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arXiv:2307.13321 · Physical Review Letters

Superradiant and Subradiant Cavity Scattering by Atom Arrays

Zhenjie Yan, Jacquelyn Ho, Yuehui Lu, Stuart J. Masson, Ana Asenjo-Garcı́a, Dan Stamper-Kurn

Published Dec 21, 2023• 60 citations
arXivHTMLPDF

Abstract

We realize collective enhancement and suppression of light scattered by an array of tweezer-trapped ^{87}Rb atoms positioned within a strongly coupled Fabry-Pérot optical cavity. We illuminate the array with light directed transverse to the cavity axis, in the low saturation regime, and detect photons scattered into the cavity. For an array with integer-optical-wavelength spacing each atom scatters light into the cavity with nearly identical scattering amplitude, leading to an observed N^{2} scaling of cavity photon number as the atom number increases stepwise from N=1 to N=8. By contrast, for an array with half-integer-wavelength spacing, destructive interference of scattering amplitudes yields a nonmonotonic, subradiant cavity intensity versus N. By analyzing the polarization of light emitted from the cavity, we find that Rayleigh scattering can be collectively enhanced or suppressed with respect to Raman scattering. We observe also that atom-induced shifts and broadenings of the cavity resonance are precisely tuned by varying the atom number and positions. Altogether, tweezer arrays provide exquisite control of atomic cavity QED spanning from the single- to the many-body regime.

