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arXiv:1909.01475 · Physical review. B./Physical review. B

Critical role of the sign structure in the doped Mott insulator: Luther-Emery versus Fermi-liquid-like state in quasi-one-dimensional ladders

Hong‐Chen Jiang, Shuai A. Chen, Zheng-Yu Weng

Published Sep 25, 2020• 25 citations
arXivHTMLPDF

Abstract

The mechanism of superconductivity in a purely interacting electron system has been one of the most challenging issues in condensed matter physics. In the BCS theory, the Landau's Fermi liquid is the ground state of weakly interacting fermions dictated by the fermion sign structure, and the superconducting instability only occurs when an additional pairing force is added. By contrast, as shown by density matrix renormalization group calculation, a quasi-one-dimensional superconducting state (specifically a Luther-Emery state) is an intrinsic ground state of the $t\ensuremath{-}J$ two-leg ladder and four-leg cylinder at finite doping. Such a Luther-Emery state with pairing can be directly turned into a Fermi-gas-like normal state without pairing by merely switching off the phase-string signs hidden in the model via two schemes, which reduce the sign structure to the trivial fermion signs associated with doped holes. It thus demonstrates a new pairing paradigm in a model-doped Mott insulator as due to the generic phase-string sign structure. Finally, as an example, the latter is explicitly shown to lead to a ``stringlike'' pairing force after adiabatically connecting to a strong anisotropic limit of the model.

