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arXiv:2007.10305 · Physical review. B./Physical review. B

Electronic and fluctuation dynamics following a quench to the superconducting phase

Christopher Stahl, Martin Eckstein

Published Jan 13, 2021• 17 citations
arXivHTMLPDF

Abstract

We investigate the dynamics of superconducting fluctuations in the attractive three-dimensional Hubbard model after a quench from the disordered phase to the ordered regime. While the long-time evolution is well understood in terms of dissipative time-dependent Ginzburg-Landau models with unstable potentials, early times are more demanding due to the inseparable dynamics of the pairing fluctuations and the electronic quasiparticles. Our simulation using the time-dependent fluctuation exchange approximation treats both degrees of freedom on the same footing and reveals a nonthermal electronic regime causing a nonmonotonous growth of the fluctuations. This feature is not directly captured by the Ginzburg-Landau theory but nevertheless remains observable beyond the thermalization time of the electrons. We further explore how the growth of the order parameter fluctuations leads to an opening of a pseudogap in the electronic spectrum and identify Andreev reflections as the dominant mechanism behind the gap opening.

DOI
10.1103/physrevb.103.035116

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We investigate the dynamics of superconducting fluctuations in the attractive three-dimensional Hubbard model after a quench from the disordered phase to the ordered regime. While the long-time evolution is well understood in terms of dissipative time-dependent Ginzburg-Landau models with unstable potentials, early times are more demanding due to the inseparable dynamics of the pairing fluctuations and the electronic quasiparticles. Our simulation using the time-dependent fluctuation exchange approximation treats both degrees of freedom on the same footing and reveals a nonthermal electronic regime causing a nonmonotonous growth of the fluctuations. This feature is not directly captured by the Ginzburg-Landau theory but nevertheless remains observable beyond the thermalization time of the electrons. We further explore how the growth of the order parameter fluctuations leads to an opening of a pseudogap in the electronic spectrum and identify Andreev reflections as the dominant mechanism behind the gap opening.
We present a framework of semiclassical superconductivity (SC) dynamics that properly includes effects of spatial fluctuations for the attractive Hubbard model. We consider both coherent and adiabatic limits. To model the coherent SC dynamics, we develop a real-space von Neumann equation based on the time-dependent Hartree-Fock-Bogoliubov theory. Applying our method to interaction quenches in the negative-UUU Hubbard model, we show that the relaxation of SC order at weak coupling is dominated by Landau-damping. At strong coupling, we find a two-stage relaxation of the pairing field: a collapse of the synchronized oscillation of Cooper pairs due to spatial inhomogeneity, followed by a slow relaxation to a quasistationary state. SC dynamics in the adiabatic limit is described by a quantum Landau-Lifshitz equation with Ginzburg-Landau relaxation. Numerical simulations of the pump-probe process show that long-time recovery of the pairing field is dominated by defect dynamics. Our results demonstrate the important role of spatial fluctuations in both limits.
We consider a lattice version of the ``negative-U′′U''U′′ Hubbard model in three dimensions, to study the crossover from a superconducting phase transition (dominated by phase fluctuation) to a regime where the amplitude of the superconducting order parameter controls the critical temperature. Starting from a fermionic Hamiltonian, we give a microscopic derivation of the effective action in terms of the relevant physical fields: the modulus and phase of the superconducting order parameter. Furthermore, by employing to the resulting coarse--grained quantum XY\mathrm{XY}XY model the phase fluctuation algebra between number and phase operators (given by the Euclidean group E2),{E}_{2}),E2​), we map the ``phase-only'' action onto a solvable quantum spherical model. We establish the self--consistent theory (involving both fermionic and bosonic degrees of freedom), and calculate the superconducting phase coherence transition temperature Tc{T}_{c}Tc​ as a function of the coupling strength ∣U∣,|U|,∣U∣, exhibiting a maximum where the behavior crosses over from BCS to Bose-Einstein (BE) condensation. We examine a pseudogap in the normal state which emerges naturally as a precursor of superconductivity at the second characteristic temperature Tg{T}_{g}Tg​ due to a state with bound pairs but without long--range phase coherence. Furthermore, we demonstrate that the reduced gaps of the model $2{\ensuremath{\Delta}}_{0}{/k}_{B}{T}_{g}\ensuremath{\sim}4$ is almost independent on the pairing strength ∣U∣/t,|U|/t,∣U∣/t, whereas $2{\ensuremath{\Delta}}_{0}{/k}_{B}{T}_{c}$ increases with increasing ∣U∣|U|∣U∣---in striking analogy with the phenomenology of the high--temperature cuprate superconductors when interpreted in terms of the BCS-BC crossover scenario.