DOI
10.1103/physrevlett.131.253603

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We realize collective enhancement and suppression of light scattered by an array of tweezer-trapped ^{87}Rb atoms positioned within a strongly coupled Fabry-Pérot optical cavity. We illuminate the array with light directed transverse to the cavity axis, in the low saturation regime, and detect photons scattered into the cavity. For an array with integer-optical-wavelength spacing each atom scatters light into the cavity with nearly identical scattering amplitude, leading to an observed N^{2} scaling of cavity photon number as the atom number increases stepwise from N=1 to N=8. By contrast, for an array with half-integer-wavelength spacing, destructive interference of scattering amplitudes yields a nonmonotonic, subradiant cavity intensity versus N. By analyzing the polarization of light emitted from the cavity, we find that Rayleigh scattering can be collectively enhanced or suppressed with respect to Raman scattering. We observe also that atom-induced shifts and broadenings of the cavity resonance are precisely tuned by varying the atom number and positions. Altogether, tweezer arrays provide exquisite control of atomic cavity QED spanning from the single- to the many-body regime.
Abstract By considering linear scattering of laser-driven cold atoms inside an undriven high-finesse optical resonator, we experimentally demonstrate effects unique to a strongly coupled vacuum field. Arranging the atoms in an incommensurate lattice with respect to the radiation wavelength, the Bragg scattering into the cavity can be suppressed by destructive interference: the atomic array is subradiant to the cavity mode under transverse illumination. We show however, that strong collective coupling leads to a drastic modification of the excitation spectrum, as evidenced by well-resolved vacuum Rabi splitting in the intensity of the fluctuations. Furthermore, we demonstrate a significant polarization rotation in the linear scattering off the subradiant array via Raman scattering induced by the strongly coupled vacuum field.
Integrating Rydberg-state control of atom-atom interactions with cavity control of atom-light interactions enables the combination of local entangling operations with photon-mediated long-range coupling, measurement, and communication. Such integration is challenging because electric fields generated by charges on cavity optics and by cavity-stabilizing actuators may disturb Rydberg-state coherence. Here, we couple a Rydberg tweezer array to a high-cooperativity optical cavity, suppressing the electric fields produced by cavity length actuation so that the residual field variation of about 3 mV/cm3~\mathrm{mV/cm}3 mV/cm rms does not limit Rydberg coherence. We demonstrate two capabilities that neither system provides alone. First, we use Purcell-enhanced fluorescence to read out atoms directly in the ground-Rydberg basis within 7.5 μs7.5~μ\mathrm{s}7.5 μs, well within the Rydberg-state lifetime, with ground- and Rydberg-state detection infidelities of 3%3\%3% and 5%5\%5%, respectively, and with low atom loss. Second, we use Rydberg-Rydberg interactions to control collective light-atom scattering into the cavity mode. Specifically, we drive blockaded Rabi oscillations between a state with two ground-state atoms, which scatter collectively with a superradiant or subradiant rate controlled by the atomic positions, and an entangled state with a single Rydberg excitation, which scatters like a single atom. These capabilities open routes toward networked Rydberg processors, mid-circuit measurements in analog quantum simulators, and many-body quantum optics with entangled emitters coupled collectively to light.
A central challenge for cavity-QED-based quantum technologies is to make high-cooperativity optical interfaces compatible with site-resolved arrays of single atoms. Here, we demonstrate optical tweezer arrays of individual 87^{87}87Rb atoms inside a fiber Fabry-Perot microcavity with single-atom cooperativity C∼90\mathcal{C} \sim 90C∼90. We combine background-free site-resolved fluorescence imaging of extended arrays with collective coupling to a common cavity mode for arrays with a mean atom number up to Nˉ≃36\bar{N} \simeq 36Nˉ≃36. These results establish a high-cooperativity platform for many-body cavity-QED with site-resolved detection and control.
Strong atom-photon interactions in optical cavities are a key resource for quantum information processing, quantum networking, and the exploration of quantum optical effects. Optical tweezer arrays offer scalable, site-resolved control of neutral atoms, but their integration with high-cooperativity cavity QED systems remains challenging. Here we combine a twelve-site 87^{87}87Rb optical tweezer array with a high-cooperativity fiber Fabry-Pérot microcavity. The array is positioned within the cavity mode and individual sites are controlled with subwavelength precision, enabling continuous tuning of the single-atom coupling strength via deterministic displacement through the standing-wave field. For up to five atoms coupled to the cavity, we measure collectively enhanced vacuum Rabi splitting and implement cavity-based non-destructive readout of the number of coupled atoms. These results establish a scalable architecture for cavity-mediated entanglement generation and many-body cavity QED with single-atom control, and they lay the foundation for fiber-integrated quantum network nodes.
Coupling between quantum emitters and modes of light is foundational to studies of quantum systems. Coherent interactions between matter and light have greatly advanced the development of quantum technologies. When an ensemble of atoms interacts with light that is confined within a cavity---a resonator for photons---light also mediates atom-atom interactions, leading to collective phenomena that cannot be extrapolated from microscopic behaviors. Understanding how interactions among quantum particles lead to macroscopic phenomena, such as phase transitions and breaking of symmetries, remains a challenge in modern physics. In this dissertation, I present results addressing this challenge in the context of mesoscopic arrays of optical-tweezer-trapped atoms interfaced with a high-finesse optical cavity. In particular, the physics we investigate arises from the collective scattering of light. Utilizing the ability to place atoms with nanometer-scale precision, we engineer superradiant and subradiant states, where control over interference of the emission from multiple atoms leads to collectively enhanced or suppressed amounts of scattered light. Building on this work, we investigate the emergence of optomechanical self-organization, mediated by superradiance in the cavity electromagnetic field. By coupling atoms to the same cavity mode, the atoms exert forces on one another through the exchange of photons, leading them to autonomously order themselves spatially. We characterize mesoscopic fluctuations and their effect on symmetry-breaking dynamics associated with self-organization. Finally, we extend this framework to theoretically investigate how the phase of the atom-cavity coupling can be altered to generate higher symmetries. Our analysis reveals first-order phase transitions and instabilities induced by non-reciprocal forces. Altogether, this work establishes a path towards realizing mesoscopic systems of complex phases of matter in cavity quantum electrodynamics with unprecedented programmability.
We consider the coupling of light, via an optical cavity, to two-dimensional atomic arrays whose lattice spacing exceeds the wavelength of the light. Such “superwavelength” spacing is typical of optical tweezer arrays. While subwavelength arrays exhibit strong atom-photon coupling, characterized by high optical reflectivity in free space, the coupling efficiency of superwavelength arrays is reduced due to collective scattering losses to high diffraction orders. We show how a moderate-finesse cavity can overcome these losses. As the scattering losses peak at certain discrete values of the lattice spacing, the spacing can be optimized to achieve efficient atom-photon coupling in the cavity. Our cavity-QED theory properly accounts for collective dipolar interactions mediated by the lossy, non-cavity-confined photon modes and for finite-size effects of both the array and the light field. These findings pave the way to harnessing the versatility of tweezer arrays for efficient atom-photon interfaces in applications of quantum computing, networking, and nonlinear optics. Published by the American Physical Society 2024