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arXiv:2009.08351 · Physical review. B./Physical review. B

Intrinsic dissipative Floquet superconductors beyond mean-field theory

Qinghong Yang, Zhesen Yang, Dong E. Liu

Published Jul 19, 2021• 8 citations
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Abstract

We study the intrinsic superconductivity in a dissipative Floquet electronic system in the presence of attractive interactions. Based on the functional Keldysh theory beyond the mean-field treatment, we find that the system shows a time-periodic bosonic condensation and reaches an intrinsic dissipative Floquet superconducting (SC) phase. Due to the interplay between dissipations and periodic modulations, the Floquet SC gap becomes ``soft'' and contains the diffusive fermionic modes with finite lifetimes. However, bosonic modes of the bosonic condensation are still propagating even in the presence of dissipations.

DOI
10.1103/physrevb.104.014512

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•Nov 11, 2021•0 citations
We study the intrinsic superconductivity in a dissipative Floquet electronic system in the presence of attractive interactions. Based on the functional Keldysh theory beyond the mean-field treatment, we find that the system shows a time-periodic bosonic condensation and reaches an intrinsic dissipative Floquet superconducting (SC) phase. Due to the interplay between dissipations and periodic modulations, the Floquet SC gap becomes ``soft'' and contains the diffusive fermionic modes with finite lifetimes. However, bosonic modes of the bosonic condensation are still propagating even in the presence of dissipations.
Abstract Periodically driven systems provide a novel route to control the topology of quantum materials. In particular, Floquet theory allows an effective band description of periodically-driven systems through the Floquet Hamiltonian. Here, we study the time evolution of d-wave superconductors irradiated with intense circularly-polarized laser light. We consider the Floquet t–J model with time-periodic interactions, and investigate its mean-field dynamics by formulating the time-dependent Gutzwiller approximation. We observe the development of the idxy-wave pairing amplitude along with the original dx2−y2{d}_{{x}^{2}-{y}^{2}}dx2−y2​ d x 2 − y 2 -wave order upon gradual increasing of the field amplitude. We further numerically construct the Floquet Hamiltonian for the steady state, with which we identify the system as the fully-gapped d + id superconducting phase with a nonzero Chern number. We explore the low-frequency regime where the perturbative approaches in the previous studies break down, and find that the topological gap of an experimentally-accessible size can be achieved at much lower laser intensities.
Driven-dissipative physics lie at the core of quantum optics. However, the full interplay between a driven quantum many-body system and its environment remains relatively unexplored in the solid state realm. In this Letter, we inspect this interplay beyond the commonly employed stroboscopic Hamiltonian picture based on the specific example of a driven superconductor. Using the Shirley-Floquet and Keldysh formalisms as well as a generalization of the notion of superconducting fitness to the driven case, we show how a drive which anticommutes with the superconducting gap operator generically induces an unusual particle-hole structure in the spectral functions from the perspective of the thermal bath. Concomitant with a driving frequency which is near resonant with the intrinsic cutoff frequency of the underlying interaction, this spectral structure can be harnessed to enhance the superconducting transition temperature. Our work paves the way for further studies for driven-dissipative engineering of exotic phases of matter in solid-state systems.
Being an exemplary model of open quantum system, the spin-boson model is widely employed in theoretical and experimental studies. Beyond the weak coupling limit, the spin-boson dynamics can be described by a time-nonlocal generalized master equation with a memory kernel accounting for the dissipative effects induced by the bosonic environment. When the spin is in addition modulated by an external time-periodic electromagnetic field, the interplay between dissipation and forcing provides a spectrum of nontrivial asymptotic states, especially so in the regime of nonlinear response. Here we implement the method for evaluating the dissipative Floquet dynamics of non-Markovian systems introduced in Magazzù et al. [Phys. Rev. A 96, 042103 (2017)2469-992610.1103/PhysRevA.96.042103] to obtain these nonequilibrium asymptotic states.
Intense time-periodic laser fields can transform the electronic structure of a solid into strongly modified Floquet-Bloch bands. While this suggests multiple pathways to induce electronic orders such as superconductivity or charge density waves, the possibility of preparing low-energy phases of Floquet Hamiltonians remains unclear because of the energy absorption at typical experimentally accessible driving frequencies. Here we investigate a realistic pathway towards laser control of electronic orders, which is the transient enhancement of fluctuating orders. Using a conserving Keldysh Green's function formalism, we simulate the buildup of short range Cooper-pair correlations out of a normal metal in the driven attractive Hubbard model. Even for frequencies only slightly above or within the bandwidth, a substantial enhancement of correlations can be achieved before the system reaches a high electronic temperature. This behavior relies on the nonthermal nature of the driven state. The effective temperature of the electrons at the Fermi surface, which more closely determines the superconducting correlations, remains lower than an estimate from the global energy density. Even though short ranged, the fluctuations can have marked signatures in the electronic spectra.
Non-Hermitian Hamiltonians provide a simple picture for inspecting dissipative systems with natural or induced gain and loss. We investigate the Floquet dynamical phase transition in the dissipative periodically time-driven XY and extended XY models, where the imaginary terms represent the physical gain and loss during the interacting processes with the environment. The time-independent effective Floquet non-Hermitian Hamiltonians disclose three regions by analyzing the non-Hermitian gap: pure real gap (real eigenvalues), pure imaginary gap, and complex gap. We show that each region of the system can be distinguished by the complex geometrical nonadiabatic phase. We have discovered that in the presence of dissipation, the Floquet dynamical phase transitions (FDPTs) still exist in the region where the time-independent effective Floquet non-Hermitian Hamiltonians reveal real eigenvalues. Opposed to expectations based on earlier works on quenched systems, our findings show that the existence of the non-Hermitian topological phase is not an essential condition for dissipative FDPTs (DFDPTs). We also demonstrate the range of driven frequency, over which the DFDPTs occur, narrows down by increasing the dissipation coupling and shrinks to a single point at the critical value of dissipation. Moreover, quantization and jumps of the dynamical geometric phase reveals the topological characteristic feature of DFDPTs in the real gap region where confined to exceptional points.
Non-Hermitian Hamiltonians provide a simple picture for inspecting dissipative systems with natural or induced gain and loss. We investigate the Floquet dynamical phase transition in the dissipative periodically time driven XY and extended XY models, where the imaginary terms represent the physical gain and loss during the interacting processes with the environment. The time-independent effective Floquet non-Hermitian Hamiltonians disclose three regions by analyzing the non-Hermitian gap: pure real gap (real eigenvalues), pure imaginary gap, and complex gap. We show that each region of the system can be distinguished by the complex geometrical non-adiabatic phase. We have discovered that in the presence of dissipation, the Floquet dynamical phase transitions (FDPTs) still exist in the region where the time-independent effective Floquet non-Hermitian Hamiltonians reveal real eigenvalues. Opposed to expectations based on earlier works on quenched systems, our findings show that the existence of the non-Hermitian topological phase is not an essential condition for dissipative FDPTs (DFDPTs). We also demonstrate the range of driven frequency, over which the DFDPTs occur, narrows down by increasing the dissipation coupling and shrinks to a single point at the critical value of dissipation. Moreover, quantization and jumps of the dynamical geometric phase reveals the topological characteristic feature of DFDPTs in the real gap region where confined to exceptional points.