control tone, we observe the Autler-Townes splitting and a giant cross-Kerr effect.\nFurthermore, we demonstrate fast operation of a single-photon router using\nthe Autler-Townes splitting. This device provides important steps towards the realization of a quantum network. This thesis describes the motivation, theoretical background, design, implementation and measurement results.
Light does not typically scatter light, as witnessed by the linearity of Maxwell’s equations. In this work, we demonstrate two superconducting circuits, in which microwave photons have well-defined energy and momentum, but their lifetime is finite due to decay into lower energy photons. The circuits we present are formed with Josephson junction arrays where strong quantum phase-slip fluctuations are present either in all of the junctions or in only a single junction. The quantum phase-slip fluctuations are shown to result in the strong inelastic photon-photon interaction observed in both circuits. The phenomenon of a single photon decay provides a new way to study multiple long-standing many-body problems important for condensed matter physics. The examples of such problems, which we cover in this work include superconductor to insulator quantum phase transition in one dimension and a general quantum impurity problem. The photon lifetime data can be treated as a rare example of a verified and useful quantum many-body simulation.
In the last decade, the field of Quantum Optics has been enriched with a completely new platform: superconducting quantum circuits, also known as circuit-QED. This platform builds on the original designs of superconducting qubits, that is few-level systems made of superconducting islands and Josephson junctions, but adds to it a new ingredient, microwave photons. In this talk I will review circuit-QED with a focus on two complementary lines of research: ultrastrong light-matter coupling and strongly correlated propagating photons. The first topic deals with novel designs of superconducting qubits, engineering their coupling to the microwave radiation field to reach Rabi frequencies that approach the qubit and photon frequencies. In this regime, known as ”ultrastrong coupling”, the rotating wave approximation from Quantum Optics is no longer valid, the vacuum may spontaneously polarize, producing photons that get bound to the qubit, and novel physics is expected to emerge. I will review recent experiments on this topic, together with various theoretical proposals to tame this ultrastrong coupling. The second topic revolves around the notion of ”propagating” photons in these circuits. Most experiments in circuit-QED so far adopted the typical configuration of artificial atoms (qubits) interacting with artificial cavities (LC resonators). This proved useful in order to reach the strong coupling regime, demonstrating Rabi oscillations and developing a variety of protocols for quantum information, tomograhy, entanglement, etc. However, recent experiments have shown that it is possible to also work with propagating photons, replacing the LC resonators with open transmission lines, and studying the scattering properties of those artificial atoms. In this context we have worked on developing new technology to detect and control these photons, engineering single-photon detectors, quantum metamaterials and photonic crystals, or even new nonlinear media based on coupled cavities.
Waveguide circuit quantum electrodynamics (waveguide circuit QED) studies light-matter interaction with superconducting circuits in one dimension. In circuit QED, natural atoms are replaced by superconducting qubits consisting of a non-linear Josephson junction, resulting in an anharmonic energy spectrum just like real atoms. With superconducting qubits, it is possible to study quantum optical phenomena and reach new regimes hard to achieve with real atoms due to weak coupling to the electromagnetic field. The reduction to one dimension in waveguide QED increases the electromagnetic field's directionality, which results in reduced losses. In this thesis, we first introduce circuit quantisation, giving the basis for the next part, where we investigate a transmon, a charge-insensitive artificial atom, coupled to a semi-infinite transmission line. An atom coupled to a semi-infinite waveguide is referred to as an atom in front of a mirror and is the subject of all appended papers. We proceed by summarising Paper I and III's main results: in Paper I, we investigate the spontaneous emission of a transmon coupled to a semi-infinite transmission line, where we take time-delay effects into account. We find that the system dynamics strongly depend on the coupling strength to the transmission line and the atom's position with respect to the electromagnetic field, leading to the Purcell effect or the convergence to a dark state with finite excitation probability. In the high-impedance regime, which we investigate in Paper III, the properties of the transmon coupled to the high-impedance transmission line change drastically. It becomes highly reflective and creates its own cavity with the mirror, resulting in the emergence of cavity modes and vacuum Rabi oscillations in the spontaneous emission dynamics. In the next chapter of the thesis, we demonstrate how to quantise an electromagnetic field and derive a light-matter interaction Hamiltonian within dipole approximation. We then give an introduction to open quantum systems and derive the quantum-optical master equation in Lindblad form. Furthermore, we introduce the dressed state picture, where the interaction of light and matter is so strong that the individual energy levels of light and matter are no longer separable. Both the quantum optical master equation and the dressed state picture are relevant in Paper II and IV. In Paper II, an experimental collaboration, we perform several experiments to characterise and discriminate different decay rates of a superconducting qubit coupled to the end of a transmission line. One experiment measured the atomic fluorescence spectral density, which shows an asymmetry for off-resonant driving, resulting from pure dephasing: an effect that we explain in more detail in this thesis and Paper II. In Paper IV, we theoretically investigate amplification mechanisms realised by different set-ups of an atom coupled to a semi-infinite waveguide. In the considered systems, the amplification of a probe field happens either due to population inversion between the pure states or dressed states or multi-photon processes. We find that compared to an open waveguide, we can achieve a higher gain in the amplification with a semi-infinite waveguide.