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arXiv:2010.00159 · Physical Review A

Direct observation of ion micromotion in a linear Paul trap

Liudmila A. Zhukas, Maverick J. Millican, P. Švihra, ANDREI NOMEROTSKI, B. B. Blinov

Published Feb 11, 2021• 28 citations
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Abstract

In this paper, direct observation of micromotion for multiple ions in a laser-cooled trapped ion crystal is discussed along with a measurement technique for micromotion amplitude. Micromotion is directly observed using a time-resolving, single-photon-sensitive camera that provides both fluorescence and position data for each ion on the nanosecond time scale. Micromotion amplitude and phase for each ion in the crystal are measured, allowing this method to be sensitive to tilts and shifts of the ion chain from the null of the radio-frequency quadrupole potential in the linear trap. Spatial resolution makes this micromotion detection technique suitable for complex ion configurations, including two-dimensional geometries. It does not require any additional equipment or laser beams, and the modulation of the cooling lasers or trap voltages is not necessary for detection as it is in other methods.

DOI
10.1103/physreva.103.023105

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In this paper, direct observation of micromotion for multiple ions in a laser-cooled trapped ion crystal is discussed along with a measurement technique for micromotion amplitude. Micromotion is directly observed using a time-resolving, single-photon-sensitive camera that provides both fluorescence and position data for each ion on the nanosecond time scale. Micromotion amplitude and phase for each ion in the crystal are measured, allowing this method to be sensitive to tilts and shifts of the ion chain from the null of the radio-frequency quadrupole potential in the linear trap. Spatial resolution makes this micromotion detection technique suitable for complex ion configurations, including two-dimensional geometries. It does not require any additional equipment or laser beams, and the modulation of the cooling lasers or trap voltages is not necessary for detection as it is in other methods.
For experiments with ions confined in a Paul trap, minimization of micromotion is often essential. In order to diagnose and compensate micromotion we have implemented a method that allows for finding the position of the radio-frequency (rf) null reliably and efficiently, in principle, without any variation of direct current (dc) voltages. We apply a trap modulation technique and focus-scanning imaging to extract three-dimensional ion positions for various rf drive powers and analyze the power dependence of the equilibrium position of the trapped ion. In contrast to commonly used methods, the search algorithm directly makes use of a physical effect as opposed to efficient numerical minimization in a high-dimensional parameter space. Using this method we achieve a compensation of the residual electric field that causes excess micromotion in the radial plane of a linear Paul trap down to $0.09\phantom{\rule{4pt}{0ex}}\text{V}\phantom{\rule{0.16em}{0ex}}{\text{m}}^{\ensuremath{-}1}$. Additionally, the precise position determination of a single harmonically trapped ion employed here can also be utilized for the detection of small forces. This is demonstrated by determining light pressure forces with a precision of 135 yN. As the method is based on imaging only, it can be applied to several ions simultaneously and is independent of laser direction and thus well suited to be used with, for example, surface-electrode traps.
Precise control of charged particles in radio-frequency (Paul) traps requires minimising excess micromotion induced by stray electric fields. We present a method to detect and compensate such fields through amplitude modulation of the radio-frequency trapping field. Modulation at frequencies close to the motional modes of the trapped particle excites coherent motion whose amplitude linearly depends on the stray field. In trapped-ion experiments, this motion can be detected by recording the arrival times of photons scattered during laser cooling. Only a single laser beam is required to resolve fields in multiple directions. In a demonstration using a 88Sr+^{88}\mathrm{Sr}^{+}88Sr+ ion in a surface electrode trap, we achieve a sensitivity of 0.1 V m−1 / Hz0.1\, \mathrm{V}\, \mathrm{m}^{-1}\, /\, \sqrt{\mathrm{Hz}}0.1Vm−1/Hz​ and a minimal uncertainty of 0.015 V m−10.015\, \mathrm{V}\, \mathrm{m}^{-1}0.015Vm−1.
Micromotion of ions in Paul traps has several adverse effects, including alterations of atomic transition line shapes, significant second-order Doppler shifts in high-accuracy studies, and limited confinement time in the absence of cooling. The ac electric field that causes the micromotion may also induce significant Stark shifts in atomic transitions. We describe three methods of detecting micromotion. The first relies on the change of the average ion position as the trap potentials are changed. The second monitors the amplitude of the sidebands of a narrow atomic transition, caused by the first-order Doppler shift due to the micromotion. The last technique detects the Doppler shift induced modulation of the fluorescence rate of a broad atomic transition. We discuss the detection sensitivity of each method to Doppler and Stark shifts, and show experimental results using the last technique.
We have fabricated a miniature three-segment linear Paul trap with r 0=0.6 mm and 2Z 0=4 mm. In order to perform quantum-state manipulation of trapped 40 Ca+ ions, we discuss the required harmonic oscillation frequencies which allow us to perform effective sideband cooling and have measured those that depend on the dimensions of the trap. A laser beam that has a component in the radial direction of the linear trap as well as that propagating along the trap axis has been used to detect the fluorescence spectra of the 42 S 1/2–42 P 1/2 transition. We have observed that the profile of the fluorescence spectrum obtained with the side laser beam is markedly different from that obtained with the axial laser beam due to micromotion. By applying additional DC voltages, the micromotion has been compensated, its amplitude has been estimated, and crystallization has been observed for two 40 Ca+ and four 40 Ca+ ions.
It is currently thought that the laser cooling of an ordered ion array, an ion crystal, is qualitatively the same as that of a single ion. We show that this assumption is strongly violated in recent experiments in Paul traps, due to ion micromotion. Our analysis demonstrates an unexpected laser damping instability that induces an ion-crystal order-chaos transition and also explains why ion crystals in Paul traps have been limited to less than 100 ions. We directly observe the effects of ion micromotion on the laser cooling of a single trapped Ba+{\mathrm{Ba}}^{+}Ba+ ion by a new technique.