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arXiv:2103.02416 · Applied Physics Letters

Nanoscale continuous quantum light sources based on driven dipole emitter arrays

Raphael Holzinger, Maria Moreno-Cardoner, Helmut Ritsch

Published Jul 12, 2021• 29 citations
arXivHTMLPDF

Abstract

Regular arrays of two-level emitters at distances smaller than that of the transition wavelength collectively scatter, absorb, and emit photons. The strong inter-particle dipole coupling creates large energy shifts of the collective delocalized excitations, which generates a highly nonlinear response at the single and few photon level. This should allow us to implement nanoscale non-classical light sources via weak coherent illumination. At the generic tailored examples of regular chains or polygons, we show that the fields emitted perpendicular to the illumination direction exhibit a strong directional confinement with genuine quantum properties as antibunching. For short interparticle distances, superradiant directional emission can enhance the radiated intensity by an order of magnitude compared to a single atom focused to a strongly confined solid angle but still keeping the anti-bunching parameter at the level of g(2)(0)≈10−2.

DOI
10.1063/5.0049270

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Regular arrays of two-level emitters at distances smaller than that of the transition wavelength collectively scatter, absorb, and emit photons. The strong inter-particle dipole coupling creates large energy shifts of the collective delocalized excitations, which generates a highly nonlinear response at the single and few photon level. This should allow us to implement nanoscale non-classical light sources via weak coherent illumination. At the generic tailored examples of regular chains or polygons, we show that the fields emitted perpendicular to the illumination direction exhibit a strong directional confinement with genuine quantum properties as antibunching. For short interparticle distances, superradiant directional emission can enhance the radiated intensity by an order of magnitude compared to a single atom focused to a strongly confined solid angle but still keeping the anti-bunching parameter at the level of g(2)(0)≈10−2.
Subwavelength arrays of quantum emitters feature unique and largely design-able nonlinear optical properties. As a generic example we study a sub-wavelength sized ring of identical dipoles with an extra identical absorbing emitter at the center. For a 9-ring one finds the most efficient antenna configuration to direct single incoming photons to the center without re-emission. Interestingly, for very tiny structures sizes below a tenth of a wavelength, a full quantum description predicts an even larger absorption enhancement than a mean field model using a classical dipole approximation. We identify the origin of the enhancement in the appearance of a collective dark state with dominant center occupation. By special design of the center absorber one thus can harness the same efficiency enhancement also at different wavelengths and for other geometric structures. On the one hand this idea could be the basis of a new generation of highly efficient and selective nano antennas, while on the other hand, it could be an important piece towards understanding the surprising efficiency of natural light harvesting molecules. Adding gain via active dipoles in such nano ring systems allows to design minimalist laser like classical light sources. In the nonlinear operating regime at stronger pump fields these systems transform to non-classical light sources with tailor-able spatio-temporal emission upon coherent illumination.
A ring of dipole-coupled quantum emitters positioned at subwavelength distances possesses only a few radiant but many subradiant collective excitations with lifetimes growing exponentially with the atom number. These exhibit a three-dimensionally confined spatial radiation field pattern and form nanoscale high-QQQ optical resonators. Tailoring size, orientation, and distance between two rings allows for increasing the ratio of coherent ring-to-ring energy transfer versus free-space emission by orders of magnitude. In particular, the more dark and delocalized over several sites are excitons, the higher is their fidelity for transport to a second ring.
Collective excitations in regular structures of strongly interacting driven dipoles have been found to lead to strongly antibunched statistics of the emitted photons $[{g}^{(2)}(0)\ensuremath{\ll}0.5]$, but precise control of the number of emitters and their spatial distribution is in general a complex experimental task. We overcome this limitation by showing quantum light emission from densely packed driven dipoles does not require their arrangement in any specific structure, pointing strongly towards possible single-photon sources based on hot thermal vapors confined within nanocells, or on irregular quantum dot ensembles.