We study the phase fluctuations in the normal state of generic two-dimensional superconducting systems with sss-wave pairing. The effect of phase fluctuations of the pairing fields can be dealt with perturbatively using disorder averaging, after we treat the local superconducting order parameter as a static disordered background. It is then confirmed that the phase fluctuations above the two-dimensional Berezinskii-Kosterlitz-Thouless transition lead to a significant broadening of the single-particle spectrum, giving birth to the pseudogap phenomenon. Quantitatively, the broadening of spectral weights near the BCS gap is characterized by the ratio of the superconducting coherence length and the spatial correlation length of the superconducting pairing order parameter. Our results are tested on the fermionic attractive-UUU Hubbard model on the square lattice, using the unbiased determinant quantum Monte Carlo method and stochastic analytic continuation.
We derive a Ginzburg–Landau (GL) expansion in the disordered attractive Hubbard model within the combined Nozieres–Schmitt-Rink and DMFT+Σ approximation. Restricting ourselves to the homogeneous expansion, we analyze the disorder dependence of GL expansion coefficients for a wide range of attractive potentials U, from the weak BCS coupling region to the strong-coupling limit, where superconductivity is described by Bose–Einstein condensation (BEC) of preformed Cooper pairs. We show that for the a semielliptic “bare” density of states of the conduction band, the disorder influence on the GL coefficients A and B before quadratic and quartic terms of the order parameter, as well as on the specific heat discontinuity at the superconducting transition, is of a universal nature at any strength of the attractive interaction and is related only to the general widening of the conduction band by disorder. In general, disorder growth increases the values of the coefficients A and B, leading either to a suppression of the specific heat discontinuity (in the weak-coupling limit), or to its significant growth (in the strong-coupling region). However, this behavior actually confirms the validity of the generalized Anderson theorem, because the disorder dependence of the superconducting transition temperature T c, is also controlled only by disorder widening of the conduction band (density of states).
Results are presented for the time evolution of fermions initially in a nonzero temperature normal phase, following the switch on of an attractive interaction. The dynamics are studied in the disordered phase close to the critical point, where the superfluid fluctuations are large. The analysis is conducted within a two-particle irreducible, large NNN approximation. The system is considered from the perspective of critical quenches where it is shown that the fluctuations follow universal model A dynamics. A signature of this universality is found in a singular correction to the fermion lifetime, given by a scaling form ${t}^{(3\ensuremath{-}d)/2}{S}_{d}({\ensuremath{\varepsilon}}^{2}t)$, where ddd is the spatial dimension, ttt is the time since the quench, and $\ensuremath{\varepsilon}$ is the fermion energy. The singular behavior of the spectral density is interpreted as arising due to incoherent Andreev reflections off superfluid fluctuations.
Results are presented for the quench dynamics of a clean and interacting electron system, where the quench involves varying the strength of the attractive interaction along arbitrary quench trajectories. The initial state before the quench is assumed to be a normal electron gas, and the dynamics is studied in a regime where long-range order is absent, but nonequilibrium superconducting fluctuations need to be accounted for. A quantum kinetic equation using a two-particle irreducible formalism is derived. Conservation of energy, particle number, and momentum emerge naturally, with the conserved currents depending on both the electron Green's functions and the Green's functions for the superconducting fluctuations. The quantum kinetic equation is employed to derive a kinetic equation for the current, and the transient optical conductivity relevant to pump-probe spectroscopy is studied. The general structure of the kinetic equation for the current is also justified by a phenomenological approach that assumes model F in the Halperin-Hohenberg classification, corresponding to a nonconserved order parameter coupled to a conserved density. Linear response conductivity and the diffusion coefficients in thermal equilibrium are also derived, and connections with Aslamazov-Larkin fluctuation corrections are highlighted. Results are also presented for the time evolution of the local density of states. It is shown that Andreev scattering processes result in an enhanced density of states at low frequencies. For a quench trajectory corresponding to a sudden quench to the critical point, the density of states is shown to grow in a manner where the time after the quench plays the role of the inverse detuning from the critical point.