DOI
10.1103/physrevb.102.104512

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The mechanism of superconductivity in a purely interacting electron system has been one of the most challenging issues in condensed matter physics. In the BCS theory, the Landau's Fermi liquid is the ground state of weakly interacting fermions dictated by the fermion sign structure, and the superconducting instability only occurs when an additional pairing force is added. By contrast, as shown by density matrix renormalization group calculation, a quasi-one-dimensional superconducting state (specifically a Luther-Emery state) is an intrinsic ground state of the t\ensuremath−Jt\ensuremath{-}Jt\ensuremath−J two-leg ladder and four-leg cylinder at finite doping. Such a Luther-Emery state with pairing can be directly turned into a Fermi-gas-like normal state without pairing by merely switching off the phase-string signs hidden in the model via two schemes, which reduce the sign structure to the trivial fermion signs associated with doped holes. It thus demonstrates a new pairing paradigm in a model-doped Mott insulator as due to the generic phase-string sign structure. Finally, as an example, the latter is explicitly shown to lead to a ``stringlike'' pairing force after adiabatically connecting to a strong anisotropic limit of the model.
Understanding the doped Mott insulator is a central challenge in condensed matter physics. In this work, we first explicitly identify a new sign structure in the $t\text{\ensuremath{-}}{t}^{\ensuremath{'}}\text{\ensuremath{-}}J$ model on the square lattice that replaces the conventional Fermi statistics for weakly interacting electrons. Then we show that the singular, i.e., the phase-string part of the sign structure in the partition function can be precisely turned off in a modified model. The density matrix renormalization group method is then employed to study these two models comparatively on finite-size systems, which is designed to unveil the consequences of the phase-string component. We find that the hole pairing is present not only in the quasi-long-range superconducting phase but also in the stripe phase of the $t\text{\ensuremath{-}}{t}^{\ensuremath{'}}\text{\ensuremath{-}}J$ model. However, once the phase-string is switched off, both the superconducting and stripe orders together with the underlying hole pairing disappear. The corresponding ground state reduces to a trivial Fermi-liquid-like state with small hole Fermi pockets that is decoupled from the antiferromagnetic spin background. It is in sharp contrast to the original $t\text{\ensuremath{-}}{t}^{\ensuremath{'}}\text{\ensuremath{-}}J$ model where large Fermi surfaces can be restored in the stripe phase found at ${t}^{\ensuremath{'}}/t<0$ or the superconducting phase at ${t}^{\ensuremath{'}}/t>0$ in the six-leg ladder calculation. Our study clearly demonstrates that the strong correlation effect in doped Mott insulator should be mainly attributed to the long-range quantum entanglement between the spin and charge, which is, nonperturbatively, beyond a simple spin-charge separation under the no double occupancy constraint.
How the ground-state nature can be dramatically changed by the distinct underlying spin correlation is a central issue of doped Mott insulators.The two-leg XXZ ladder provides a prototypical spin background, which can be tuned from a long-range Néel order to a short-range spin liquid via the superexchange anisotropy, giving rise to a complex phase diagram at finite doping.By density matrix renormalization group method, we show that although the charge is always self-localized in the Néel ordered phase, a second insulating phase emerges in which the doped holes become paired but remain localized while the transverse spin-spin correlation reduces to short-ranged one to make the Néel order classical.Only when the Néel order totally disappears by further reducing anisotropy does the pairing become truly coherent as characterized by a Luther-Emery state.In sharp contrast, the pairing is totally absent in the in-plane ferromagnetic XXZ regime, where a direct transition from the charge self-localization in the Néel ordered phase to a Fermi-gas-like state in the spin liquid phase is found.A consistent physical picture is briefly discussed.
Cooper pairing instability in a Fermi liquid is well understood by the BCS theory, but pairing mechanism for doped Mott insulators still remains elusive. Previously it has been shown by density matrix renormalization group (DMRG) method that a single doped hole is always self-localized due to the quantum destructive interference of the phase string signs hidden in the t-J ladders. Here we report a DMRG investigation of hole binding in the same model, where a novel pairing-glue scheme beyond the BCS realm is discovered. Specifically, we show that, in addition to spin pairing due to superexchange interaction, the strong frustration of the phase string signs on the kinetic energy gets effectively removed by pairing the charges, which results in strong binding of two holes. By contrast, if the phase string signs are "switched off" artificially, the pairing strength diminishes significantly even if the superexchange coupling remains the same. In the latter, unpaired holes behave like coherent quasiparticles with pairing drastically weakened, whose sole origin may be attributed to the resonating-valence-bond (RVB) pairing of spins. Such non-BCS pairing mechanism is therefore beyond the RVB picture and may shed important light on the high-T(c) cuprate superconductors.
Motivated by recent experiments on ultracold fermionic spin-1/2 6^66Li atoms in a Lieb lattice at various Hubbard repulsion UUU and filling fractions nnn (Lebrat et al., arXiv:2404.17555), we conduct a density matrix renormalization group (DMRG) analysis of the Hubbard model on a two-leg Lieb ladder. At half-filling, we find a ferrimagnetic Mott insulating ground state, consistent with Lieb's theorem. Away from half-filling, a state with finite total spin S⃗2≠0\vec{S}^2 \neq 0S2=0 and vanishing charge gap persists down to filling nc≈2/3n_c \approx 2/3nc​≈2/3. For lower, incommensurate fillings, the system is described by a Luttinger liquid with one charge and one spin mode. Intriguingly, in a narrow window near nc=2/3n_c = 2/3nc​=2/3, close to the onset of ferromagnetic order, we identify a superconducting Luther-Emery phase with dominant sxys_{xy}sxy​-wave pairing.
A lightly doped single-band Hubbard model on a two-leg ladder exhibits a Luther-Emery phase, whereas the three-band Hubbard ladder behaves as a Luttinger liquid upon hole doping. To understand this discrepancy, we present a systematic density-matrix renormalization group study of the three-band Hubbard model on two-leg cylinders with further-neighbor particle hoppings. The inclusion of the longer-range hopping is motivated by the studies of the single-band Hubbard model in which the further-neighbor hopping terms are suggested to be crucial for the unconventional superconductivity. When the longer-range hopping parameters are small, the ground state is a Luttinger liquid having mutually commensurate superconducting, charge, and spin density wave correlations. Increasing the longer-range hopping drives a transition into a Luther-Emery phase with quasi-long-ranged superconducting and charge orders but short-ranged spin-spin correlations. By down-folding the three-band Hubbard model into an effective $t\text{\ensuremath{-}}{t}^{\ensuremath{'}}\text{\ensuremath{-}}J\text{\ensuremath{-}}{J}^{\ensuremath{'}}$ model, we find that in the Luther-Emery phase, both the nearest- and second-neighbor kinetic energies are enhanced due to an effective increase of copper-oxygen hybridization. Amplifying intercell oxygen orbital hopping mirrors the benefits of reducing the charge transfer energy, causing doped holes to favor oxygen orbitals and strengthening superconducting pairing.
We investigate the pairing tendencies in the hole-doped Haldane spin-1 chain. To allow for doping, we extend the original spin chain Hamiltonian into a fermionic model involving a two-orbital Hubbard chain at intermediate or strong repulsive interaction strengths UUU and for degenerate orbitals. At half filling and large UUU, the ferromagnetic Hund's coupling, JH{J}_{\mathrm{H}}JH​, generates effective spin-1 moments, with antiferromagnetic correlations between sites. Using large-scale density matrix renormalization group calculations, we accurately study the system's behavior under light hole-doping. For U=1.6U=1.6U=1.6 in units of the noninteracting bandwidth and for ${J}_{\mathrm{H}}/U\ensuremath{\gtrsim}0.275$, we find that singlet pairing dominates the long-distance physics, establishing this system as a promising platform for repulsively mediated superconductivity. We provide concrete examples of materials that could realize the physics described here. We also provide evidence that the system approaches a Luther-Emery liquid state at large system sizes, reminiscent of the behavior of doped one-orbital two-leg ladders at weak coupling, which also have superconducting tendencies. The numerically calculated central charge approaches one in the thermodynamic limit, indicating a single gapless mode as is expected for the Luther-Emery state. Exponents characterizing the power-law decays of singlet pair-pair and charge density-density correlations are determined, and found to approximately satisfy the Luther-Emery identity.