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arXiv:1912.08065 · OSA Continuum

Absolute frequency measurements of the 1S0 → 1P1 transition in ytterbium

T. Lauprêtre, Lucas Groult, Bachir Achi, Michael Petersen, Y. Kersalé, Marion Delehaye, Clément Lacroûte

Published Jan 9, 2020• 9 citations
arXivHTMLPDF

Abstract

The ytterbium atom is widely used in the fields of atomic physics, cavity quantum electrodynamics, quantum information processing, and optical frequency standards. There is however a strong dispersion among the reported values of the 1S0 → 1P1 transition frequency. In this article, we present two independent measurements of the absolute frequency of this transition performed with two different wavemeters using atomic fluorescence spectroscopy. The cancellation of Doppler shifts is obtained by fine tuning the angle between the probe laser and the atomic beam. The resulting 174Yb isotope transition frequency is estimated to be 751 526 537 ± 27 MHz.

DOI
10.1364/osac.3.000050

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The ytterbium atom is widely used in the fields of atomic physics, cavity quantum electrodynamics, quantum information processing, and optical frequency standards. There is however a strong dispersion among the reported values of the 1S0 → 1P1 transition frequency. In this article, we present two independent measurements of the absolute frequency of this transition performed with two different wavemeters using atomic fluorescence spectroscopy. The cancellation of Doppler shifts is obtained by fine tuning the angle between the probe laser and the atomic beam. The resulting 174Yb isotope transition frequency is estimated to be 751 526 537 ± 27 MHz.
We demonstrate a simple technique to measure the resonant frequency of the 398.9-nm ${}^{1}{S}_{0}\ensuremath{\leftrightarrow}{}^{1}{P}_{1}$ transition for the different Yb isotopes. The technique, which works by observing and aligning fluorescence spots, has enabled us to measure transition frequencies and isotope shifts with an accuracy of 60 MHz. We provide wavelength measurements for the transition that differ from previously published work. Our technique also allows for the determination of Doppler-shifted transition frequencies for photoionization experiments when the atomic beam and the laser beam are not perpendicular and furthermore allows us to determine the average velocity of the atoms along the direction of the atomic beam.
We report the experimental results on measuring the isotope shifts and hyperfine splittings of all ytterbium isotopes for a 399-nm transition by using a quite simple and novel method. It benefits from the advantages of the modulation transfer spectroscopy in an ytterbium hollow cathode lamp and the Doppler-free spectroscopy in a collimated ytterbium atomic beam. The key technique in this experiment is simultaneously measuring the frequency separations of the two spectra twice, and the separation difference between two measurements is solely determined by the well-defined frequency of an acousto-optics modulator. Compared with the most of previously reported experimental results, ours are more accurate and completed, which will provide the useful information for developing a more accurate theoretical model to describe the interaction inside an ytterbium atom.
We report the direct excitation of the highly forbidden (6s2) 1S0 <--> (6s6p) 3P0 optical transition in two odd isotopes of neutral ytterbium. As the excitation laser frequency is scanned, absorption is detected by monitoring the depletion from an atomic cloud at approximately 70 microK in a magneto-optical trap. The measured frequency in 171Yb (F=1/2) is 518,295,836,591.6 +/- 4.4 kHz. The measured frequency in 173Yb (F=5/2) is 518,294,576,847.6 +/- 4.4 kHz. Measurements are made with a femtosecond-laser frequency comb calibrated by the National Institute of Standards and Technology cesium fountain clock and represent nearly a 10(6)-fold reduction in uncertainty. The natural linewidth of these J=0 to J=0 transitions is calculated to be approximately 10 mHz, making them well suited to support a new generation of optical atomic clocks based on confinement in an optical lattice.
Optical frequency measurements of the intercombination line $(6{s}^{2})\phantom{\rule{0.16em}{0ex}}^{1}S_{0}\ensuremath{-}(6s6p)\phantom{\rule{0.16em}{0ex}}^{3}P_{1}$ in the isotopes of ytterbium are carried out with the use of sub-Doppler fluorescence spectroscopy on an atomic beam. A dispersive signal is generated to which a master laser is locked, while frequency counting of an auxiliary beat signal is performed via a frequency comb referenced to a hydrogen maser. The relative separations between the lines are used to evaluate the 3P1^{3}P_{1}3P1​-level magnetic dipole and electric quadrupole constants for the fermionic isotopes. The center of gravity for the 3P1^{3}P_{1}3P1​ levels in 171Yb^{171}\mathrm{Yb}171Yb and 173Yb^{173}\mathrm{Yb}173Yb are also evaluated, where we find significant disagreement with previously reported values. These hyperfine constants provide a valuable testbed for atomic many-body computations in ytterbium.
The narrow linewidth of1S0-3P1657 nm clock transition makes it a promising quantum frequency reference. In this experiment, the fast1S0-1P1423 nm transition is used to detect the narrow1S0-3P1657 nm clock transition. Therefore, the frequency stability of the 423 nm laser determines the performance of the optical frequency standard. Here we investigate the frequency shift properties of the neutral calcium atoms'1S0-1P1transition at 423 nm. We measure the frequency shift caused by temperature, laser power, and laser beam pointing.
This work has focused on two atoms, Sr and Yb, due in part to the relatively high abundance of their odd isotopes, the use of which is necessary for appreciable direct excitation probability. The Sr clock transition has been measured (with an uncertainty of 20 kHz) using atoms in a magneto-optic trap (MOT), and has been excited with atoms confined in a one dimensional lattice. Here we report direct excitation of the Yb clock transition (at 578 nm) with atoms in a second-stage MOT, and the first fs-laser comb-based absolute measurements of the clock frequency for two different isotopes. These measurements lead to a nearly millionfold improvement in our knowledge of the transition frequencies, an important step toward Doppler-free spectroscopy of Yb atoms in a lattice.