arXiv:2311.13440 · Physical review. B./Physical review. B

Luther-Emery liquid and dominant singlet superconductivity in the hole-doped Haldane spin-1 chain

Pontus Laurell, J. Herbrych, Gonzalo Álvarez, Elbio R. Dagotto

Published Aug 26, 2024• 5 citations

Abstract

We investigate the pairing tendencies in the hole-doped Haldane spin-1 chain. To allow for doping, we extend the original spin chain Hamiltonian into a fermionic model involving a two-orbital Hubbard chain at intermediate or strong repulsive interaction strengths $U$ and for degenerate orbitals. At half filling and large $U$, the ferromagnetic Hund's coupling, ${J}_{\mathrm{H}}$, generates effective spin-1 moments, with antiferromagnetic correlations between sites. Using large-scale density matrix renormalization group calculations, we accurately study the system's behavior under light hole-doping. For $U=1.6$ in units of the noninteracting bandwidth and for ${J}_{\mathrm{H}}/U\ensuremath{\gtrsim}0.275$, we find that singlet pairing dominates the long-distance physics, establishing this system as a promising platform for repulsively mediated superconductivity. We provide concrete examples of materials that could realize the physics described here. We also provide evidence that the system approaches a Luther-Emery liquid state at large system sizes, reminiscent of the behavior of doped one-orbital two-leg ladders at weak coupling, which also have superconducting tendencies. The numerically calculated central charge approaches one in the thermodynamic limit, indicating a single gapless mode as is expected for the Luther-Emery state. Exponents characterizing the power-law decays of singlet pair-pair and charge density-density correlations are determined, and found to approximately satisfy the Luther-Emery identity.

DOI: 10.1103/physrevb.110.064515

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arXiv:2311.13440 · Physical review. B./Physical review. B

Luther-Emery liquid and dominant singlet superconductivity in the hole-doped Haldane spin-1 chain

Pontus Laurell, J. Herbrych, Gonzalo Álvarez, Elbio R. Dagotto

Published Aug 26, 2024• 5 citations

arXiv HTML PDF

Abstract

U

and for degenerate orbitals. At half filling and large

U

, the ferromagnetic Hund's coupling,

{J}_{\mathrm{H}}

, generates effective spin-1 moments, with antiferromagnetic correlations between sites. Using large-scale density matrix renormalization group calculations, we accurately study the system's behavior under light hole-doping. For

U=1.6

in units of the noninteracting bandwidth and for

{J}_{\mathrm{H}}/U\ensuremath{\gtrsim}0.275

, we find that singlet pairing dominates the long-distance physics, establishing this system as a promising platform for repulsively mediated superconductivity. We provide concrete examples of materials that could realize the physics described here. We also provide evidence that the system approaches a Luther-Emery liquid state at large system sizes, reminiscent of the behavior of doped one-orbital two-leg ladders at weak coupling, which also have superconducting tendencies. The numerically calculated central charge approaches one in the thermodynamic limit, indicating a single gapless mode as is expected for the Luther-Emery state. Exponents characterizing the power-law decays of singlet pair-pair and charge density-density correlations are determined, and found to approximately satisfy the Luther-Emery identity.