We predict collective free-space lasing in a dense nanoscopic emitter arrangement where dipole-dipole coupled atomic emitters synchronize their emission and exhibit lasing behavior without the need for an optical resonator. At the example of a subwavelength-spaced linear emitter chain with varying fractions of pumped and unpumped emitters, we present a comprehensive study of this mirrorless lasing phenomenon. The total radiated power transitions from subradiant suppression under weak pumping to superradiant enhancement at stronger pumping, while exhibiting directional emission confined to a narrow spatial angle. At the same time multiple independent spectral emission lines below the lasing threshold merge toward a single narrow spectral line at high pump power. The most substantial enhancement and line narrowing occur when a fraction of unpumped atoms is present. We show that this leads to superradiant lasing near the bare atomic frequency, making the system a promising candidate for a minimalist active optical frequency reference.
Recent experimental advances in preparing regular defect-free 2D arrays of atoms with optical traps have offered new opportunities to engineer strong collective couplings between light and atoms as quantum optical dipoles. Applications of such collective light-matter interactions include the realization of atom-thick mirrors, retrieval of quantum memories with high efficiency, or the implementation of topological quantum optics. I will present novel applications in the context of quantum networking. First, I will discuss the design of a chiral photonic quantum link, where distant single atoms interact by exchanging photons propagating in a unique direction in free space. This is achieved by coupling both single atoms, representing qubits implemented using a pair of Rydberg states, to bi-layer atomic arrays which act as quantum phased-array antennas. Exploiting the combination of a “Rydberg-dressing” laser and a control laser driving the atomic arrays, an effective Rydberg dipole-dipole interaction can be engineered between atoms and atomic arrays as quantum emitters, allowing to match the spatial modes of spontaneously emitted and absorbed photons to a Gaussian mode of interest. In this way, we realize a chiral quantum interface, i.e., where atoms couple to photonic modes with a unique direction of propagation. This setup provides a basic building block of a novel platform for quantum networks in free space, i.e., without requiring coupling atoms to modes of cavities or nanostructures, which I will illustrate with the deterministic coherent transfer of quantum states between single atoms with high fidelity. Second, I will discuss the collective radiation properties of two distant single-layer atomic arrays acting as quantum memories. This system can support a long-lived non-local superposition state of atomic excitations exhibiting strong subradiance. This “dark” mode consists of an atomic excitation which is delocalized between the two distant atomic arrays, in such a way that the overall radiation is strongly suppressed by quantum interference. I will describe the preparation of these states and their application as resource of non-local entanglement. In particular, by weakly driving the arrays, the state of the quantum memories, localized in each array, can be transferred to this “non-local” subradiant state, allowing again for a deterministic coherent quantum state transfer with high fidelity between the memories. Finally, I will discuss experimental realizations using cold atoms in optical trap arrays, and the effect of experimental imperfections in the arrays, such as finite defect probability, temperature, and depth of the optical traps.
We examine angular distribution of the probability of correlated fluorescence photon emission from a linear chain of identical equidistant two-level atoms. We selectively excite one of the atoms by a resonant laser field. The atoms are coupled to each other via the dipole-dipole interaction and collective spontaneous emission. Our attention is focused on the simultaneous observation of correlated pairs of photons. It is found that the interference between the emitting atoms can result in a highly directional emission of photon pairs. These pairs of photons exhibit strong correlations and their emission is highly concentrated into specific directions. We demonstrate the crucial role of the selective coherent excitation in such a geometrical configuration. Shifting the driving field from an atom located at one end of the chain to the other causes the radiation pattern to flip to the opposite half of the detection plane. Furthermore, we find that atomic systems in which only an atom situated at a particular position within the linear chain is driven by a laser field can radiate correlated twin photons in directions along which the radiation of single photons is significantly reduced. Alternatively, superbunching in the emitted photon statistics preferentially occurs in directions of negligible or vanishing single-photon emission. The effect of superbunching strengthens as more emitters are added to the chain. Depending on the number of atoms and the position of the driven atom within the chain, the strongly correlated pairs of photons can be emitted into few well-defined directions.