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arXiv:2005.04299 · Physical Review Letters

Superatom Picture of Collective Nonclassical Light Emission and Dipole Blockade in Atom Arrays

L. A. Williamson, Magnus O. Borgh, Janne Ruostekoski

Published Aug 13, 2020• 73 citations
arXivHTMLPDF

Abstract

We show that two-time, second-order correlations of scattered photons from planar arrays and chains of atoms display nonclassical features that can be described by a superatom picture of the canonical single-atom g_{2}(τ) resonance fluorescence result. For the superatom, the single-atom linewidth is replaced by the linewidth of the underlying collective low light-intensity eigenmode. Strong light-induced dipole-dipole interactions lead to a correlated response, suppressed joint photon detection events, and dipole blockade that inhibits multiple excitations of the collective atomic state. For targeted subradiant modes, the nonclassical nature of emitted light can be dramatically enhanced even compared with that of a single atom.

DOI
10.1103/physrevlett.125.073602

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We realize collective enhancement and suppression of light scattered by an array of tweezer-trapped ^{87}Rb atoms positioned within a strongly coupled Fabry-Pérot optical cavity. We illuminate the array with light directed transverse to the cavity axis, in the low saturation regime, and detect photons scattered into the cavity. For an array with integer-optical-wavelength spacing each atom scatters light into the cavity with nearly identical scattering amplitude, leading to an observed N^{2} scaling of cavity photon number as the atom number increases stepwise from N=1 to N=8. By contrast, for an array with half-integer-wavelength spacing, destructive interference of scattering amplitudes yields a nonmonotonic, subradiant cavity intensity versus N. By analyzing the polarization of light emitted from the cavity, we find that Rayleigh scattering can be collectively enhanced or suppressed with respect to Raman scattering. We observe also that atom-induced shifts and broadenings of the cavity resonance are precisely tuned by varying the atom number and positions. Altogether, tweezer arrays provide exquisite control of atomic cavity QED spanning from the single- to the many-body regime.
The recoil of atoms in arrays due to the emission or absorption of photons is studied for subwavelength interatomic spacing. The atoms in the array interact with each other through collective dipole-dipole interactions and with the incident laser field in the low-intensity limit. Shining uniform light on the array gives rise to patterns of excitation and recoil in the array. They arise due to the interference of different eigenmodes of excitation. The relation between the recoil and the decay dynamics is studied when the array is in its excitation eigenstates. The recoil experienced by a subradiant collective decay is substantially larger than that from independent atom decay.
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The recoil of atoms in arrays due to the emission or absorption of photons is studied for subwavelength interatomic spacing. The atoms in the array interact with each other through collective dipole-dipole interactions and with the incident laser field in the low-intensity limit. Shining uniform light on the array gives rise to patterns of excitation and recoil in the array. They arise due to the interference of different eigenmodes of excitation. The relation between the recoil and the decay dynamics is studied when the array is in its excitation eigenstates. The recoil experienced by a subradiant collective decay is substantially larger than that from independent atom decay. A method to calculate the rate of recoil when steady state has been achieved with a constant influx of photons is also described.
We experimentally study resonant light scattering by a one-dimensional randomly filled chain of cold two-level atoms. By a local measurement of the light scattered along the chain, we observe constructive interferences in light-induced dipole-dipole interactions between the atoms. They lead to a shift of the collective resonance despite the average interatomic distance being larger than the wavelength of the light. This result demonstrates that strong collective effects can be enhanced by structuring the geometrical arrangement of the ensemble. We also explore the high intensity regime where atoms cannot be described classically. We compare our measurement to a mean-field, nonlinear coupled-dipole model accounting for the saturation of the response of a single atom.