DOI: 10.1103/physrevb.110.064515

Related papers

Pairing tendencies in a two-orbital Hubbard model in one dimension

N. D. Patel, Alberto Nocera, Gonzalo Álvarez +2 more

The recent discovery of superconductivity under high pressure in the ladder compound ${\mathrm{BaFe}}_{2}{\mathrm{S}}_{3}$ has opened a new field of research in iron-based superconductors with focus on quasi-one-dimensional geometries. In this publication, using the density matrix renormalization group technique, we study a two-orbital Hubbard model defined in one-dimensional chains. Our main result is the presence of hole binding tendencies at intermediate Hubbard $U$ repulsion and robust Hund coupling ${J}_{H}/U=0.25$ . Binding does not occur either in weak coupling or at very strong coupling. The pair-pair correlations that are dominant near half-filling, or of similar strength as the charge and spin correlation channels, involve hole-pair operators that are spin singlets, use nearest-neighbor sites, and employ different orbitals for each hole. The Hund coupling strength, presence of robust magnetic moments, and antiferromagnetic correlations among them are important for the binding tendencies found here.The recent discovery of superconductivity under high pressure in the ladder compound ${\mathrm{BaFe}}_{2}{\mathrm{S}}_{3}$ has opened a new field of research in iron-based superconductors with focus on quasi-one-dimensional geometries. In this publication, using the density matrix renormalization group technique, we study a two-orbital Hubbard model defined in one-dimensional chains. Our main result is the presence of hole binding tendencies at intermediate Hubbard $U$ repulsion and robust Hund coupling ${J}_{H}/U=0.25$. Binding does not occur either in weak coupling or at very strong coupling. The pair-pair correlations that are dominant near half-filling, or of similar strength as the charge and spin correlation channels, involve hole-pair operators that are spin singlets, use nearest-neighbor sites, and employ different orbitals for each hole. The Hund coupling strength, presence of robust magnetic moments, and antiferromagnetic correlations among them are important for the binding tendencies found here.

arXiv:1705.08780Physical review. B./Physical review. BJul 31, 201730 citations

Doped Two Orbital Chains with Strong Hund's Rule Couplings - Ferromagnetism, Spin Gap, Singlet and Triplet Pairings

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Different models for doping of two-orbital chains with mobile $S=1/2$ fermions and strong, ferromagnetic (FM) Hund's rule couplings stabilizing the S=1 spins are investigated by density matrix renormalization group (DMRG) methods. The competition between antiferromagnetic (AF) and FM order leads to a rich phase diagram with a narrow FM region for weak AF couplings and strongly enhanced triplet pairing correlations. Without a level difference between the orbitals, the spin gap persists upon doping, whereas gapless spin excitations are generated by interactions among itinerant polarons in the presence of a level difference. In the charge sector we find dominant singlet pairing correlations without a level difference, whereas upon the inclusion of a Coulomb repulsion between the orbitals or with a level difference, charge density wave (CDW) correlations decay slowest. The string correlation functions remain finite upon doping for all models.Different models for doping of two-orbital chains with mobile $S=1/2$ fermions and strong, ferromagnetic (FM) Hund's rule couplings stabilizing the S=1 spins are investigated by density matrix renormalization group (DMRG) methods. The competition between antiferromagnetic (AF) and FM order leads to a rich phase diagram with a narrow FM region for weak AF couplings and strongly enhanced triplet pairing correlations. Without a level difference between the orbitals, the spin gap persists upon doping, whereas gapless spin excitations are generated by interactions among itinerant polarons in the presence of a level difference. In the charge sector we find dominant singlet pairing correlations without a level difference, whereas upon the inclusion of a Coulomb repulsion between the orbitals or with a level difference, charge density wave (CDW) correlations decay slowest. The string correlation functions remain finite upon doping for all models.

arXiv:cond-mat/0006439Journal of the Physical Society of JapanFeb 15, 200110 citations

Pair-density-wave superconductor from doping Haldane chain and rung-singlet ladder

