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arXiv:2005.08308 · Physical Review Letters

Anomalous Spin-Charge Separation in a Driven Hubbard System

Hongmin Gao, Jonathan R. Coulthard, Dieter Jaksch, Jordi Mur-Petit

Published Nov 2, 2020• 11 citations
arXivHTMLPDF

Abstract

Spin-charge separation (SCS) is a striking manifestation of strong correlations in low-dimensional quantum systems, whereby a fermion splits into separate spin and charge excitations that travel at different speeds. Here, we demonstrate that periodic driving enables control over SCS in a Hubbard system near half filling. In one dimension, we predict analytically an exotic regime where charge travels slower than spin and can even become "frozen," in agreement with numerical calculations. In two dimensions, the driving slows both charge and spin and leads to complex interferences between single-particle and pair-hopping processes.

DOI
10.1103/physrevlett.125.195301

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Spin-charge separation (SCS) is a striking manifestation of strong correlations in low-dimensional quantum systems, whereby a fermion splits into separate spin and charge excitations that travel at different speeds. Here, we demonstrate that periodic driving enables control over SCS in a Hubbard system near half filling. In one dimension, we predict analytically an exotic regime where charge travels slower than spin and can even become "frozen," in agreement with numerical calculations. In two dimensions, the driving slows both charge and spin and leads to complex interferences between single-particle and pair-hopping processes.
Obtaining a microscopic understanding of the dynamics in strongly correlated electronic systems has remained a challenge for many decades. The interplay between the spin and charge degrees of freedom in these materials at different temperatures and dopant concentrations is not well understood and is still an area of intense scientific research. Recently, quantum simulators based on ultracold atoms in optical lattices have emerged as a promising platform to probe strongly correlated fermionic systems. This thesis reports on the work carried out with a quantum gas microscope of ultracold fermionic Li-6, where Fermi-Hubbard systems are prepared and imaged with single site spin and density resolution. The main results of the thesis explore the microscopic dynamics underlying one-dimensional materials, where individual constituents such as the electron with charge e and spin-1/2 are not relevant to the description of the system anymore and are instead replaced by spin and charge excitations that can propagate independent of one another - a phenomenon called spin-charge separation. In our quantum simulator, we use analogous one-dimensional Fermi-Hubbard chains of Li-6, to perform time- and space-resolved microscopy of the spin and charge excitations following a local quench. By extracting their strikingly different velocities and showing an absence of binding between the excitations, we demonstrate spin-charge separation. Our microscopic technique also allows us to quantitatively extract the excess spin carried by the spin excitiation, connecting our results to the phenomenon of fractionalization. In another set of experiments, Fermi-Hubbard chains are probed at equilibrium and incommensurate spin correlations arising in the presence of both density doping and spin polarization are observed. The wavevector of these incommensurate correlations are found to have a linear dependence on doping and polarization. Finally, the effect of the spin-charge interplay is probed in the crossover from one to two dimensions. The spin correlations across dopants are seen to be dramatically different in two dimensions, and the strong antiferromagnetic correlations across dopants present in one dimension disappear. For a single dopant in a fully two dimensional system, the spin-charge interplay manifests as a distorted spin cloud surrounding the dopant, indicating the formation of a magnetic polaron. The experiments reported here demonstrate the power of a quantum simulator; by probing the physics of strongly correlated systems in real space with unprecedented resolution, we can zoom into emergent phenomena, validate theories and access regimes that are not possible in other experimental settings.
In this article we study quantum phases and the phase diagram of a Fermi-Hubbard model under periodic driving that has been realized in recent cold-atom experiments, in particular, when the driving frequency is nearly resonant with the interaction energy. Due to the driving, the effective Hamiltonian contains a correlated hopping term where the density occupation strongly modifies the hopping strength. Focusing on half filling, in addition to the charge- and spin-density wave phases, large regions of ferromagnetic phase and phase separation are discovered in the weakly interacting regime. The mechanism of this ferromagnetism is attributed to the correlated hopping, because the hopping strength within a ferromagnetic domain is normalized to a larger value than the hopping strength across the domain. Thus, the kinetic energy drives the system into a ferromagnetic phase. We note that this is a different mechanism, in contrast to the well-known Stoner mechanism for ferromagnetism where the ferromagnetism is driven by interaction energy.
We propose using ultracold fermionic atoms trapped in a periodically shaken optical lattice as a quantum simulator of the $t\text{\ensuremath{-}}J$ Hamiltonian, which describes the dynamics in doped antiferromagnets and is thought to be relevant to the problem of high-temperature superconductivity in the cuprates. We show analytically that the effective Hamiltonian describing this system for off-resonant driving is the $t\text{\ensuremath{-}}J$ model with additional pair hopping terms, whose parameters can all be controlled by the drive. We then demonstrate numerically using tensor network methods for a one-dimensional (1D) lattice that a slow modification of the driving strength allows near-adiabatic transfer of the system from the ground state of the underlying Hubbard model to the ground state of the effective $t\text{\ensuremath{-}}J$ Hamiltonian. Finally, we report exact diagonalization calculations illustrating the control achievable on the dynamics of spin-singlet pairs in 2D lattices utilizing this technique with current cold-atom quantum-simulation technology. These results open new routes to explore the interplay between density and spin in strongly correlated fermionic systems through their out-of-equilibrium dynamics.
The question of spin-charge separation in two-dimensional lattices has been addressed by numerical simulations of the motion of one hole in a half-filled band. The calculations have been performed on finite clusters with Hubbard and t-J models. By comparing the time evolution of spin and charge polarization currents in one and two dimensions, evidence in favor of spin-charge separation in two dimensions is presented. In contrast with this, spin-charge separation is absent in a highly doped, metallic, system.
The persistent current and spin-charge separation are studied in a one-dimensional (1D) Hubbard ring with side sites connected to the even sites of the ring. At half filling, the persistent current is always paramagnetic and has a period of flux quantum. Away from half filling, as the onsite repulsion UUU increases, the sign of the current may oscillate depending on the total number of electrons Ne{N}_{e}Ne​ and the hopping ttt between the ring site and the side site. For small hopping ttt, the number of electrons ${N}_{e}^{\ensuremath{'}}$ in the ring sites plays an important role in determining the sign of the current. In contrast to the 1D Hubbard model, a weak or a moderate UUU can strongly enhance the persistent current while the hopping ttt always suppresses the current. The study on the transmittance of the ring with two connected leads indicates that in the large UUU and small ttt case, the transmittance varies with a period $1∕{N}_{e}^{\ensuremath{'}}$ of a flux quantum, demonstrating a spin-charge separation in this system.
Strong electron correlations lie at the origin of high-temperature superconductivity. Its essence is believed to be captured by the Fermi-Hubbard model of repulsively interacting fermions on a lattice. Here we report on the site-resolved observation of charge and spin correlations in the two-dimensional (2D) Fermi-Hubbard model realized with ultracold atoms. Antiferromagnetic spin correlations are maximal at half-filling and weaken monotonically upon doping. At large doping, nearest-neighbor correlations between singly charged sites are negative, revealing the formation of a correlation hole, the suppressed probability of finding two fermions near each other. As the doping is reduced, the correlations become positive, signaling strong bunching of doublons and holes, in agreement with numerical calculations. The dynamics of the doublon-hole correlations should play an important role for transport in the Fermi-Hubbard model.