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arXiv:2005.13302 · Physical Review Letters

E 8 Spectra of Quasi-One-Dimensional Antiferromagnet BaCo 2 V 2 O 8 under Transverse Field

Haiyuan Zou, Yi Cui, Xiao Wang, Zhao Zhang, Jiahao Yang, Guangyong Xu, Akira Okutani, Masayuki Hagiwara, Masaaki Matsuda, Gang Wang, Giuseppe Mussardo, Kristóf Hódsági, Márton Kormos, Zhangzhen He, Shojiro Kimura, Rong Yu, Weiqiang Yu, Jie Ma, Jianda Wu

Published Aug 9, 2021• 57 citations
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Abstract

We report ^{51}V NMR and inelastic neutron scattering (INS) measurements on a quasi-1D antiferromagnet BaCo_{2}V_{2}O_{8} under transverse field along the [010] direction. The scaling behavior of the spin-lattice relaxation rate above the Néel temperatures unveils a 1D quantum critical point (QCP) at H_{c}^{1D}≈4.7 T, which is masked by the 3D magnetic order. With the aid of accurate analytical analysis and numerical calculations, we show that the zone center INS spectrum at H_{c}^{1D} is precisely described by the pattern of the 1D quantum Ising model in a magnetic field, a class of universality described in terms of the exceptional E_{8} Lie algebra. These excitations are nondiffusive over a certain field range when the system is away from the 1D QCP. Our results provide an unambiguous experimental realization of the massive E_{8} phase in the compound, and open a new experimental route for exploring the dynamics of quantum integrable systems as well as physics beyond integrability.

DOI
10.1103/physrevlett.127.077201

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We report ^{51}V NMR and inelastic neutron scattering (INS) measurements on a quasi-1D antiferromagnet BaCo_{2}V_{2}O_{8} under transverse field along the [010] direction. The scaling behavior of the spin-lattice relaxation rate above the Néel temperatures unveils a 1D quantum critical point (QCP) at H_{c}^{1D}≈4.7 T, which is masked by the 3D magnetic order. With the aid of accurate analytical analysis and numerical calculations, we show that the zone center INS spectrum at H_{c}^{1D} is precisely described by the pattern of the 1D quantum Ising model in a magnetic field, a class of universality described in terms of the exceptional E_{8} Lie algebra. These excitations are nondiffusive over a certain field range when the system is away from the 1D QCP. Our results provide an unambiguous experimental realization of the massive E_{8} phase in the compound, and open a new experimental route for exploring the dynamics of quantum integrable systems as well as physics beyond integrability.
Exceptional E8_88​ symmetry in spin dynamics of quasi-one-dimensional antiferromagnet BaCo2_22​V2_22​O8_88​
Exotic excitations can emerge in the vicinity of a quantum phase transition. When the quantum critical point of the one-dimensional (1D) transverse field Ising model is perturbed by a longitudinal magnetic field, it was predicted that its massive excitations are precisely described by the exceptional E8_88​ Lie algebra. Here we show an unambiguous experimental realization of the massive E8_88​ phase in the quasi-1D antiferromagnetic material BaCo2_22​V2_22​O8_88​, via nuclear magnetic resonance and inelastic neutron scattering measurements, and detailed theoretical analysis. The large separation between the masked 1D and 3D quantum critical points of the system allows us to identify, for the first time, the full 8 single-particle E8_88​ excitations as well as various multi-particle states in the spin excitation spectrum. Our results open new experimental route for exploring the dynamics of quantum integrable systems and physics beyond integrability, and thus bridge key physics in condensed matter and statistical field theory.
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In this article, we report on inelastic neutron scattering measurements on a quasi-1D antiferromagnet BaCo2_22​V2_22​O8_88​ under a transverse magnetic field applied along the (0,1,0) direction. Combining results of inelastic neutron scattering experiments, analytical analysis, and numerical simulations, we precisely studied the E8E_8E8​ excitations appearing in the whole Brillouin zone at Bc1D≈4.7B_c^{1D}\approx 4.7Bc1D​≈4.7 T. The energy scan at Q=(0,0,2)Q=(0,0,2)Q=(0,0,2) reveals a match between the data and the theoretical prediction of energies of multiple E8E_8E8​ excitations. Furthermore, dispersions of the lightest three E8E_8E8​ particles have been clearly observed, confirming the existence of the E8E_8E8​ particles in BaCo2_22​V2_22​O8_88​. Our results lay down a concrete ground to systematically study the physics of the exotic E8E_8E8​ particles.
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Quantum integrability emerging near a quantum critical point (QCP) is manifested by an exotic excitation spectrum that is organized by the associated algebraic structure. A well-known example is the emergent E8{E}_{8}E8​ integrability near the QCP of a transverse field Ising chain (TFIC), which was long predicted theoretically and initially proposed to be realized in the quasi-one-dimensional (q1D) quantum magnet CoNb2O6{\mathrm{CoNb}}_{2}{\mathrm{O}}_{6}CoNb2​O6​. However, later measurements on the spin excitation spectrum of this material revealed a series of satellite peaks in low energies that go beyond the description of the E8{E}_{8}E8​ Lie algebra. Motivated by this experimental progress, we hereby revisit the spin excitations of CoNb2O6{\mathrm{CoNb}}_{2}{\mathrm{O}}_{6}CoNb2​O6​ by combining numerical calculation and analytical analysis. We show that, as effects of strong interchain fluctuations, the spectrum of the system near the 1D QCP is characterized by an emergent D8(1){D}_{8}^{(1)}D8(1)​ Lie algebra instead of the E8{E}_{8}E8​ one. We further show that the D8(1){D}_{8}^{(1)}D8(1)​ spectrum can be realized in a broad class of interacting quantum systems. Our results advance the exploration and manipulation of integrability in quantum critical systems.
We study the dynamics of the quasi-one-dimensional Ising-Heisenberg antiferromagnet BaCo2V2O8{\mathrm{BaCo}}_{2}{\mathrm{V}}_{2}{\mathrm{O}}_{8}BaCo2​V2​O8​ under a transverse magnetic field. Combining inelastic neutron scattering experiments and theoretical analyses by field theories and numerical simulations, we mainly elucidate the structure of the spin excitation spectrum in the high-field phase, appearing above the quantum phase transition point ${\ensuremath{\mu}}_{0}{H}_{c}\ensuremath{\approx}10\phantom{\rule{0.28em}{0ex}}\mathrm{T}$. We find that it is characterized by collective solitonic excitations superimposed on a continuum. These solitons are strongly bound in pairs due to the effective staggered field induced by the nondiagonal ggg tensor of the compound and are topologically different from the fractionalized spinons in the weak-field region. The dynamical susceptibility numerically calculated with the infinite time-evolving block decimation method shows an excellent agreement with the measured spectra, which enables us to identify the dispersion branches with elementary excitations. The lowest-energy dispersion has an incommensurate nature and has a local minimum at an irrational wave number due to the applied transverse field.