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We report the numerical discovery of a Luther-Emery liquid with pair-density-wave (PDW) correlations from doping either (i) a spin-one Haldane chain or (ii) a two-leg ladder in the rung-singlet phase in which the doped charges occupy a single leg. We model these systems using a generalized Kondo model. The itinerant electrons are correlated and described by the $t\text{\ensuremath{-}}J$ model, and are further coupled to a spin- $1/2$ Heisenberg model through the Kondo coupling ${J}_{K}$ . When the density of electrons $x$ is one, the Mott insulator is in a Haldane phase or in a rung-singlet phase depending on whether ${J}_{K}$ is negative or positive. Upon doping, a pair-density-wave with $\mathbf{Q}=\ensuremath{\pi}$ can emerge for both signs of ${J}_{K}$ . In the ${J}_{K}\ensuremath{\rightarrow}\ensuremath{-}\ensuremath{\infty}$ limit, the model reduces to the recently proposed type II $t\ensuremath{-}J$ model. We also identify a composite order parameter for the superconductor, which can be understood as a Cooper pair formed by two nearby fermionic spin-polarons. Our model and the predicted PDW phase can be experimentally realized by doping $S=1$ chains formed by ${\mathrm{Ni}}^{2+}$ in a solid-state system or a two-leg ladder of fermionic cold atoms with a potential bias between legs, which preferentially dopes carriers into a single leg. Long-range order of the PDW can be achieved in quasi-one-dimensional system with finite interwire coupling.We report the numerical discovery of a Luther-Emery liquid with pair-density-wave (PDW) correlations from doping either (i) a spin-one Haldane chain or (ii) a two-leg ladder in the rung-singlet phase in which the doped charges occupy a single leg. We model these systems using a generalized Kondo model. The itinerant electrons are correlated and described by the $t\text{\ensuremath{-}}J$ model, and are further coupled to a spin-$1/2$ Heisenberg model through the Kondo coupling ${J}_{K}$. When the density of electrons $x$ is one, the Mott insulator is in a Haldane phase or in a rung-singlet phase depending on whether ${J}_{K}$ is negative or positive. Upon doping, a pair-density-wave with $\mathbf{Q}=\ensuremath{\pi}$ can emerge for both signs of ${J}_{K}$. In the ${J}_{K}\ensuremath{\rightarrow}\ensuremath{-}\ensuremath{\infty}$ limit, the model reduces to the recently proposed type II $t\ensuremath{-}J$ model. We also identify a composite order parameter for the superconductor, which can be understood as a Cooper pair formed by two nearby fermionic spin-polarons. Our model and the predicted PDW phase can be experimentally realized by doping $S=1$ chains formed by ${\mathrm{Ni}}^{2+}$ in a solid-state system or a two-leg ladder of fermionic cold atoms with a potential bias between legs, which preferentially dopes carriers into a single leg. Long-range order of the PDW can be achieved in quasi-one-dimensional system with finite interwire coupling.

arXiv:2202.01224Physical review. B./Physical review. BJul 5, 202224 citations

Absence of Luther-Emery superconducting phase in the three-band model for cuprate ladders

Jeong-Pil Song, S. Mazumdar, Rudolf Torsten Clay

Correlated-electron theories of superconductivity in layered cuprates often start from the premise of a gapped spin-liquid phase proximate to the superconducting state. This assumption is justified based on analytical and numerical demonstrations of a superconducting Luther-Emery phase in the doped 2-leg one-band Hubbard ladder, and the perceived analogy between coupled ladders and the two-dimensional ${\mathrm{CuO}}_{2}$ layer. We demonstrate from accurate density matrix renormalization group studies the absence of the superconducting Luther-Emery phase in the doped 2-leg three-band ladder consisting of both copper and oxygen, even as the spin gap is large in the undoped three-band ladder. For realistic oxygen-oxygen hopping and Hubbard repulsion on the oxygen atoms, density-density rather than pairing correlations are dominant at long range. This result is equally valid whether or not the oxygens outside the ladder proper, over and above the rung and leg oxygens, are included in the computation. These results demonstrate the critical importance of oxygen orbitals, and raise disturbing questions about the applicability of many of the existing correlated-electron theories of superconductivity.Correlated-electron theories of superconductivity in layered cuprates often start from the premise of a gapped spin-liquid phase proximate to the superconducting state. This assumption is justified based on analytical and numerical demonstrations of a superconducting Luther-Emery phase in the doped 2-leg one-band Hubbard ladder, and the perceived analogy between coupled ladders and the two-dimensional ${\mathrm{CuO}}_{2}$ layer. We demonstrate from accurate density matrix renormalization group studies the absence of the superconducting Luther-Emery phase in the doped 2-leg three-band ladder consisting of both copper and oxygen, even as the spin gap is large in the undoped three-band ladder. For realistic oxygen-oxygen hopping and Hubbard repulsion on the oxygen atoms, density-density rather than pairing correlations are dominant at long range. This result is equally valid whether or not the oxygens outside the ladder proper, over and above the rung and leg oxygens, are included in the computation. These results demonstrate the critical importance of oxygen orbitals, and raise disturbing questions about the applicability of many of the existing correlated-electron theories of superconductivity.

arXiv:2010.10609Physical review. B./Physical review. BSep 13, 20219 citations

Recovery of a Luther-Emery phase in the three-band Hubbard ladder with longer-range hopping

Luhang Yang, Thomas Devereaux, Hong‐Chen Jiang

A lightly doped single-band Hubbard model on a two-leg ladder exhibits a Luther-Emery phase, whereas the three-band Hubbard ladder behaves as a Luttinger liquid upon hole doping. To understand this discrepancy, we present a systematic density-matrix renormalization group study of the three-band Hubbard model on two-leg cylinders with further-neighbor particle hoppings. The inclusion of the longer-range hopping is motivated by the studies of the single-band Hubbard model in which the further-neighbor hopping terms are suggested to be crucial for the unconventional superconductivity. When the longer-range hopping parameters are small, the ground state is a Luttinger liquid having mutually commensurate superconducting, charge, and spin density wave correlations. Increasing the longer-range hopping drives a transition into a Luther-Emery phase with quasi-long-ranged superconducting and charge orders but short-ranged spin-spin correlations. By down-folding the three-band Hubbard model into an effective $t\text{\ensuremath{-}}{t}^{\ensuremath{'}}\text{\ensuremath{-}}J\text{\ensuremath{-}}{J}^{\ensuremath{'}}$ model, we find that in the Luther-Emery phase, both the nearest- and second-neighbor kinetic energies are enhanced due to an effective increase of copper-oxygen hybridization. Amplifying intercell oxygen orbital hopping mirrors the benefits of reducing the charge transfer energy, causing doped holes to favor oxygen orbitals and strengthening superconducting pairing.A lightly doped single-band Hubbard model on a two-leg ladder exhibits a Luther-Emery phase, whereas the three-band Hubbard ladder behaves as a Luttinger liquid upon hole doping. To understand this discrepancy, we present a systematic density-matrix renormalization group study of the three-band Hubbard model on two-leg cylinders with further-neighbor particle hoppings. The inclusion of the longer-range hopping is motivated by the studies of the single-band Hubbard model in which the further-neighbor hopping terms are suggested to be crucial for the unconventional superconductivity. When the longer-range hopping parameters are small, the ground state is a Luttinger liquid having mutually commensurate superconducting, charge, and spin density wave correlations. Increasing the longer-range hopping drives a transition into a Luther-Emery phase with quasi-long-ranged superconducting and charge orders but short-ranged spin-spin correlations. By down-folding the three-band Hubbard model into an effective $t\text{\ensuremath{-}}{t}^{\ensuremath{'}}\text{\ensuremath{-}}J\text{\ensuremath{-}}{J}^{\ensuremath{'}}$ model, we find that in the Luther-Emery phase, both the nearest- and second-neighbor kinetic energies are enhanced due to an effective increase of copper-oxygen hybridization. Amplifying intercell oxygen orbital hopping mirrors the benefits of reducing the charge transfer energy, causing doped holes to favor oxygen orbitals and strengthening superconducting pairing.

Physical review. B./Physical review. BJul 15, 20247 citations

Absence of Luther-Emery Phase in the Three-Band Model for Cuprate Ladders

Jeong-Pil Song, S. Mazumdar, Rudolf Torsten Clay

Correlated-electron theories of superconductivity in cuprates often start from the premise of a gapped spin-liquid phase proximate to the superconducting state. This assumption is based on, (i) demonstrations of a Luther-Emery phase with dominant superconducting correlations in the doped 2-leg one-band Hubbard ladder, and (ii) the perceived analogy between coupled ladders and the square lattice. We demonstrate from accurate density matrix renormalization group calculations the absence of the Luther-Emery phase in the doped 2-leg three-band ladder consisting of both copper and oxygen. For realistic oxygen-oxygen hopping and Hubbard repulsion on the oxygen atoms, the decay of the superconducting pair correlation with distance is almost indistinguishable from that of free fermions. Our results caste severe doubts on many of the existing correlated-electron theories of superconductivity.Correlated-electron theories of superconductivity in cuprates often start from the premise of a gapped spin-liquid phase proximate to the superconducting state. This assumption is based on, (i) demonstrations of a Luther-Emery phase with dominant superconducting correlations in the doped 2-leg one-band Hubbard ladder, and (ii) the perceived analogy between coupled ladders and the square lattice. We demonstrate from accurate density matrix renormalization group calculations the absence of the Luther-Emery phase in the doped 2-leg three-band ladder consisting of both copper and oxygen. For realistic oxygen-oxygen hopping and Hubbard repulsion on the oxygen atoms, the decay of the superconducting pair correlation with distance is almost indistinguishable from that of free fermions. Our results caste severe doubts on many of the existing correlated-electron theories of superconductivity.

Oct 20, 20200 citations

U

and for degenerate orbitals. At half filling and large

U

, the ferromagnetic Hund's coupling,

{J}_{\mathrm{H}}

U=1.6

in units of the noninteracting bandwidth and for

{J}_{\mathrm{H}}/U\ensuremath{\gtrsim}0.275

The recent discovery of superconductivity under high pressure in the ladder compound

{\mathrm{BaFe}}_{2}{\mathrm{S}}_{3}

has opened a new field of research in iron-based superconductors with focus on quasi-one-dimensional geometries. In this publication, using the density matrix renormalization group technique, we study a two-orbital Hubbard model defined in one-dimensional chains. Our main result is the presence of hole binding tendencies at intermediate Hubbard

U

repulsion and robust Hund coupling

{J}_{H}/U=0.25

. Binding does not occur either in weak coupling or at very strong coupling. The pair-pair correlations that are dominant near half-filling, or of similar strength as the charge and spin correlation channels, involve hole-pair operators that are spin singlets, use nearest-neighbor sites, and employ different orbitals for each hole. The Hund coupling strength, presence of robust magnetic moments, and antiferromagnetic correlations among them are important for the binding tendencies found here.

Different models for doping of two-orbital chains with mobile

S=1/2

fermions and strong, ferromagnetic (FM) Hund's rule couplings stabilizing the S=1 spins are investigated by density matrix renormalization group (DMRG) methods. The competition between antiferromagnetic (AF) and FM order leads to a rich phase diagram with a narrow FM region for weak AF couplings and strongly enhanced triplet pairing correlations. Without a level difference between the orbitals, the spin gap persists upon doping, whereas gapless spin excitations are generated by interactions among itinerant polarons in the presence of a level difference. In the charge sector we find dominant singlet pairing correlations without a level difference, whereas upon the inclusion of a Coulomb repulsion between the orbitals or with a level difference, charge density wave (CDW) correlations decay slowest. The string correlation functions remain finite upon doping for all models.

1/2

Heisenberg model through the Kondo coupling

{J}_{K}

. When the density of electrons

x

is one, the Mott insulator is in a Haldane phase or in a rung-singlet phase depending on whether

{J}_{K}

is negative or positive. Upon doping, a pair-density-wave with $\mathbf{Q}=\ensuremath{\pi}$ can emerge for both signs of

{J}_{K}

. In the ${J}_{K}\ensuremath{\rightarrow}\ensuremath{-}\ensuremath{\infty}$ limit, the model reduces to the recently proposed type II $t\ensuremath{-}J$ model. We also identify a composite order parameter for the superconductor, which can be understood as a Cooper pair formed by two nearby fermionic spin-polarons. Our model and the predicted PDW phase can be experimentally realized by doping

S=1

chains formed by

{\mathrm{Ni}}^{2+}

in a solid-state system or a two-leg ladder of fermionic cold atoms with a potential bias between legs, which preferentially dopes carriers into a single leg. Long-range order of the PDW can be achieved in quasi-one-dimensional system with finite interwire coupling.

{\mathrm{CuO}}_{2}

layer. We demonstrate from accurate density matrix renormalization group studies the absence of the superconducting Luther-Emery phase in the doped 2-leg three-band ladder consisting of both copper and oxygen, even as the spin gap is large in the undoped three-band ladder. For realistic oxygen-oxygen hopping and Hubbard repulsion on the oxygen atoms, density-density rather than pairing correlations are dominant at long range. This result is equally valid whether or not the oxygens outside the ladder proper, over and above the rung and leg oxygens, are included in the computation. These results demonstrate the critical importance of oxygen orbitals, and raise disturbing questions about the applicability of many of the existing correlated-electron theories of superconductivity.